Diabolical points in the magnetic spectrum of Fe_8 molecules

The magnetic molecule Fe_8 has been predicted and observed to have a rich pattern of degeneracies in its spectrum as an external magnetic field is varied. These degeneracies have now been recognized to be diabolical points. This paper analyzes the diabolicity and all essential properties of this system using elementary perturbation theory. A variety of arguments is gievn to suggest that an earlier semiclassical result for a subset of these points may be exactly true for arbitrary spinComment: uses europhys.sty package; 3 embedded ps figure

Instanton picture of the spin tunneling in the Lipkin model

A consistent theory of the ground state energy and its splitting due to the process of tunneling for the Lipkin model is presented. For the functional integral in terms of the spin coherent states for the partition function of the model we accurately calculate the trivial and the instanton saddle point contributions. We show that such calculation has to be perfomed very accurately taking into account the discrete nature of the functional integral. Such accurate consideration leads to finite corrections to a naive continous consideration. We present comparison with numerical calculation of the ground state energy and the tunneling splitting and with the results obtained by the quasiclassical method and get excellent agreement.Comment: REVTEX, 32 pages, 3 figure

Static magnetization induced by time-periodic fields with zero mean

We consider a single spin in a constant magnetic field or an anisotropy field. We show that additional external time-periodic fields with zero mean may generate nonzero time-averaged spin components which are vanishing for the time-averaged Hamiltonian. The reason is a lowering of the dynamical symmetry of the system. A harmonic signal with proper orientation is enough to display the effect. We analyze the problem both with and without dissipation, both for quantum spins (s=1/2,1) and classical spins. The results are of importance for controlling the system's state using high or low frequency fields and for using new resonance techniques which probe internal system parameters, to name a few.Comment: 11 pages, 2 figure

Strong Coupling Theory of Two Level Atoms in Periodic Fields

We present a new convergent strong coupling expansion for two-level atoms in external periodic fields, free of secular terms. As a first application, we show that the coherent destruction of tunnelling is a third-order effect. We also present an exact treatment of the high-frequency region, and compare it with the theory of averaging. The qualitative frequency spectrum of the transition probability amplitude contains an effective Rabi frequency.Comment: 4 pages with 3 figure

Quantum-Classical Phase Transition of Escape rate in Biaxial Spin Particles

The escape rates of the biaxial single domain spin particles with and without an applied magnetic field are investigated. Using the strict potential field description of spin systems developed by Ulyanov and Zaslavskii we obtain new effective Hamiltonians which are considered to be in exact spin-coordinate correspondence unlike the well studied effective Hamiltonians with the approximate correspondence. The sharp first-order transition is found in both cases. The phase diagram of the transitions depending on the anisotropy constant and the external field is also given.Comment: 15 pages, 8 figure

Ising spin glass models versus Ising models: an effective mapping at high temperature III. Rigorous formulation and detailed proof for general graphs

Recently, it has been shown that, when the dimension of a graph turns out to be infinite dimensional in a broad sense, the upper critical surface and the corresponding critical behavior of an arbitrary Ising spin glass model defined over such a graph, can be exactly mapped on the critical surface and behavior of a non random Ising model. A graph can be infinite dimensional in a strict sense, like the fully connected graph, or in a broad sense, as happens on a Bethe lattice and in many random graphs. In this paper, we firstly introduce our definition of dimensionality which is compared to the standard definition and readily applied to test the infinite dimensionality of a large class of graphs which, remarkably enough, includes even graphs where the tree-like approximation (or, in other words, the Bethe-Peierls approach), in general, may be wrong. Then, we derive a detailed proof of the mapping for all the graphs satisfying this condition. As a byproduct, the mapping provides immediately a very general Nishimori law.Comment: 25 pages, 5 figures, made statements in Sec. 10 cleare

Quantum dynamics of crystals of molecular nanomagnets inside a resonant cavity

It is shown that crystals of molecular nanomagnets exhibit enhanced magnetic relaxation when placed inside a resonant cavity. Strong dependence of the magnetization curve on the geometry of the cavity has been observed, providing evidence of the coherent microwave radiation by the crystals. A similar dependence has been found for a crystal placed between Fabry-Perot superconducting mirrors. These observations open the possibility of building a nanomagnetic microwave laser pumped by the magnetic field

Nonequilibrium dynamics of a simple stochastic model

We investigate the low-temperature dynamics of a simple stochastic model, introduced recently in the context of the physics of glasses. The slowest characteristic time at equilibrium diverges exponentially at low temperature. On smaller time scales, the nonequilibrium dynamics of the system exhibits an aging regime. We present an analytical study of the scaling behaviour of the mean energy, of its local correlation and response functions, and of the associated fluctuation-dissipation ratio throughout the regime of low temperature and long times. This analysis includes the aging regime, the convergence to equilibrium, and the crossover behaviour between them.Comment: 36 pages, plain tex, 7 figures, to be published by Journal of Physics