777 research outputs found
Solid-solid phase transition in hard ellipsoids
We present a computer simulation study of the crystalline phases of hard
ellipsoids of revolution. A previous study [Phys. Rev. E, \textbf{75}, 020402
(2007)] showed that for aspect ratios the previously suggested
stretched-fcc phase [Mol. Phys., \textbf{55}, 1171 (1985)] is unstable with
respect to a simple monoclinic phase with two ellipsoids of different
orientations per unit cell (SM2). In order to study the stability of these
crystalline phases at different aspect ratios and as a function of density we
have calculated their free energies by thermodynamic integration. The
integration path was sampled by an expanded ensemble method in which the
weights were adjusted by the Wang-Landau algorithm.
We show that for aspect ratios the SM2 structure is more stable
than the stretched-fcc structure for all densities above solid-nematic
coexistence. Between and our calculations reveal a
solid-solid phase transition
Novel crystal phase in suspensions of hard ellipsoids
We present a computer simulation study on the crystalline phases of hard
ellipsoids of revolution. For aspect ratios greater than or equal to 3 the
previously suggested stretched-fcc phase [D. Frenkel and B. M. Mulder, Mol.
Phys. 55, 1171 (1985)] is replaced by a novel crystalline phase. Its unit cell
contains two ellipsoids with unequal orientations. The lattice is simple
monoclinic. The angle of inclination of the lattice, beta, is a very soft
degree of freedom, while the two right angles are stiff. For one particular
value of beta, the close-packed version of this crystal is a specimen of the
family of superdense packings recently reported [Donev et al., Phys. Rev. Lett.
92, 255506 (2004)]. These results are relevant for studies of nucleation and
glassy dynamics of colloidal suspensions of ellipsoids.Comment: 4 pages, 4 figure
Quantum Phase Transitions in the Itinerant Ferromagnet ZrZn
We report a study of the ferromagnetism of ZrZn, the most promising
material to exhibit ferromagnetic quantum criticality, at low temperatures
as function of pressure . We find that the ordered ferromagnetic moment
disappears discontinuously at =16.5 kbar. Thus a tricritical point
separates a line of first order ferromagnetic transitions from second order
(continuous) transitions at higher temperature. We also identify two lines of
transitions of the magnetisation isotherms up to 12 T in the plane where
the derivative of the magnetization changes rapidly. These quantum phase
transitions (QPT) establish a high sensitivity to local minima in the free
energy in ZrZn, thus strongly suggesting that QPT in itinerant
ferromagnets are always first order
Parasitic small-moment-antiferromagnetism and non-linear coupling of hidden order and antiferromagnetism in URu2Si2 observed by Larmor diffraction
We report simultaneous measurements of the distribution of lattice constants
and the antiferromagnetic moment in high-purity URu2Si2, using both Larmor and
conventional neutron diffraction, as a function of temperature and pressure up
to 18 kbar. We establish that the tiny moment in the hidden order (HO) state is
purely parasitic and quantitatively originates from the distribution of lattice
constants. Moreover, the HO and large-moment antiferromagnetism (LMAF) at high
pressure are separated by a line of first-order phase transitions, which ends
in a bicritical point. Thus the HO and LMAF are coupled non-linearly and must
have different symmetry, as expected of the HO being, e.g., incommensurate
orbital currents, helicity order, or multipolar order.Comment: 4 pages, 4 figure
The quantum phase transition of itinerant helimagnets
We investigate the quantum phase transition of itinerant electrons from a
paramagnet to a state which displays long-period helical structures due to a
Dzyaloshinskii instability of the ferromagnetic state. In particular, we study
how the self-generated effective long-range interaction recently identified in
itinerant quantum ferromagnets is cut-off by the helical ordering. We find that
for a sufficiently strong Dzyaloshinskii instability the helimagnetic quantum
phase transition is of second order with mean-field exponents. In contrast, for
a weak Dzyaloshinskii instability the transition is analogous to that in
itinerant quantum ferromagnets, i.e. it is of first order, as has been observed
in MnSi.Comment: 5 pages RevTe
Imaging and manipulation of skyrmion lattice domains in Cu2OSeO3
Nanoscale chiral skyrmions in noncentrosymmetric helimagnets are promising
binary state variables in high-density, low-energy nonvolatile memory.
Skyrmions are ubiquitous as an ordered, single-domain lattice phase, which
makes it difficult to write information unless they are spatially broken up
into smaller units, each representing a bit. Thus, the formation and
manipulation of skyrmion lattice domains is a prerequisite for memory
applications. Here, using an imaging technique based on resonant magnetic x-ray
diffraction, we demonstrate the mapping and manipulation of skyrmion lattice
domains in Cu2OSeO3. The material is particularly interesting for applications
owing to its insulating nature, allowing for electric field-driven domain
manipulation.Comment: 4 pages, 3 figure
Uniaxial pressure dependence of magnetic order in MnSi
We report comprehensive small angle neutron scattering (SANS) measurements
complemented by ac susceptibility data of the helical order, conical phase and
skyrmion lattice phase (SLP) in MnSi under uniaxial pressures. For all
crystallographic orientations uniaxial pressure favours the phase for which a
spatial modulation of the magnetization is closest to the pressure axis.
Uniaxial pressures as low as 1kbar applied perpendicular to the magnetic field
axis enhance the skyrmion lattice phase substantially, whereas the skyrmion
lattice phase is suppressed for pressure parallel to the field. Taken together
we present quantitative microscopic information how strain couples to magnetic
order in the chiral magnet MnSi.Comment: 23 pages, includes supplemen
Reciprocal space mapping of magnetic order in thick epitaxial MnSi films
We report grazing incidence small angle neutron scattering (GISANS) and
complementary off-specular neutron reflectometry (OSR) of the magnetic order in
a single-crystalline epitaxial MnSi film on Si(111) in the thick film limit.
Providing a means of direct reciprocal space mapping, GISANS and OSR reveal a
magnetic modulation perpendicular to the films under magnetic fields parallel
and perpendicular to the film, where additional polarized neutron reflectometry
(PNR) and magnetization measurements are in excellent agreement with the
literature. Regardless of field orientation, our data does not suggest the
presence of more complex spin textures, notably the formation of skyrmions.
This observation establishes a distinct difference with bulk samples of MnSi of
similar thickness under perpendicular field, in which a skyrmion lattice
dominates the phase diagram. Extended x-ray absorption fine structure
measurements suggest that small shifts of the Si positions within the
unstrained unit cell control the magnetic state, representing the main
difference between the films and thin bulk samples
Quantum Tricritical Points in NbFe
Quantum critical points (QCPs) emerge when a 2nd order phase transition is
suppressed to zero temperature. In metals the quantum fluctuations at such a
QCP can give rise to new phases including unconventional superconductivity.
Whereas antiferromagnetic QCPs have been studied in considerable detail
ferromagnetic (FM) QCPs are much harder to access. In almost all metals FM QCPs
are avoided through either a change to 1st order transitions or through an
intervening spin-density-wave (SDW) phase. Here, we study the prototype of the
second case, NbFe. We demonstrate that the phase diagram can be modelled
using a two-order-parameter theory in which the putative FM QCP is buried
within a SDW phase. We establish the presence of quantum tricritical points
(QTCPs) at which both the uniform and finite susceptibility diverge. The
universal nature of our model suggests that such QTCPs arise naturally from the
interplay between SDW and FM order and exist generally near a buried FM QCP of
this type. Our results promote NbFe as the first example of a QTCP, which
has been proposed as a key concept in a range of narrow-band metals, including
the prominent heavy-fermion compound YbRhSi.Comment: 21 pages including S
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