21,614 research outputs found
Electronic phase separation in the rare earth manganates, (La1-xLnx)0.7Ca0.3MnO3 (Ln = Nd, Gd and Y)
All the three series of manganates showsaturation magnetization
characteristic of ferromagnetism, with the ferromagnetic Tc decreasing with
increasing in x up to a critical value of x, xc (xc = 0.6, 0.3, 0.2
respectively for Nd, Gd, Y). For x > xc, the magnetic moments are considerably
smaller showing a small increase around TM, the value of TM decreasing slightly
with increase in x or decrease in . The ferromagnetic compositions (x xc)
show insulator-metal (IM) transitions, while the compositions with x > xc are
insulating. The magnetic and electrical resistivity behavior of these
manganates is consistent with the occurrence of phase separation in the
compositions around xc, corresponding to a critical average radius of the
A-site cation, , of 1.18 A. Both Tc and TIM increase linearly when < rA
> > or x xc as expected of a homogenous ferromagnetic phase. Both Tc
and TM decrease linearly with the A-site cation size disorder at the A-site as
measured by the variance s2. Thus, an increase in s2 favors the insulating AFM
state. Percolative conduction is observed in the compositions with > <
rAc >. Electron transport properties in the insulating regime for x > xc
conforms to the variable range hopping mechanism. More interestingly, when x >
xc, the real part of dielectric constant (e') reaches a high value (104-106) at
ordinary temperatures dropping to a very small (~500) value below a certain
temperature, the value of which decreases with decreasing frequency.Comment: 27 pages; 11 figures, Submitted to J.Phys:Condens Matte
Magnetic and electron transport properties of the rare-earth cobaltates, La0.7-xLnxCa0.3CoO3 (Ln = Pr, Nd, Gd and Dy) : A case of phase separation
Magnetic and electrical properties of four series of rare earth cobaltates of
the formula La0.7-xLnxCa0.3CoO3 with Ln = Pr, Nd, Gd and Dy have been
investigated. Compositions close to x = 0.0 contain large ferromagnetic
clusters or domains, and show Brillouin-like behaviour of the field-cooled DC
magnetization data with fairly high ferromagnetic Tc values, besides low
electrical resistivities with near-zero temperature coefficients. The
zero-field-cooled data generally show a non-monotonic behaviour with a peak at
a temperatures slightly lower than Tc. The near x = 0.0 compositions show a
prominent peak corresponding to the Tc in the AC-susceptibility data. The
ferromagnetic Tc varies linearly with x or the average radius of the A-site
cations, (rA). With increase in x or decrease in (rA), the magnetization value
at any given temperature decreases markedly and the AC-susceptibility
measurements show a prominent transition arising from small magnetic clusters
with some characteristics of a spin-glass. Electrical resistivity increases
with increase in x, showed a significant increase around a critical value of x
or (rA), at which composition the small clusters also begin to dominate. These
properties can be understood in terms of a phase separation scenario wherein
large magnetic clusters give way to smaller ones with increase in x, with both
types of clusters being present in certain compositions. The changes in
magnetic and electrical properties occur parallely since the large
ferromagnetic clusters are hole-rich and the small clusters are hole-poor.
Variable-range hopping seems to occur at low temperatures in these cobaltates.Comment: 23 pages including figure
Comment on ''the controlled charge ordering and evidence of the metallic state in PrCaMnO films''
In a recent paper (2000 \QTR{it}{J. Phys.: Condens. Matter} \QTR{bf}{12}
L133) Lee \QTR{it}{et al.} have studied the transport properties of
PrCaMnO thin films. They claimed that they are able to
controlled the charge-ordered (CO) state by the lattice strains. We propose
herein another alternative since another indexation of the orientation of the
film can be found leading to almost no distortion of the cell, as compared to
the bulk compound.Comment: 2 page
Interplay of 4f-3d Magnetism and Ferroelectricity in DyFeO3
DyFeO3 exhibits a weak ferromagnetism (TNFe ~ 645 K) that disappears below a
spin-reorientation (Morin) transition at TSRFe ~ 50 K. It is also known that
applied magnetic field induces ferroelectricity at the magnetic ordering
temperature of Dy-ions (TNDy ~ 4.5 K). Here, we show that the ferroelectricity
exists in the weak ferromagnetic state (TSRFe < T < TN,C) without applying
magnetic field, indicating the crucial role of weak ferromagnetism in inducing
ferroelectricity. 57Fe M\"ossbauer studies show that hyperfine field (Bhf)
deviates from mean field-like behaviour that is observed in the weak
ferromagnetic state and decreases below the onset of spin-reorientation
transition (80 K), implying that the Bhf above TSR had additional contribution
from Dy-ions due to induced magnetization by the weak ferromagnetic moment of
Fe-sublattice and below TSR, this contribution decreases due to collinear
ordering of Fe-sublattice. These results clearly demonstrate the presence of
magnetic interactions between Dy(4f) and Fe(3d) and their correlation with
ferroelectricity in the weak ferromagnetic state of DyFeO3.Comment: 5 pages, 6 figures, published in EP
On the instantaneous distribution of vertical velocity in the monsoon field and structure of the monsoon circulation
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Cyclogenesis in the Bay of Bengal and Arabian sea
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