160 research outputs found
Effect of Mn substitution by Ga on the optical properties of a metallic manganite
In a metallic manganite like La(2/3)Sr(1/3)MnO(3), the substitution of Mn(+3)
by Ga(+3) dilutes the ferromagnetic order and locally cancels the Jahn-Teller
distortion, without heavily affecting the crystal structure. One can thus
follow the changes in the charge dynamics induced by Ga, until the
ferro-metallic manganite is turned into an insulator. Here this phenomenon is
studied in detail through the infrared reflectivity of five samples of
La(2/3)Sr(1/3)Mn(1-x)Ga(x)O(3), with x increasing from 0 to 0.30 and for 50 < T
< 320 K. A simple model which links the measured optical parameters to the
magnetization M(x, T) well describes the behavior of the plasma frequency, the
scattering rate, and the mid-infrared absorption along the metal-to-insulator
transition.Comment: 8 pages including 7 figure
Optical Properties of (SrMnO3)n/(LaMnO3)2n superlattices: an insulator-to-metal transition observed in the absence of disorder
We measure the optical conductivity of (SrMnO3)n/(LaMnO3)2n superlattices
(SL) for n=1,3,5, and 8 and 10 < T < 400 K. Data show a T-dependent insulator
to metal transition (IMT) for n \leq 3, driven by the softening of a polaronic
mid-infrared band. At n = 5 that softening is incomplete, while at the
largest-period n=8 compound the MIR band is independent of T and the SL remains
insulating. One can thus first observe the IMT in a manganite system in the
absence of the disorder due to chemical doping. Unsuccessful reconstruction of
the SL optical properties from those of the original bulk materials suggests
that (SrMnO3)n/(LaMnO3)2n heterostructures give rise to a novel electronic
state.Comment: Published Online in Nano Letters, November 8, 2010;
http://pubs.acs.org/doi/abs/10.1021/nl1022628; 5 pages, 3 figure
Magnetic imaging of pearl vortices in artificially layered (Ba 0.9Nd0.1CuO2+x)m/(CaCuO 2)n systems
We have used scanning SQUID magnetometry to image vortices in ultrathin (Ba0.9Nd0.1CuO2+x)(m)/(CaCuO2)(n) high temperature superconductor samples, with as few as three superconducting CuO2 planes. The Pearl lengths (Lambda=2lambda(L)(2)/d, lambda(L) the London penetration depth, d the superconducting film thickness) in these samples, as determined by fits to the vortex images, agree with those by local susceptibility measurements, and can be as long as 1 mm. The in-plane penetration depths lambda(ab) inferred from the Pearl lengths are longer than many bulk cuprates with comparable critical temperatures. We speculate on the causes of the long penetration depths, and on the possibility of exploiting the unique properties of these superconductors for basic experiments
Role of interband scattering in neutron irradiated MgB thin films by Scanning Tunneling Spectroscopy measurements
A series of MgB thin films systematically disordered by neutron
irradiation have been studied by Scanning Tunneling Spectroscopy. The c-axis
orientation of the films allowed a reliable determination of local density of
state of the band. With increasing disorder, the conductance peak moves
towards higher voltages and becomes lower and broader, indicating a monotonic
increase of the gap and of the broadening parameter. These results are
discussed in the frame of two-band superconductivity.Comment: The text will be submitted in Latex format, and the corresponding pdf
file should take 6 pages. There are 5 figures (eps files submitted) and 1
tabl
Dissipation in ultra-thin current-carrying superconducting bridges; evidence for quantum tunneling of Pearl vortices
We have made current-voltage (IV) measurements of artificially layered
high- thin-film bridges. Scanning SQUID microscopy of these films provides
values for the Pearl lengths that exceed the bridge width, and shows
that the current distributions are uniform across the bridges. At high
temperatures and high currents the voltages follow the power law , with , and at high temperatures and
low-currents the resistance is exponential in temperature, in good agreement
with the predictions for thermally activated vortex motion. At low
temperatures, the IV's are better fit by linear in . This is
expected if the low temperature dissipation is dominated by quantum tunneling
of Pearl vortices.Comment: 5 pages, 7 fig
Multiple double-exchange mechanism by Mn-doping in manganite compounds
Double-exchange mechanisms in REAEMnO manganites (where
RE is a trivalent rare-earth ion and AE is a divalent alkali-earth ion) relies
on the strong exchange interaction between two Mn and Mn ions
through interfiling oxygen 2p states. Nevertheless, the role of RE and AE ions
has ever been considered "silent" with respect to the DE conducting mechanisms.
Here we show that a new path for DE-mechanism is indeed possible by partially
replacing the RE-AE elements by Mn-ions, in La-deficient
LaMnO thin films. X-ray absorption spectroscopy demonstrated
the relevant presence of Mn ions, which is unambiguously proved to be
substituted at La-site by Resonant Inelastic X-ray Scattering. Mn is
proved to be directly correlated to the enhanced magneto-transport properties
because of an additional hopping mechanism trough interfiling Mn-ions,
theoretically confirmed by calculations within the effective single band model.
The very idea to use Mn both as a doping element and an ions
electronically involved in the conduction mechanism, has never been foreseen,
revealing a new phenomena in transport properties of manganites. More
important, such a strategy might be also pursed in other strongly correlated
materials.Comment: 6 pages, 5 figure
Evolution of magnetic phases and orbital occupation in (SrMnO3)n/(LaMnO3)2n superlattices
The magnetic and electronic modifications induced at the interfaces in
(SrMnO)/(LaMnO) superlattices have been investigated
by linear and circular magnetic dichroism in the Mn L x-ray absorption
spectra. Together with theoretical calculations, our data demonstrate that the
charge redistribution across interfaces favors in-plane ferromagnetic (FM)
order and orbital occupation, in agreement with the
average strain. Far from interfaces, inside LaMnO, electron localization
and local strain favor antiferromagnetism (AFM) and
orbital occupation. For the high density of interfacial planes ultimately
leads to dominant FM order forcing the residual AFM phase to be in-plane too,
while for the FM layers are separated by AFM regions having
out-of-plane spin orientation.Comment: accepted for publication as a Rapid Communication in Physical Review
Analysis of Metal-Insulator Crossover in Strained {SrRuO}3 Thin Films by X-ray Photoelectron Spectroscopy
The electronic properties of ultrathin epitaxial films of strontium ruthenate SrRuO3 perovskite oxide are modified by epitaxial strain, as determined by growing by pulsed laser deposition, on different the substrates. Electron transport measurements indicated that tensile strain deformation of the SrRuO3 unit cell reduces the metallicity of the material and reduces the metal-insulator-transition (MIT) temperatures. The shrinkage of the Ru-O-Ru buckling angle due to compressive strain is counterweighted by the increased overlap of the conduction Ru-4d orbitals with the O-2p ones due to the smaller interatomic distances resulting into an increased MIT temperature, i.e. a more conducting material. In the more metallic samples the core level x-ray photoemission spectroscopy lineshapes show the occurrence of an extra-peak at the lower binding energies of the main Ru-3d peaks that is attributed to screening, as observed in volume sensitive photoemission of the unstrained material
Intrinsic nonlinearity probed by intermodulation distortion microwave measurements on high quality MgB2 thin films
The two tone intermodulation distortion arising in MgB2 thin films
synthesized by hybrid physical-chemical vapour deposition is studied in order
to probe the influence of the two bands on the nonlinear response of this
superconductor. The measurements are carried out by using a dielectrically
loaded copper cavity operating at 7 GHz. Microwave data on samples having
critical temperatures above 41 K, very low resistivity values, and residual
resistivity ratio larger than 10, are shown. The dependence of the nonlinear
surface losses and of the third order intermodulation products on the power
feeding the cavity and on the temperature is analyzed. At low power, the signal
arising from distortion versus temperature shows the intrinsic s-wave behavior
expected for this compound. Data are compared with measurements performed on Nb
and YBCO thin films using the same technique.Comment: Revised version. Submitted to APL on October 7th 200
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