278 research outputs found
A two-dimensional, two-electron model atom in a laser pulse: exact treatment, single active electron-analysis, time-dependent density functional theory, classical calculations, and non-sequential ionization
Owing to its numerical simplicity, a two-dimensional two-electron model atom,
with each electron moving in one direction, is an ideal system to study
non-perturbatively a fully correlated atom exposed to a laser field. Frequently
made assumptions, such as the ``single active electron''- approach and
calculational approximations, e.g. time dependent density functional theory or
(semi-) classical techniques, can be tested. In this paper we examine the
multiphoton short pulse-regime. We observe ``non-sequential'' ionization, i.e.\
double ionization at lower field strengths as expected from a sequential,
single active electron-point of view. Since we find non-sequential ionization
also in purely classical simulations, we are able to clarify the mechanism
behind this effect in terms of single particle trajectories. PACS Number(s):
32.80.RmComment: 10 pages, 16 figures (gzipped postscript), see also
http://www.physik.tu-darmstadt.de/tqe
Lower entropy bounds and particle number fluctuations in a Fermi sea
We demonstrate, in an elementary manner, that given a partition of the single
particle Hilbert space into orthogonal subspaces, a Fermi sea may be factored
into pairs of entangled modes, similar to a BCS state. We derive expressions
for the entropy and for the particle number fluctuations of a subspace of a
fermi sea, at zero and finite temperatures, and relate these by a lower bound
on the entropy. As an application we investigate analytically and numerically
these quantities for electrons in the lowest Landau level of a quantum Hall
sample.Comment: shorter version, typos fixe
Energy levels and lifetimes of Gd IV and enhancement of the electron dipole moment
We have calculated energy levels and lifetimes of 4f7 and 4f6 5d
configurations of Gd IV using Hartree-Fock and configuration interaction
methods. This allows us to reduce significantly the uncertainty of the
theoretical determination of the electron electric dipole moment (EDM)
enhancement factor in this ion and, correspondingly, in gadolinium-containing
garnets for which such measurements were recently proposed. Our new value for
the EDM enhancement factor of Gd+3 is -2.2 +- 0.5. Calculations of energy
levels and lifetimes for Eu~III are used to control the accuracy.Comment: Submitted to Phys. Rev. A 6 pages, 0 figures, 3 table
Ionization state, excited populations and emission of impurities in dynamic finite density plasmas: I. The generalized collisional-radiative model for light elements
The paper presents an integrated view of the population structure and its role in establishing the ionization state of light elements in dynamic, finite density, laboratory and astrophysical plasmas. There are four main issues, the generalized collisional-radiative picture for metastables in dynamic plasmas with Maxwellian free electrons and its particularizing to light elements, the methods of bundling and projection for manipulating the population equations, the systematic production/use of state selective fundamental collision data in the metastable resolved picture to all levels for collisonal-radiative modelling and the delivery of appropriate derived coefficients for experiment analysis. The ions of carbon, oxygen and neon are used in illustration. The practical implementation of the methods described here is part of the ADAS Project
Dielectronic Recombination of Argon-Like Ions
We present a theoretical investigation of dielectronic recombination (DR) of
Ar-like ions that sheds new light on the behavior of the rate coefficient at
low-temperatures where these ions form in photoionized plasmas. We provide
results for the total and partial Maxwellian-averaged DR rate coefficients from
the initial ground level of K II -- Zn XIII ions. It is expected that these new
results will advance the accuracy of the ionization balance for Ar-like M-shell
ions and pave the way towards a detailed modeling of astrophysically relevant
X-ray absorption features. We utilize the AUTOSTRUCTURE computer code to obtain
the accurate core-excitation thresholds in target ions and carry out
multiconfiguration Breit-Pauli (MCBP) calculations of the DR cross section in
the independent-processes, isolated-resonance, distorted-wave (IPIRDW)
approximation. Our results mediate the complete absence of direct DR
calculations for certain Ar-like ions and question the reliability of the
existing empirical rate formulas, often inferred from renormalized data within
this isoelectronic sequence
Dielectronic recombination data for dynamic finite-density plasmas I. Goals and methodology
A programme is outlined for the assembly of a comprehensive dielectronic
recombination database within the generalized collisional--radiative (GCR)
framework. It is valid for modelling ions of elements in dynamic finite-density
plasmas such as occur in transient astrophysical plasmas such as solar flares
and in the divertors and high transport regions of magnetic fusion devices. The
resolution and precision of the data are tuned to spectral analysis and so are
sufficient for prediction of the dielectronic recombination contributions to
individual spectral line emissivities. The fundamental data are structured
according to the format prescriptions of the Atomic Data and Analysis Structure
(ADAS) and the production of relevant GCR derived data for application is
described and implemented following ADAS. The requirements on the dielectronic
recombination database are reviewed and the new data are placed in context and
evaluated with respect to older and more approximate treatments. Illustrative
results validate the new high-resolution zero-density dielectronic
recombination data in comparison with measurements made in heavy-ion storage
rings utilizing an electron cooler. We also exemplify the role of the
dielectronic data on GCR coefficient behaviour for some representative light
and medium weight elements.Comment: 14 Pages, 9 Figures. Submitted to Astronomy & Astrophysics April 12,
200
Convergent calculations of positron scattering from molecular hydrogen
An overview is given of the recently developed adiabatic-nuclei convergent closecoupling method for positron-molecule scattering. Fixed-nuclei single-centre calculations of positron-H2 scattering are presented. Particular emphasis is given to demonstrating convergence with increasing size of the basis and the projectile partial-wave expansion. Results are converged to within ±5%
Threshold detachment of negative ions by electron impact
The description of threshold fragmentation under long range repulsive forces
is presented. The dominant energy dependence near threshold is isolated by
decomposing the cross section into a product of a back ground part and a
barrier penetration probability resulting from the repulsive Coulomb
interaction. This tunneling probability contains the dominant energy variation
and it can be calculated analytically based on the same principles as Wannier's
description for threshold ionization under attractive forces. Good agreement is
found with the available experimental cross sections on detachment by electron
impact from , and .Comment: 4 pages, 4 figures (EPS), to appear in Phys.Rev.Lett, Feb. 22nd, 199
A large-scale R-matrix calculation for electron-impact excitation of the Ne O-like ion
The five J levels within a or ground state complex provide
an excellent testing ground for the comparison of theoretical line ratios with
astrophysically observed values, in addition to providing valuable electron
temperature and density diagnostics. The low temperature nature of the line
ratios ensure that the theoretically derived values are sensitive to the
underlying atomic structure and electron-impact excitation rates. Previous
R-matrix calculations for the Ne O-like ion exhibit large spurious
structure in the cross sections at higher electron energies, which may affect
Maxwellian averaged rates even at low temperatures. Furthermore, there is an
absence of comprehensive excitation data between the excited states that may
provide newer diagnostics to compliment the more established lines discussed in
this paper. To resolve these issues, we present both a small scale 56-level
Breit-Pauli (BP) calculation and a large-scale 554 levels R-matrix Intermediate
Coupling Frame Transformation (ICFT) calculation that extends the scope and
validity of earlier JAJOM calculations both in terms of the atomic structure
and scattering cross sections. Our results provide a comprehensive
electron-impact excitation data set for all transitions to higher shells.
The fundamental atomic data for this O-like ion is subsequently used within a
collisional radiative framework to provide the line ratios across a range of
electron temperatures and densities of interest in astrophysical observations.Comment: 17 pages, 8 figure
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Electron-Impact Ionization of Be-like C III, N IV, and O V
We present recent measurements of absolute electron-impact ionization cross sections for Be-like C III, N IV, and O V forming Li-like C IV, N V, and O VI. The measurements were taken using the crossed-beams apparatus at Oak Ridge National Laboratory. A gas cell beam attenuation method was used to independently measure the metastable fractions present in the ion beams. The measured ionization cross sections were compared with calculations using the R-matrix with pseudostates and distorted-wave theoretical methods. Best agreement is found with the R-matrix with pseudostates cross sections results that account for the metastable fractions inferred from the gas attenuation measurements. We present a set of recommended rate coefficients for electron-impact single ionization from the ground state and metastable term of each ion
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