Redundancy of classical and quantum correlations during decoherence

We analyze the time dependence of entanglement and total correlations between a system and fractions of its environment in the course of decoherence. For the quantum Brownian motion model we show that the entanglement and total correlations have rather different dependence on the size of the environmental fraction. Redundancy manifests differently in both types of correlations and can be related with induced--classicality. To study this we introduce a new measure of redundancy and compare it with the existing one.Comment: 6 pages, 4 figure

Aerosol-assisted metallo-organic chemical vapour deposition of Bi2Se3 films using single-molecule precursors: the crystal structure of bismuth(m) dibutyldiselenocarbamate

The complexes [Bi{Se2CN(C2H5)2}3], [Bi{Se2CN(C4H9)2}3], [Bi{Se2CN(CH3)(C4H9)}3] and [Bi{Se2CN(CH3)(C6H13)}3] have been synthesized and characterized structurally using IR, 1H and 13C NMR. In addition, the crystal structure of [Bi{Se2CN(C4H9)2}3] was determined by single-crystal X-ray diffraction, showing the bismuth centre coordinated to three dialkyldiselenocarbamate ligands through the selenium donor atoms. The Bi(III) compounds were used as precursors for the deposition of Bi2Se3 films on glass substrates through aerosol-assisted metallo-organic chemical vapour deposition (AA-MOCVD)

The first dinuclear zinc(II) dithiocarbarnate complex with butyl substituent groups

The crystal structure of the title compound, bis( -N,N- dibutyldithiocarbamato- 2S:S0)bis[(N,N-dibutyldithiocarba\- forcelb]mato- 2S,S0)zinc(II)], [Zn2(C9H18NS2)4], has been determined at 180 K. The structure contains two crystallographically unique Zn2+ metal centres, showing almost identical slightly distorted tetrahedral coordination environments, and forming a dinuclear complex with two skew-bridging syn-N,N-dibutyldithiocarbamate ligands. Two other dithiocarbamate ligands are connected to the Zn2+ centres in a syn,syn-chelate coordination mode

A Method for Modeling Decoherence on a Quantum Information Processor

We develop and implement a method for modeling decoherence processes on an N-dimensional quantum system that requires only an $N^2$-dimensional quantum environment and random classical fields. This model offers the advantage that it may be implemented on small quantum information processors in order to explore the intermediate regime between semiclassical and fully quantum models. We consider in particular $\sigma_z\sigma_z$ system-environment couplings which induce coherence (phase) damping, though the model is directly extendable to other coupling Hamiltonians. Effective, irreversible phase-damping of the system is obtained by applying an additional stochastic Hamiltonian on the environment alone, periodically redressing it and thereby irreversibliy randomizing the system phase information that has leaked into the environment as a result of the coupling. This model is exactly solvable in the case of phase-damping, and we use this solution to describe the model's behavior in some limiting cases. In the limit of small stochastic phase kicks the system's coherence decays exponentially at a rate which increases linearly with the kick frequency. In the case of strong kicks we observe an effective decoupling of the system from the environment. We present a detailed implementation of the method on an nuclear magnetic resonance quantum information processor.Comment: 12 pages, 9 figure

Decoherence and the rate of entropy production in chaotic quantum systems

We show that for an open quantum system which is classically chaotic (a quartic double well with harmonic driving coupled to a sea of harmonic oscillators) the rate of entropy production has, as a function of time, two relevant regimes: For short times it is proportional to the diffusion coefficient (fixed by the system--environment coupling strength). For longer times (but before equilibration) there is a regime where the entropy production rate is fixed by the Lyapunov exponent. The nature of the transition time between both regimes is investigated.Comment: Revtex, 4 pages, 3 figures include

Quantum effects after decoherence in a quenched phase transition

We study a quantum mechanical toy model that mimics some features of a quenched phase transition. Both by virtue of a time-dependent Hamiltonian or by changing the temperature of the bath we are able to show that even after classicalization has been reached, the system may display quantum behaviour again. We explain this behaviour in terms of simple non-linear analysis and estimate relevant time scales that match the results of numerical simulations of the master-equation. This opens new possibilities both in the study of quantum effects in non-equilibrium phase transitions and in general time-dependent problems where quantum effects may be relevant even after decoherence has been completed.Comment: 7 pages, 7 figures, revtex, important revisions made. To be published in Phys. Rev.

Classical Dynamics of the Quantum Harmonic Chain

The origin of classical predictability is investigated for the one dimensional harmonic chain considered as a closed quantum mechanical system. By comparing the properties of a family of coarse-grained descriptions of the chain, we conclude that local coarse-grainings in this family are more useful for prediction than nonlocal ones. A quantum mechanical system exhibits classical behavior when the probability is high for histories having the correlations in time implied by classical deterministic laws. But approximate classical determinism holds only for certain coarse-grainings and then only if the initial state of the system is suitably restricted. Coarse-grainings by the values of the hydrodynamic variables (integrals over suitable volumes of densities of approximately conserved quantities) define the histories usually used in classical physics. But what distinguishes this coarse-graining from others? This paper approaches this question by analyzing a family of coarse-grainings for the linear harmonic chain. At one extreme in the family the chain is divided into local groups of $N$ atoms. At the other extreme the $N$ atoms are distributed nonlocally over the whole chain. Each coarse-graining follows the average (center of mass) positions of the groups and ignores the ``internal'' coordinates within each group, these constituting a different environment for each coarse-graining. We conclude that noise, decoherence, and computational complexity favor locality over nonlocality for deterministic predictability.Comment: 38 pages RevTeX 3.0 + 4 figures (postscript). Numerous minor corrections. Submitted to Physical Review

Adaptive Optics Imaging of IRAS 18276-1431: a bipolar pre-planetary nebula with circumstellar "searchlight beams" and "arcs"

We present high-angular resolution images of the post-AGB nebula IRAS18276-1431 (also known as OH17.7-2.0) obtained with the Keck II Adaptive Optics (AO) system in its Natural Guide Star (NGS) mode in the Kp, Lp, and Ms near-infrared bands. We also present supporting optical F606W and F814W HST images as well as interferometric observations of the 12CO(J=1-0), 13CO(J=1-0), and 2.6mm continuum emission with OVRO. The envelope of IRAS18276-1431 displays a clear bipolar morphology in our optical and NIR images with two lobes separated by a dark waist and surrounded by a faint 4.5"x3.4" halo. Our Kp-band image reveals two pairs of radial ``searchlight beams'' emerging from the nebula center and several intersecting, arc-like features. From our CO data we derive a mass of M>0.38[D/3kpc]^2 Msun and an expansion velocity v_exp=17km/s for the molecular envelope. The density in the halo follows a radial power-law proportional to r^-3, which is consistent with a mass-loss rate increasing with time. Analysis of the NIR colors indicates the presence of a compact central source of ~300-500K dust illuminating the nebula in addition to the central star. Modeling of the thermal IR suggests a two-shell structure in the dust envelope: 1) an outer shell with inner and outer radius R_in~1.6E16cm and R_out>~1.25E17cm, dust temperature T_d~105-50K, and a mean mass-loss rate of Mdot~1E-3Msun/yr; and 2) an inner shell with R_in~6.3E14cm, T_dust~500-105K, and Mdot~3E-5Msun/yr. An additional population of big dust grains (radius a>~0.4mm) with T_dust=150-20K and mass M_dust=(0.16-1.6)E-3 [D/3kpc]^2 Msun can account for the observed sub-mm and mm flux excess. The mass of the envelope enclosed within R_out=1.25E17cm derived from SED modeling is ~1[D/3kpc]^2 Msun.Comment: 46 pages, 14 figures, 3 tables, accepted for publication in ApJ. Figures 12 & 13 in low resolution. Full resolution versions are available upon request to the first autho

Decoherence suppression via environment preparation

To protect a quantum system from decoherence due to interaction with its environment, we investigate the existence of initial states of the environment allowing for decoherence-free evolution of the system. For models in which a two-state system interacts with a dynamical environment, we prove that such states exist if and only if the interaction and self-evolution Hamiltonians share an eigenstate. If decoherence by state preparation is not possible, we show that initial states minimizing decoherence result from a delicate compromise between the environment and interaction dynamics.Comment: 4 pages, 2 figure

The Isaacson expansion in quantum cosmology

This paper is an application of the ideas of the Born-Oppenheimer (or slow/fast) approximation in molecular physics and of the Isaacson (or short-wave) approximation in classical gravity to the canonical quantization of a perturbed minisuperspace model of the kind examined by Halliwell and Hawking. Its aim is the clarification of the role of the semiclassical approximation and the backreaction in such a model. Approximate solutions of the quantum model are constructed which are not semiclassical, and semiclassical solutions in which the quantum perturbations are highly excited.Comment: Revtex, 11 journal or 24 preprint pages. REPLACEMENT: A comment on previous work by Dowker and Laflamme is corrected. Utah preprint UU-REL-93/3/1