Characterization of the second- and third-order nonlinear optical susceptibilities of monolayer MoS2_2 using multiphoton microscopy

We report second- and third-harmonic generation in monolayer MoS$_\mathrm{2}$ as a tool for imaging and accurately characterizing the material's nonlinear optical properties under 1560 nm excitation. Using a surface nonlinear optics treatment, we derive expressions relating experimental measurements to second- and third-order nonlinear sheet susceptibility magnitudes, obtaining values of $|\chi_s^{(2)}|=2.0\times10^{-20}$ m$^2$ V$^{-1}$ and for the first time for monolayer MoS$_\mathrm{2}$, $|\chi_s^{(3)}|=1.7\times10^{-28}$ m$^3$ V$^{-2}$. These sheet susceptibilities correspond to effective bulk nonlinear susceptibility values of $|\chi_{b}^{(2)}|=2.9\times10^{-11}$ m V$^{-1}$ and $|\chi_{b}^{(3)}|=2.4\times10^{-19}$ m$^2$ V$^{-2}$, accounting for the sheet thickness. Experimental comparisons between MoS$_\mathrm{2}$ and graphene are also performed, demonstrating $\sim$3.4 times stronger third-order sheet nonlinearity in monolayer MoS$_\mathrm{2}$, highlighting the material's potential for nonlinear photonics in the telecommunications C band.Comment: Accepted by 2D Materials, 28th Oct 201

A comparative study for the pair-creation contact process using series expansions

A comparative study between two distinct perturbative series expansions for the pair-creation contact process is presented. In contrast to the ordinary contact process, whose supercritical series expansions provide accurate estimates for its critical behavior, the supercritical approach does not work properly when applied to the pair-creation process. To circumvent this problem a procedure is introduced in which one-site creation is added to the pair-creation. An alternative method is the generation of subcritical series expansions which works even for the case of the pure pair-creation process. Differently from the supercritical case, the subcritical series yields estimates that are compatible with numerical simulations

Mean-field calculation of critical parameters and log-periodic characterization of an aperiodic-modulated model

We employ a mean-field approximation to study the Ising model with aperiodic modulation of its interactions in one spatial direction. Two different values for the exchange constant, $J_A$ and $J_B$, are present, according to the Fibonacci sequence. We calculated the pseudo-critical temperatures for finite systems and extrapolate them to the thermodynamic limit. We explicitly obtain the exponents $\beta$, $\delta$, and $\gamma$ and, from the usual scaling relations for anisotropic models at the upper critical dimension (assumed to be 4 for the model we treat), we calculate $\alpha$, $\nu$, $\nu_{//}$, $\eta$, and $\eta_{//}$. Within the framework of a renormalization-group approach, the Fibonacci sequence is a marginal one and we obtain exponents which depend on the ratio $r \equiv J_B/J_A$, as expected. But the scaling relation $\gamma = \beta (\delta -1)$ is obeyed for all values of $r$ we studied. We characterize some thermodynamic functions as log-periodic functions of their arguments, as expected for aperiodic-modulated models, and obtain precise values for the exponents from this characterization.Comment: 17 pages, including 9 figures, to appear in Phys. Rev.

Spectroscopy of brown dwarf candidates in IC 348 and the determination of its substellar IMF down to planetary masses

Context. Brown dwarfs represent a sizable fraction of the stellar content of our Galaxy and populate the transition between the stellar and planetary mass regime. There is however no agreement on the processes responsible for their formation. Aims. We have conducted a large survey of the young, nearby cluster IC 348, to uncover its low-mass brown dwarf population and study the cluster properties in the substellar regime. Methods. Deep optical and near-IR images taken with MegaCam and WIRCam at the Canada-France-Hawaii Telescope (CFHT) were used to select photometric candidate members. A spectroscopic follow-up of a large fraction of the candidates was conducted to assess their youth and membership. Results. We confirmed spectroscopically 16 new members of the IC 348 cluster, including 13 brown dwarfs, contributing significantly to the substellar census of the cluster, where only 30 brown dwarfs were previously known. Five of the new members have a L0 spectral type, the latest-type objects found to date in this cluster. At 3 Myr, evolutionary models estimate these brown dwarfs to have a mass of ~13 Jupiter masses. Combining the new members with previous census of the cluster, we constructed the IMF complete down to 13 Jupiter masses. Conclusions. The IMF of IC 348 is well fitted by a log-normal function, and we do not see evidence for variations of the mass function down to planetary masses when compared to other young clusters.Comment: Accepted to A&A (8 November 2012

Density-based mixing parameter for hybrid functionals

A very popular ab-initio scheme to calculate electronic properties in solids is the use of hybrid functionals in density functional theory (DFT) that mixes a portion of Fock exchange with DFT functionals. In spite of their success, a major problem still remains, related to the use of one single mixing parameter for all materials. Guided by physical arguments that connect the mixing parameter to the dielectric properties of the solid, and ultimately to its band gap, we propose a method to calculate this parameter from the electronic density alone. This method is able to cut significantly the error of traditional hybrid functionals for large and small gap materials, while retaining a good description of structural properties. Moreover, its implementation is simple and leads to a negligible increase of the computational time.Comment: submitte

Efficiency of low versus high airline pressure in stunning cattle with a pneumatically powered penetrating captive bolt gun

The efficiency of stunning cattle was assessed in 443 animals (304 pure Zebu and 139 crossbred cattle), being mainly mature bulls and cows. Cattle were stunned using a Jarvis pneumatically powered penetrating captive bolt gun operating with low (160–175 psi, N = 82) and high (190 psi, N = 363) airline pressure, which was within the manufactures specifications. Signs of brain function and the position of the shots on the heads were recorded after stunning. Velocity of the captive bolt and its physical parameters were calculated. Cattle shot with low pressures showed more rhythmic respiration (27 vs. 8%, P < 0.001), less tongue protrusion (4 vs. 12%, P = 0.03) and less masseter relaxation (22 vs. 48%, P < 0.001). There was an increased frequency of shots in the ideal position when cattle were shot with the low compared to high airline pressures (15.3 vs. 3.1%). Bolt velocity and its physical parameters were significantly (P < 0.01) higher when using high pressure. Airline pressures below 190 psi are inappropriate when shooting adult Zebu beef cattle with pneumatically powered penetrating captive bolt guns

Exact Solutions of the Klein-Gordon Equation in the Presence of a Dyon, Magnetic Flux and Scalar Potential in the Specetime of Gravitational Defects

In this paper we analyse the relativistic quantum motion of a charged spin-0 particle in the presence of a dyon, Aharonov-Bohm magnetic field and scalar potential, in the spacetimes produced by an idealized cosmic string and global monopole. In order to develop this analysis, we assume that the dyon and the Aharonov-Bohm magnetic field are superposed to both gravitational defects. Two distinct configurations for the scalar potential, $S(r)$, are considered: $i)$ the potential proportional to the inverse of the radial distance, i.e., $S\propto1/r$, and $ii)$ the potential proportional to this distance, i.e., $S\propto r$. For both cases the center of the potentials coincide with the dyon's position. In the case of the cosmic string the Aharonov-Bohm magnetic field is considered along the defect, and for the global monopole this magnetic field pierces the defect. The energy spectra are computed for both cases and explicitly shown their dependence on the electrostatic and scalar coupling constants. Also we analyse scattering states of the Klein-Gordon equations, and show how the phase shifts depend on the geometry of the spacetime and on the coupling constants parameter.Comment: To be published in CQG. Minor comments adde

Chaotic Interaction of Langmuir Solitons and Long Wavelength Radiation

In this work we analyze the interaction of isolated solitary structures and ion-acoustic radiation. If the radiation amplitude is small solitary structures persists, but when the amplitude grows energy transfer towards small spatial scales occurs. We show that transfer is particularly fast when a fixed point of a low dimensional model is destroyed.Comment: LaTex + 4 eps file