1,392 research outputs found
Effect of exchange interaction on superparamagnetic relaxation
We use Langer's approach to calculate the reaction rate of a system of two
(classical) spins interacting via the exchange coupling in a magnetic field
, with uniaxial anisotropy of constant .
We find a particular value of the exchange coupling, that is , where , which separates two regimes
corresponding to a two-stage and one-stage switching.
For the N\'eel-Brown result for the one-spin problem is recovered.Comment: 7 pages, 2 eps figures, fig.1 of better quality can be provided upon
reques
Spin glass like transition in a highly concentrated Fe-C nanoparticle system
A highly concentrated (17 vol.%) Fe-C nano-particle system, with a narrow
size distribution nm, has been investigated using magnetic ac
susceptibility measurements covering a wide range of frequencies (17 mHz - 170
Hz). A dynamic scaling analysis gives evidence for a phase transition to a low
temperature spin-glass-like phase. The critical exponents associated with the
transition are and . The reason why
the scaling analysis works for this sample, while it may not work for other
samples exhibiting collective behavior as evidenced by aging phenomena, is that
the single particle contribution to is vanishingly small for
and hence all slow dynamics is due to collective behavior. This criterion can
only be fulfilled for a highly concentrated nano-particle sample with a narrow
size distribution.Comment: 2 pages, 3 figures, Proceeding for ICM200
Geometric Aspects of the Dipolar Interaction in Lattices of Small Particles
The hysteresis curves of systems composed of small interacting magnetic
particles, regularly placed on stacked layers, are obtained with Monte Carlo
simulations. The remanence as a function of temperature, in interacting
systems, presents a peak that separates two different magnetic states. At low
temperatures, small values of remanence are a consequence of antiferromagnetic
order due to the dipolar interaction. At higher values of temperature the
increase of the component normal to the lattice plane is responsible for the
small values of remanence. The effect of the number of layers, coordination
number and distance between particles are investigated.Comment: 5 pages, 7 figure
Role of dipolar interactions in a system of Ni nanoparticles studied by magnetic susceptibility measurements
The role of dipolar interactions among Ni nanoparticles (NP) embedded in an
amorphous SiO2/C matrix with different concentrations has been studied
performing ac magnetic susceptibility Chi_ac measurements. For very diluted
samples, with Ni concentrations < 4 wt % Ni or very weak dipolar interactions,
the data are well described by the Neel-Arrhenius law. Increasing Ni
concentration to values up to 12.8 wt % Ni results in changes in the
Neel-Arrhenius behavior, the dipolar interactions become important, and need to
be considered to describe the magnetic response of the NPs system. We have
found no evidence of a spin-glasslike behavior in our Ni NP systems even when
dipolar interactions are clearly present.Comment: 7 pages, 5 figures, 3 table
Within-day dynamics of plant–pollinator networks are dominated by early flower closure: an experimental test of network plasticity
Temporal variability of plant–pollinator interactions is important for fully understanding the structure, function, and stability of plant–pollinator networks, but most network studies so far have ignored within-day dynamics. Strong diel dynamics (e.g., a regular daily cycle) were found for networks with Cichorieae, which typically close their flowers around noon. Here, we experimentally prevented early flower closure to test whether these dynamics are driven by the temporally limited availability of Cichorieae, or by timing of pollinator activity. We further tested if the dynamics involving Cichorieae and their pollinators also affect the dynamics on other plants in the network. Finally, we explored the structure of such manipulated networks (with Cichorieae available in the morning and afternoon) compared to unmanipulated controls (Cichorieae available only in the morning). We found that flower closure of Cichorieae is indeed an important driver of diel network dynamics, while other drivers of pollinator timing appeared less important. If Cichorieae flowers were available in the afternoon, they were visited by generalist and specialist pollinators, which overall decreased link turnover between morning and afternoon. Effects of afternoon availability of Cichorieae on other plants in the network were inconclusive: pollinator switching to and from Cichorieae tended to increase. On the level of the aggregated (full-day) network, the treatment resulted in increased dominance of Cichorieae, reducing modularity and increasing plant generality. These results highlight that network dynamics can be predicted by knowledge of diel or seasonal phenology, and that fixed species timing assumptions will misrepresent the expected dynamics.Fil: Schwarz, Benjamin. Albert Ludwigs University of Freiburg; AlemaniaFil: Dormann, Carsten F.. Albert Ludwigs University of Freiburg; AlemaniaFil: Vazquez, Diego P.. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza. Instituto Argentino de Investigaciones de las Zonas Áridas. Provincia de Mendoza. Instituto Argentino de Investigaciones de las Zonas Áridas. Universidad Nacional de Cuyo. Instituto Argentino de Investigaciones de las Zonas Áridas; Argentina. Universidad Nacional de Cuyo. Facultad de Ciencias Exactas y Naturales; ArgentinaFil: Fründ, Jochen. Albert Ludwigs University of Freiburg; Alemani
Micro-SQUID technique for studying the temperature dependence of switching fields of single nanoparticles
An improved micro-SQUID technique is presented allowing us to measure the
temperature dependence of the magnetisation switching fields of single
nanoparticles well above the critical superconducting temperature of the SQUID.
Our first measurements on 3 nm cobalt nanoparticle embedded in a niobium matrix
are compared to the Neel Brown model describing the magnetisation reversal by
thermal activation over a single anisotropy barrier.Comment: 3 pages, 4 figures; conference proceeding: 1st Joint European
Magnetic Symposia (JEMS'01), Grenoble (France), 28th August - 1st September,
200
ESR of MnO embedded in silica nanoporous matrices with different topologies
Electron spin resonance (ESR) experiments were performed with
antiferromagnetic MnO confined within a porous vycor-type glass and within
MCM-type channel matrices. A signal from confined MnO shows two components from
crystallized and amorphous MnO and depends on the pore topology. Crystallized
MnO within a porous glass shows a behavior having many similarities to the
bulk. In contrast with the bulk the strong ESR signal due to disordered
"surface" spins is observed below the magnetic transition. With the decrease of
channel diameter the fraction of amorphous MnO increases while the amount of
crystallized MnO decreases. The mutual influence of amorphous and crystalline
MnO is observed in the matrices with a larger channel diameter. In the matrices
with a smaller channel diameter the ESR signal mainly originates from amorphous
MnO and its behavior is typical for the highly disordered magnetic system.Comment: 7 pages pdf file, 5 figure
Magnetic properties of polypyrrole - coated iron oxide nanoparticles
Iron oxide nanoparticles were prepared by sol -gel process. Insitu
polymerization of pyrrole monomer in the presence of oxygen in iron oxide
ethanol suspension resulted in a iron oxide - polypyrrole nanocomposite. The
structure and magnetic properties were investigated for varying pyrrole
concentrations. The presence of the gamma - iron oxide phase and polypyrrole
were confirmed by XRD and FTIR respectively. Agglomeration was found to be
comparatively much reduced for the coated samples, as shown by TEM. AC
susceptibility measurements confirmed the superparamagnetic behaviour.
Numerical simulations performed for an interacting model system are performed
to estimate the anisotropy and compare favourably with experimental results.Comment: 11 pages,8 figure
Magnetic relaxation in finite two-dimensional nanoparticle ensembles
We study the slow phase of thermally activated magnetic relaxation in finite
two-dimensional ensembles of dipolar interacting ferromagnetic nanoparticles
whose easy axes of magnetization are perpendicular to the distribution plane.
We develop a method to numerically simulate the magnetic relaxation for the
case that the smallest heights of the potential barriers between the
equilibrium directions of the nanoparticle magnetic moments are much larger
than the thermal energy. Within this framework, we analyze in detail the role
that the correlations of the nanoparticle magnetic moments and the finite size
of the nanoparticle ensemble play in magnetic relaxation.Comment: 21 pages, 4 figure
Structural and magnetic properties of CoPt mixed clusters
In this present work, we report a structural and magnetic study of mixed
Co58Pt42 clusters. MgO, Nb and Si matrix can be used to embed clusters,
avoiding any magnetic interactions between particles. Transmission Electron
Microscopy (TEM) observations show that Co58Pt42 supported isolated clusters
are about 2nm in diameter and crystallized in the A1 fcc chemically disordered
phase. Grazing Incidence Small Angle X-ray Scattering (GISAXS) and Grazing
Incidence Wide Angle X-ray Scattering (GIWAXS) reveal that buried clusters
conserve these properties, interaction with matrix atoms being limited to their
first atomic layers. Considering that 60% of particle atoms are located at
surface, this interactions leads to a drastic change in magnetic properties
which were investigated with conventional magnetometry and X-Ray Magnetic
Circular Dichro\"{i}sm (XMCD). Magnetization and blocking temperature are
weaker for clusters embedded in Nb than in MgO, and totally vanish in silicon
as silicides are formed. Magnetic volume of clusters embedded in MgO is close
to the crystallized volume determined by GIWAXS experiments. Cluster can be
seen as a pure ferromagnetic CoPt crystallized core surrounded by a
cluster-matrix mixed shell. The outer shell plays a predominant role in
magnetic properties, especially for clusters embedded in niobium which have a
blocking temperature 3 times smaller than clusters embedded in MgO
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