Relativistic and topological domainwall signatures in spin space.

186 p

Multistep magnetization switching in orthogonally twisted ferromagnetic monolayers

The advent of twist-engineering in two-dimensional (2D) crystals enables the design of van der Waals (vdW) heterostructures exhibiting emergent properties. In the case of magnets, this approach can afford artificial antiferromagnets with tailored spin arrangements. Here, we fabricate an orthogonally-twisted bilayer by twisting 90 degrees two CrSBr ferromagnetic monolayers with an easy-axis in-plane anisotropy. The magneto-transport properties reveal multistep magnetization switching with a magnetic hysteresis opening, that is absent in the pristine case. By tuning the magnetic field, we modulate the remanent state and coercivity and select between hysteretic and non-hysteretic magneto-resistance scenarios. This complexity pinpoints spin anisotropy as a key aspect in twisted magnetic superlattices. Our results highlight the control over the magnetic properties in vdW heterostructures, leading to a variety of field-induced phenomena and opening a fruitful playground for creating desired magnetic symmetries and manipulating non-collinear magnetic configurations.Comment: Main Text + Supplementary Informatio

Inertial domain wall characterization in layered multisublattice antiferromagnets

The motion of a Neel-like 180 degrees domain wall induced by a time-dependent staggered spin-orbit field in the layered collinear antiferromagnet Mn2Au is explored. Through an effective version of the two sublattice nonlinear a-model which does not take into account the antiferromagnetic exchange interaction directed along the tetragonal c-axis, it is possible to replicate accurately the relativistic and inertial traces intrinsic to the magnetic texture dynamics obtained through atomistic spin dynamics simulations for quasistatic processes. In the case in which the steady-state magnetic soliton motion is extinguished due to the abrupt shutdown of the external stimulus, its stored relativistic exchange energy is transformed into a complex translational mobility, being the rigid domain wall profile approximation no longer suitable. Although it is not feasible to carry out a detailed follow-up of its temporal evolution in this case, it is possible to predict the inertial-based distance travelled by the domain wall in relation to its steady-state relativistic mass. This exhaustive dynamical characterization for different time-dependent regimes of the driving force is of potential interest in antiferromagnetic domain wall-based device applications.R.R.-E., K.Y.G., and R.M.O. thanks O. Chubykalo-Fesenko, S. Khmelevskyi, A. A. Sapozhnik, M. Jourdan, A. K. Zvezdin, and B. A. Ivanov for the fruitful discussions that have helped us to improve this manuscript. The work of R.M.O. and K.Y.G. was partially supported by the STSM Grants from the COST Action CA17123 "Ultrafast opto-magneto-electronics for non-dissipative information technology''. K.Y.G. acknowledges support by IKERBASQUE (the Basque Foundation for Science) and the Spanish Ministry of Science and Innovation under grant PID2019-108075RB-C33/AEI/10.13039/501100011033

Generalized form of the magnetic anisotropy field in micromagnetic and atomistic spin models

We present a general approach to the derivation of the effective anisotropy field which determines the dynamical behavior of magnetic spins according to the Landau-Lifshitz-Gilbert equation. The approach is based on the gradient in spherical polar coordinates with the final results being expressed in Cartesian coordinates as usually applied in atomistic and micromagnetic model calculations. The approach is generally valid for all orders of anisotropies including higher-order combinations of azimuthal and rotational anisotropies often found in functional magnetic materials such as permanent magnets and an emerging class of antiferromagnetic materials with applications in spintronics. Anisotropies are represented in terms of spherical harmonics which have the important property of rational temperature scaling. Effective field vectors are given for anisotropies up to sixth order, presenting a unified framework for implementing higher-order magnetic anisotropies in numerical simulations

Spin-dependent transport in diffusive systems with intrinsic spin-orbit coupling

Master in Nanoscience.Peer reviewe

Magnetic imaging and domain nucleation in CrSBr down to the 2D limit

Recent advancements in two-dimensional (2D) materials have revealed the potential of van der Waals magnets, and specifically of their magnetic anisotropy that allows applications down to the two-dimensional limit. Among these materials, CrSBr has emerged as a promising candidate, because its intriguing magnetic and electronic properties have appeal for both fundamental and applied research in spintronics or magnonics. Here, we use nano SQUID-on-tip (SOT) microscopy to obtain direct magnetic imaging of CrSBr flakes with thicknesses ranging from monolayer (N = 1) to few-layer (N = 5). The ferromagnetic order is preserved down to the monolayer, while the antiferromagnetic coupling of the layers starts from the bilayer case. For odd layers, at zero applied magnetic field, we directly image the stray field resulting from the uncompensated layer. We also measure the progressive spin reorientation along the out-of-plane direction (hard axis) with a finite applied magnetic field, allowing us to evaluate the anisotropy constant, which remains stable down to the monolayer and is close to the bulk value. Finally, by controlling the size of the applied magnetic field, we can observe the formation of Néel magnetic domain walls down to the single layer limit

Multistep magnetization switching in orthogonally twisted ferromagnetic monolayers

The authors present magnetotransport measurements to demonstrate multistep magnetization switching in orthogonally twisted CrSBr ferromagnetic monolayers.QN/vanderSarlabQN/van der Zant La