28 research outputs found
Ab Initio Spatial Phase Retrieval via Fluorescence Intensity Triple Correlations
A complete method for ab initio phase retrieval via spatial intensity triple correlations is described. Simulations demonstrate accurate phase retrieval for clusters of classical incoherent emitters
Ab Initio Spatial Phase Retrieval via Fluorescence Intensity Triple Correlations
A complete method for ab initio phase retrieval via spatial intensity triple
correlations is described. Simulations demonstrate accurate phase retrieval for
clusters of classical incoherent emitters
Collapsing lattice animals and lattice trees in two dimensions
We present high statistics simulations of weighted lattice bond animals and
lattice trees on the square lattice, with fugacities for each non-bonded
contact and for each bond between two neighbouring monomers. The simulations
are performed using a newly developed sequential sampling method with
resampling, very similar to the pruned-enriched Rosenbluth method (PERM) used
for linear chain polymers. We determine with high precision the line of second
order transitions from an extended to a collapsed phase in the resulting
2-dimensional phase diagram. This line includes critical bond percolation as a
multicritical point, and we verify that this point divides the line into two
different universality classes. One of them corresponds to the collapse driven
by contacts and includes the collapse of (weakly embeddable) trees, but the
other is {\it not yet} bond driven and does not contain the Derrida-Herrmann
model as special point. Instead it ends at a multicritical point where a
transition line between two collapsed phases (one bond-driven and the other
contact-driven) sparks off. The Derrida-Herrmann model is representative for
the bond driven collapse, which then forms the fourth universality class on the
transition line (collapsing trees, critical percolation, intermediate regime,
and Derrida-Herrmann). We obtain very precise estimates for all critical
exponents for collapsing trees. It is already harder to estimate the critical
exponents for the intermediate regime. Finally, it is very difficult to obtain
with our method good estimates of the critical parameters of the
Derrida-Herrmann universality class. As regards the bond-driven to
contact-driven transition in the collapsed phase, we have some evidence for its
existence and rough location, but no precise estimates of critical exponents.Comment: 11 pages, 16 figures, 1 tabl
Simulations of lattice animals and trees
The scaling behaviour of randomly branched polymers in a good solvent is
studied in two to nine dimensions, using as microscopic models lattice animals
and lattice trees on simple hypercubic lattices. As a stochastic sampling
method we use a biased sequential sampling algorithm with re-sampling, similar
to the pruned-enriched Rosenbluth method (PERM) used extensively for linear
polymers. Essentially we start simulating percolation clusters (either site or
bond), re-weigh them according to the animal (tree) ensemble, and prune or
branch the further growth according to a heuristic fitness function. In
contrast to previous applications of PERM, this fitness function is {\it not}
the weight with which the actual configuration would contribute to the
partition sum, but is closely related to it. We obtain high statistics of
animals with up to several thousand sites in all dimension 2 <= d <= 9. In
addition to the partition sum (number of different animals) we estimate
gyration radii and numbers of perimeter sites. In all dimensions we verify the
Parisi-Sourlas prediction, and we verify all exactly known critical exponents
in dimensions 2, 3, 4, and >= 8. In addition, we present the hitherto most
precise estimates for growth constants in d >= 3. For clusters with one site
attached to an attractive surface, we verify the superuniversality of the
cross-over exponent at the adsorption transition predicted by Janssen and
Lyssy. Finally, we discuss the collapse of animals and trees, arguing that our
present version of the algorithm is also efficient for some of the models
studied in this context, but showing that it is {\it not} very efficient for
the `classical' model for collapsing animals.Comment: 17 pages RevTeX, 29 figures include
Transient vibration and product formation of photoexcited CS2 measured by time-resolved x-ray scattering
We have observed details of the internal motion and dissociation channels in photoexcited carbon disulfide (CS<sub>2</sub>) using time-resolved x-ray scattering (TRXS). Photoexcitation of gas-phase CS<sub>2</sub> with a 200 nm laser pulse launches oscillatory bending and stretching motion, leading to dissociation of atomic sulfur in under a picosecond. During the first 300 fs following excitation, we observe significant changes in the vibrational frequency as well as some dissociation of the C-S bond, leading to atomic sulfur in the both <sup>1</sup>D and <sup>3</sup>P states. Beyond 1400 fs, the dissociation is consistent with primarily <sup>3</sup>P atomic sulfur dissociation. This channel-resolved measurement of the dissociation time is based on our analysis of the time-windowed dissociation radial velocity distribution, which is measured using the temporal Fourier transform of the TRXS data aided by a Hough transform that extracts the slopes of linear features in an image. The relative strength of the two dissociation channels reflects both their branching ratio and differences in the spread of their dissociation times. Measuring the time-resolved dissociation radial velocity distribution aids the resolution of discrepancies between models for dissociation proposed by prior photoelectron spectroscopy work