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Thesis (Ed.M.)--Boston Universit

Supercurrent Spectroscopy of Andreev States

We measure the excitation spectrum of a superconducting atomic contact. In addition to the usual continuum above the superconducting gap, the single particle excitation spectrum contains discrete, spin-degenerate Andreev levels inside the gap. Quasiparticle excitations are induced by a broadband on-chip microwave source and detected by measuring changes in the supercurrent flowing through the atomic contact. Since microwave photons excite quasiparticles in pairs, two types of transitions are observed: Andreev transitions, which consists of putting two quasiparticles in an Andreev level, and transitions to odd states with a single quasiparticle in an Andreev level and the other one in the continuum. In contrast to absorption spectroscopy, supercurrent spectroscopy allows detection of long-lived odd states.Comment: typos correcte

Exciting Andreev pairs in a superconducting atomic contact

The Josephson effect describes the flow of supercurrent in a weak link, such as a tunnel junction, nanowire, or molecule, between two superconductors. It is the basis for a variety of circuits and devices, with applications ranging from medicine to quantum information. Currently, experiments using Josephson circuits that behave like artificial atoms are revolutionizing the way we probe and exploit the laws of quantum physics. Microscopically, the supercurrent is carried by Andreev pair states, which are localized at the weak link. These states come in doublets and have energies inside the superconducting gap. Existing Josephson circuits are based on properties of just the ground state of each doublet and so far the excited states have not been directly detected. Here we establish their existence through spectroscopic measurements of superconducting atomic contacts. The spectra, which depend on the atomic configuration and on the phase difference between the superconductors, are in complete agreement with theory. Andreev doublets could be exploited to encode information in novel types of superconducting qubits.Comment: Submitted to Natur

Theory of microwave spectroscopy of Andreev bound states with a Josephson junction

We present a microscopic theory for the current through a tunnel Josephson junction coupled to a non-linear environment, which consists of an Andreev two-level system coupled to a harmonic oscillator. It models a recent experiment [Bretheau, Girit, Pothier, Esteve, and Urbina, Nature (London) 499, 312 (2013)] on photon spectroscopy of Andreev bound states in a superconducting atomic-size contact. We find the eigenenergies and eigenstates of the environment and derive the current through the junction due to inelastic Cooper pair tunneling. The current-voltage characteristic reveals the transitions between the Andreev bound states, the excitation of the harmonic mode that hybridizes with the Andreev bound states, as well as multi-photon processes. The calculated spectra are in fair agreement with the experimental data.Comment: 8 pages, 6 figure

Evidence for long-lived quasiparticles trapped in superconducting point contacts

We have observed that the supercurrent across phase-biased, highly transmitting atomic size contacts is strongly reduced within a broad phase interval around {\pi}. We attribute this effect to quasiparticle trapping in one of the discrete sub-gap Andreev bound states formed at the contact. Trapping occurs essentially when the Andreev energy is smaller than half the superconducting gap {\Delta}, a situation in which the lifetime of trapped quasiparticles is found to exceed 100 \mus. The origin of this sharp energy threshold is presently not understood.Comment: Article (5 pages) AND Supplemental material (14 pages). To be published in Physical Review Letter

Superconducting atomic contacts inductively coupled to a microwave resonator

We describe and characterize a microwave setup to probe the Andreev levels of a superconducting atomic contact. The contact is part of a superconducting loop inductively coupled to a superconducting coplanar resonator. By monitoring the resonator reflection coefficient close to its resonance frequency as a function of both flux through the loop and frequency of a second tone we perform spectroscopy of the transition between two Andreev levels of highly transmitting channels of the contact. The results indicate how to perform coherent manipulation of these states.Comment: 14 pages, 10 figures, to appear in special issue on break-junctions in JOPC

Dynamics of quasiparticle trapping in Andreev levels

We present a theory describing the trapping and untrapping of quasiparticles in the Andreev bound level of a single-channel weak link between two superconductors. We calculate the rates of the transitions between even and odd occupations of the Andreev level induced by absorption and emission of both photons and phonons. We apply the theory to a recent experiment [Phys. Rev. Lett. 106, 257003 (2011)] in which the dynamics of the trapping of quasiparticles in the Andreev levels of superconducting atomic contacts coupled to a Josephson junction was measured. We show that the plasma energy $h\nu_p$ of the Josephson junction defines a rather abrupt transition between a fast relaxation regime dominated by coupling to photons and a slow relaxation regime dominated by coupling to phonons. With realistic parameters the theory provides a semi-quantitative description of the experimental results.Comment: 11 pages, 9 figures. Accepted for publication in Physical Review

Adiabatic pumping through interacting quantum dots

We present a general formalism to study adiabatic pumping through interacting quantum dots. We derive a formula that relates the pumped charge to the local, instantaneous Green function of the dot. This formula is then applied to the infinite-U Anderson model both for weak and strong tunnel-coupling strengths.Comment: 4 pages, 3 figure

Radio-Frequency Single-Electron Refrigerator

We propose a cyclic refrigeration principle based on mesoscopic electron transport. Synchronous sequential tunnelling of electrons in a Coulomb-blockaded device, a normal metal-superconductor single-electron box, results in a cooling power of $\sim k_{\rm B}T \times f$ at temperature $T$ over a wide range of cycle frequencies $f$. Electrostatic work, done by the gate voltage source, removes heat from the Coulomb island with an efficiency of $\sim k_{\rm B}T/\Delta$, where $\Delta$ is the superconducting gap. The performance is not affected significantly by non-idealities, for instance by offset charges. We propose ways of characterizing the system and of its practical implementation.Comment: 5 pages, 4 figures; corrected typos, language improve

Measurement of the current-phase relation of superconducting atomic contacts

We have probed the current-phase relation of an atomic contact placed with a tunnel junction in a small superconducting loop. The measurements are in quantitative agreement with the predictions of a resistively shunted SQUID model in which the Josephson coupling of the contact is calculated using the independently determined transmissions of its conduction channels.Comment: to be published in Physical Review Letter