3,479 research outputs found
Friction as Contrast Mechanism in Heterodyne Force Microscopy
The nondestructive imaging of subsurface structures on the nanometer scale
has been a long-standing desire in both science and industry. A few impressive
images were published so far that demonstrate the general feasibility by
combining ultrasound with an Atomic Force Microscope. From different excitation
schemes, Heterodyne Force Microscopy seems to be the most promising candidate
delivering the highest contrast and resolution. However, the physical contrast
mechanism is unknown, thereby preventing any quantitative analysis of samples.
Here we show that friction at material boundaries within the sample is
responsible for the contrast formation. This result is obtained by performing a
full quantitative analysis, in which we compare our experimentally observed
contrasts with simulations and calculations. Surprisingly, we can rule out all
other generally believed responsible mechanisms, like Rayleigh scattering,
sample (visco)elasticity, damping of the ultrasonic tip motion, and ultrasound
attenuation. Our analytical description paves the way for quantitative
SubSurface-AFM imaging.Comment: 7 pages main paper + 11 pages supplementary material
Inelastic semiclassical Coulomb scattering
We present a semiclassical S-matrix study of inelastic collinear
electron-hydrogen scattering. A simple way to extract all necessary information
from the deflection function alone without having to compute the stability
matrix is described. This includes the determination of the relevant Maslov
indices. Results of singlet and triplet cross sections for excitation and
ionization are reported. The different levels of approximation -- classical,
semiclassical, and uniform semiclassical -- are compared among each other and
to the full quantum result.Comment: 9 figure
Non-adiabatic molecular association in thermal gases driven by radio-frequency pulses
The molecular association process in a thermal gas of Rb is
investigated where the effects of the envelope of the radio-frequency field are
taken into account. For experimentally relevant parameters our analysis shows
that with increasing pulse length the corresponding molecular conversion
efficiency exhibits low-frequency interference fringes which are robust under
thermal averaging over a wide range of temperatures. This dynamical
interference phenomenon is attributed to St\"uckelberg phase accumulation
between the low-energy continuum states and the dressed molecular state which
exhibits a shift proportional to the envelope of the radio-frequency pulse
intensity.Comment: 5 pages, 3 figure
Ionization and charge migration through strong internal fields in clusters exposed to intense X-ray pulses
A general scenario for electronic charge migration in finite samples
illuminated by an intense laser pulse is given. Microscopic calculations for
neon clusters under strong short pulses as produced by X-ray free-electron
laser sources confirm this scenario and point to the prominent role of field
ionization by strong internal fields. The latter leads to the fast formation of
a core-shell system with an almost static core of screened ions while the outer
shell explodes. Substituting the shell ions with a different material such as
helium as a sacrificial layer leads to a substantial improvement of the
diffraction image for the embedded cluster thus reducing the consequences of
radiation damage for coherent diffractive imaging.Comment: 5 pages, 4 figure
Effects of precipitation uncertainty on discharge calculations for main river basins
This study quantifies the uncertainty in discharge calculations caused by uncertainty in precipitation input for 294 river basins worldwide. Seven global gridded precipitation datasets are compared at river basin scale in terms of mean annual and seasonal precipitation. The representation of seasonality is similar in all datasets, but the uncertainty in mean annual precipitation is large, especially in mountainous, arctic, and small basins. The average precipitation uncertainty in a basin is 30%, but there are strong differences between basins. The effect of this precipitation uncertainty on mean annual and seasonal discharge was assessed using the uncalibrated dynamic global vegetation and hydrology model Lund-Potsdam-Jena managed land (LPJmL), yielding even larger uncertainties in discharge (average 90%). For 95 basins (out of 213 basins for which measurements were available) calibration of model parameters is problematic because the observed discharge falls within the uncertainty of the simulated discharge. A method is presented to account for precipitation uncertainty in discharge simulations
Model- and Parameteroptimization for a Constitutive Law Describing Deformation Induced Anisotropy
 
Clusters under strong VUV pulses: A quantum-classical hybrid-description incorporating plasma effects
The quantum-classical hybrid-description of rare-gas clusters interacting
with intense light pulses which we have developed is described in detail. Much
emphasis is put on the treatment of screening electrons in the cluster which
set the time scale for the evolution of the system and form the link between
electrons strongly bound to ions and quasi-free plasma electrons in the
cluster. As an example we discuss the dynamics of an Ar147 cluster exposed to a
short VUV laser pulse of 20eV photon energy.Comment: 8 pages, 9 figure
Effects of precipitation uncertainty on discharge calculations for main river basins
This study quantifies the uncertainty in discharge calculations caused by uncertainty in precipitation input for 294 river basins worldwide. Seven global gridded precipitation datasets are compared at river basin scale in terms of mean annual and seasonal precipitation. The representation of seasonality is similar in all datasets, but the uncertainty in mean annual precipitation is large, especially in mountainous, arctic, and small basins. The average precipitation uncertainty in a basin is 30%, but there are strong differences between basins. The effect of this precipitation uncertainty on mean annual and seasonal discharge was assessed using the uncalibrated dynamic global vegetation and hydrology model Lund-Potsdam-Jena managed land (LPJmL), yielding even larger uncertainties in discharge (average 90%). For 95 basins (out of 213 basins for which measurements were available) calibration of model parameters is problematic because the observed discharge falls within the uncertainty of the simulated discharge. A method is presented to account for precipitation uncertainty in discharge simulations
Semiclassical initial value calculations of collinear helium atom
Semiclassical calculations using the Herman-Kluk initial value treatment are
performed to determine energy eigenvalues of bound and resonance states of the
collinear helium atom. Both the configuration (where the classical motion
is fully chaotic) and the configuration (where the classical dynamics is
nearly integrable) are treated. The classical motion is regularized to remove
singularities that occur when the electrons collide with the nucleus. Very good
agreement is obtained with quantum energies for bound and resonance states
calculated by the complex rotation method.Comment: 24 pages, 3 figures. Submitted to J. Phys.
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