Report of Workshop on Mount Saint Helens: Its Atmospheric Effects and Potential Climatic Impact

The atmospheric and potential climatic aspects of a volcanic eruption were discussed. Measurements and techniques used in collecting the data are summarized

Physical Mechanisms Controlling Upper Tropospheric Water Vapor as Revealed by MLS Data from UARS

The seasonal changes of the upper tropospheric humidity are studied with the water vapor data from the Microwave Limb Sounder on the NASA Upper Atmosphere Research Satellite, and the winds and vertical velocity data obtained from the European Centre for Medium-Range Weather Forecasts. Using the same algorithm for vertical transport as that used for horizontal transport (Zhu and Newell, 1998), we find that the moisture in the tropical upper troposphere may be increased mainly by intensified local convection in a small portion, less than 10%, of the whole area between 40 deg S to 40 deg N. The contribution of large scale background circulations and divergence of horizontal transport is relatively small in these regions. These dynamic processes cannot be revealed by the traditional analyses of moisture fluxes. The negative feedback suggested by Lindzen (1990) also exists, if enhanced convection is concentrated in the tropics, but is apparently not the dominant process in the moisture budget

Anomalous scaling of mesoscale tropospheric humidity fluctuations

Water vapor fluctuations are measured and analyzed at an unprecedented 10-m resolution throughout the troposphere. Computation of structure functions shows that specific humidity variations observed by research aircraft over the Pacific Ocean exhibit anomalous scaling from about 50 m to 100 km in horizontal range. The scaling laws show different characteristics for the marine boundary layer, the tropical free troposphere, and the extratropical free troposphere. More specifically, boundary-layer humidity fluctuations are less smooth and more stationary than those in the free troposphere, while the extratropical free tropospheric variations are less intermittent than those in the other two regions. The anomalous scaling results argue against passive advection by a spatially smooth flow (chaotic advection) at these scales.United States. National Aeronautics and Space Administration (Grant NAG1-2173)United States. National Aeronautics and Space Administration (Grant NAG1-1901

Horizontal wavenumber spectra of winds, temperature, and trace gases during the Pacific Exploratory Missions: 2. Gravity waves, quasi-two-dimensional turbulence, and vortical modes

We examine the horizontal wavenumber spectra of horizontal velocity and potential temperature collected by aircraft above the Pacific Ocean to determine whether gravity waves, quasi-two-dimensional (Q-2-D) turbulence, or vortical modes dominate atmospheric fluctuations at scale sizes of 1–100 km and altitudes of 2–12 km. We conclude from the study of Doppler-shifting effects that Q-2-D turbulence and/or vortical modes are more prevalent than gravity waves over the ocean, except in the equatorial zone. The results are consistent with recent numerical simulations of Q-2-D turbulence, which show that the characteristic inverse cascade of energy is greatly facilitated by the presence of background rotation. Furthermore, a Stokes-parameter analysis reveals the general paucity of coherent wavelike motions, although specific cases of gravity-wave propagation are observed. Finally, a case study of a long flight segment displays a k⁻³ horizontal velocity variance spectrum at scales longer than about 100 km. A Stokes-parameter analysis indicates that these large-scale fluctuations were likely due to vortical modes rather than inertio-gravity waves.United States. National Aeronautics and Space Administration (Grant NAG1-1758)United States. National Aeronautics and Space Administration (Grant NAG1-1901

Characterizations of tropospheric turbulence and stability layers from aircraft observations

[1] Velocity, temperature, and specific humidity data collected by aircraft at 20-Hz resolution are analyzed for stability and turbulence parameters. Over 100 vertical profiles (mostly over the ocean) with a total of over 300 km in vertical airspace sampled are used. The compiled statistics show that anisotropy in the velocity fluctuations prevail down to the smallest spatial separations measured. A partitioning of convective versus dynamical instability indicates that in the free troposphere, the ratio of shear-produced turbulence to convectively produced turbulence increases from roughly 2:1 for weak turbulence (ϵ 10⁻⁴ m² s⁻³). For the boundary layer, this ratio is close to 1:1 for weak turbulence and roughly 2:1 for strong turbulence. There is also a correlation between the strength of the vertical shear in horizontal winds and the turbulence intensity. In the free troposphere the turbulence intensity is independent of the degree of static stability, whereas in the boundary layer the turbulence intensity increases with a fall in static stability. Vertical humidity gradients correlate with static stability for strong humidity gradients, which supports the basic notion that stable layers impede vertical mixing of trace gases and aerosols. Vertical shear correlates with vertical humidity gradient, so it appears that the effect of differential advection creating tracer gradients dominates the effect of differential advection destroying tracer gradients through shear-induced turbulence.United States. National Aeronautics and Space Administration (Grant NCC1-415)United States. National Aeronautics and Space Administration (Grant NAG1-2306

Observation of pollution plume capping by a tropopause fold

Airborne lidar measurements reveal a case in which a layer of high-ozone air extruding from a tropopause fold appears to cap a pollution plume and force it to spread out in the lower troposphere. The morphology of the high-ozone layer resembles a three-dimensional model of tropopause fold evolution that produces a low-altitude potential vorticity tube. This is a mechanism that can complete the irreversible transfer of air from the stratosphere, and can also affect pollution levels at the surface if the capping layer reaches the top of the boundary layer.United States. National Aeronautics and Space Administration (Grant NAG1-2306

Horizontal wavenumber spectra of winds, temperature, and trace gases during the Pacific Exploratory Missions: 1. Climatology

Aircraft-based meteorological and chemical measurements from NASA's Pacific Exploratory Missions provide a suitable database for studying the climatology of horizontal wavenumber spectra in the troposphere overlying an ocean. The wavenumber spectra of trace gas and meteorological quantities aid in identifying the physical processes producing atmospheric structures as well as provide diagnostics for general circulation models. Flight segments were distributed over altitudes ranging from about ∼50 m to 13 km and 70°S to 60°N in latitude. The spectra were averaged according to altitude and latitude regions. The wavelength range covered was typically ∼0.5–100 km. Quantities processed in this way were horizontal velocity, potential temperature, specific humidity, and the mixing ratios of ozone, methane, carbon monoxide, and carbon dioxide. Spectral power and slope (in log-log coordinates) corresponding to the wavelength regime of 6–60 km were tabulated for those measured quantities. The spectral slopes of horizontal velocity and potential temperature were generally close to −5/3 with no transition to a steeper slope at short wavelengths as seen in some other studies. Spectral slopes of the tracer species also ranged around −5/3. This agreement in form of the dynamical and tracer spectra is consistent with both the gravity-wave advection and quasi two-dimensional turbulence models. In the upper troposphere the spectral power for all quantities except specific humidity tended to be greater at latitudes higher than 30° compared to latitudes lower than 30°. This latitudinal trend confirms the earlier results of the Global Atmospheric Sampling Program.United States. National Aeronautics and Space Administration (Grant NAG1-1758)United States. National Aeronautics and Space Administration (Grant NAG1-1901

Observations of convective and dynamical instabilities in tropopause folds and their contribution to stratosphere-troposphere exchange

With aircraft-mounted in situ and remote sensing instruments for dynamical, thermal, and chemical measurements we studied two cases of tropopause folding. In both folds we found Kelvin-Helmholtz billows with horizontal wavelength of ∼900 m and thickness of ∼120 m. In one case the instability was effectively mixing the bottomside of the fold, leading to the transfer of stratospheric air into the troposphere. Also, we discovered in both cases small-scale secondary ozone maxima shortly after the aircraft ascended past the topside of the fold that corresponded to regions of convective instability. We interpreted this phenomenon as convectively breaking gravity waves. Therefore we posit that convectively breaking gravity waves acting on tropopause folds must be added to the list of important irreversible mixing mechanisms leading to stratosphere-troposphere exchange.United States. National Aeronautics and Space Administration (Grant NAG2-1105)United States. National Aeronautics and Space Administration (Grant NAGl-1758)United States. National Aeronautics and Space Administration (Grant NAGl-1901

Ozone and aerosol distributions and air mass characteristics over the South Pacific during the burning season

In situ and laser remote measurements of gases and aerosols were made with airborne instrumentation to establish a baseline chemical signature of the atmosphere above the South Pacific Ocean during the NASA Global Tropospheric Experiment (GTE)/Pacific Exploratory Mission‐Tropics A (PEM‐Tropics A) conducted in August‐October 1996. This paper discusses general characteristics of the air masses encountered during this experiment using an airborne lidar system for measurements of the large‐scale variations in ozone (O3) and aerosol distributions across the troposphere, calculated potential vorticity (PV) from the European Centre for Medium‐Range Weather Forecasting (ECMWF), and in situ measurements for comprehensive air mass composition. Between 8°S and 52°S, biomass burning plumes containing elevated levels of O3, over 100 ppbv, were frequently encountered by the aircraft at altitudes ranging from 2 to 9 km. Air with elevated O3 was also observed remotely up to the tropopause, and these air masses were observed to have no enhanced aerosol loading. Frequently, these air masses had some enhanced PV associated with them, but not enough to explain the observed O3 levels. A relationship between PV and O3 was developed from cases of clearly defined O3 from stratospheric origin, and this relationship was used to estimate the stratospheric contribution to the air masses containing elevated O3 in the troposphere. The frequency of observation of the different air mass types and their average chemical composition is discussed in this paper

Large-scale ozone and aerosol distributions, air mass characteristics, and ozone fluxes over the western Pacific Ocean in late winter/early spring

Large‐scale measurements of ozone (O3) and aerosol distributions were made from the NASA DC‐8 aircraft during the Transport and Chemical Evolution over the Pacific (TRACE‐P) field experiment conducted in February–April 2001. Remote measurements were made with an airborne lidar to provide O3 and multiple‐wavelength aerosol backscatter profiles from near the surface to above the tropopause along the flight track. In situ measurements of O3, aerosols, and a wide range of trace gases were made onboard the DC‐8. Five‐day backward trajectories were used in conjunction with the O3 and aerosol distributions on each flight to indicate the possible origin of observed air masses, such as from biomass burning regions, continental pollution, desert regions, and oceanic regions. Average latitudinal O3 and aerosol scattering ratio distributions were derived from all flights west of 150°E, and these distributions showed the average latitude and altitude dependence of different dynamical and chemical processes in determining the atmospheric composition over the western Pacific. TRACE‐P (TP) showed an increase in the average latitudinal distributions of both O3 and aerosols compared to PEM‐West B (PWB), which was conducted in February–March 1994. O3, aerosol, and potential vorticity levels were used to identify nine air mass types and quantify their frequency of occurrence as a function of altitude. This paper discusses the characteristics of the different air mass types encountered during TP and compares them to PWB. These results confirmed that most of the O3 increase in TP was due to photochemistry. The average latitudinal eastward O3 flux in the western Pacific during TP was found to peak near 32°N with a total average O3 flux between 14 and 46°N of 5.2 Tg/day. The eastward total CO flux was calculated to be 2.2 Tg‐C/day with ∼6% estimated from Asia. The Asian flux of CO2 and CH4 was estimated at 4.9 and 0.06 Tg‐C/day