17 research outputs found
Quantum inelastic conductance through molecular wires
We calculate non-perturbatively the inelastic effects on the conductance
through a conjugated molecular wire-metal heterojunction, including realistic
electron-phonon coupling. We show that at sub-band-gap energies the current is
dominated by quantum coherent transport of virtual polarons through the
molecule. In this regime, the tunneling current is strongly increased relative
to the case of elastic scattering. It is essential to describe the full quantum
coherence of the polaron formation and transport in order to obtain correct
physics. Our results are generally applicable to one-dimensional atomic or
molecular wires.Comment: 4 pages, 4 figures, accepted for publication in Physical Review
Letter
Coherent electron-phonon coupling and polaron-like transport in molecular wires
We present a technique to calculate the transport properties through
one-dimensional models of molecular wires. The calculations include inelastic
electron scattering due to electron-lattice interaction. The coupling between
the electron and the lattice is crucial to determine the transport properties
in one-dimensional systems subject to Peierls transition since it drives the
transition itself. The electron-phonon coupling is treated as a quantum
coherent process, in the sense that no random dephasing due to electron-phonon
interactions is introduced in the scattering wave functions. We show that
charge carrier injection, even in the tunneling regime, induces lattice
distortions localized around the tunneling electron. The transport in the
molecular wire is due to polaron-like propagation. We show typical examples of
the lattice distortions induced by charge injection into the wire. In the
tunneling regime, the electron transmission is strongly enhanced in comparison
with the case of elastic scattering through the undistorted molecular wire. We
also show that although lattice fluctuations modify the electron transmission
through the wire, the modifications are qualitatively different from those
obtained by the quantum electron-phonon inelastic scattering technique. Our
results should hold in principle for other one-dimensional atomic-scale wires
subject to Peierls transitions.Comment: 21 pages, 8 figures, accepted for publication in Phys. Rev. B (to
appear march 2001
Mission ethnographique et linguistique Dakar-Djibouti.
Flandin P.-E., Doumergue Gaston, Roustan M. Mission ethnographique et linguistique Dakar-Djibouti.. In: Journal de la Société des Africanistes, 1931, tome 1, fascicule 2. pp. 300-303
Mission ethnographique et linguistique Dakar-Djibouti.
Flandin P.-E., Doumergue Gaston, Roustan M. Mission ethnographique et linguistique Dakar-Djibouti.. In: Journal de la Société des Africanistes, 1931, tome 1, fascicule 2. pp. 300-303