328 research outputs found
Template nanowires for spintronics applications: nanomagnet microwave resonators functioning in zero applied magnetic field
Low-cost spintronic devices functioning in zero applied magnetic field are
required for bringing the idea of spin-based electronics into the real-world
industrial applications. Here we present first microwave measurements performed
on nanomagnet devices fabricated by electrodeposition inside porous membranes.
In the paper, we discuss in details a microwave resonator consisting of three
nanomagnets, which functions in zero external magnetic field. By applying a
microwave signal at a particular frequency, the magnetization of the middle
nanomagnet experiences the ferromagnetic resonance (FMR), and the device
outputs a measurable direct current (spin-torque diode effect). Alternatively,
the nanodevice can be used as a microwave oscillator functioning in zero field.
In order to test the resonators at microwave frequencies, we developed a simple
measurement set-up.Comment: 21 pages (main text - 13 pages + Supporting Information
Optically switched magnetism in photovoltaic perovskite CHNH(Mn:Pb)I
The demand for ever-increasing density of information storage and speed of
manipulation boosts an intense search for new magnetic materials and novel ways
of controlling the magnetic bit. Here, we report the synthesis of a
ferromagnetic photovoltaic CHNH(Mn:Pb)I material in which the
photo-excited electrons rapidly melt the local magnetic order through the
Ruderman-Kittel-Kasuya-Yosida interactions without heating up the spin system.
Our finding offers an alternative, very simple and efficient way of optical
spin control, and opens an avenue for applications in low power, light
controlling magnetic devices
Atomic and Electronic Structure of a Rashba - Junction at the BiTeI Surface
The non-centrosymmetric semiconductor BiTeI exhibits two distinct surface
terminations that support spin-split Rashba surface states. Their ambipolarity
can be exploited for creating spin-polarized - junctions at the
boundaries between domains with different surface terminations. We use scanning
tunneling microscopy/spectroscopy (STM/STS) to locate such junctions and
investigate their atomic and electronic properties. The Te- and I-terminated
surfaces are identified owing to their distinct chemical reactivity, and an
apparent height mismatch of electronic origin. The Rashba surface states are
revealed in the STS spectra by the onset of a van Hove singularity at the band
edge. Eventually, an electronic depletion is found on interfacial Te atoms,
consistent with the formation of a space charge area in typical -
junctions.Comment: 5 pages, 4 figure
Strong out-of-plane magnetic anisotropy of Fe adatoms on BiTe
The electronic and magnetic properties of individual Fe atoms adsorbed on the
surface of the topological insulator BiTe(111) are investigated.
Scanning tunneling microscopy and spectroscopy prove the existence of two
distinct types of Fe species, while our first-principles calculations assign
them to Fe adatoms in the hcp and fcc hollow sites. The combination of x-ray
magnetic circular dichroism measurements and angular dependent magnetization
curves reveals out-of-plane anisotropies for both species with anisotropy
constants of meV/atom and meV/atom. These values are well in line with the results of
calculations.Comment: 6 pages, 3 figure
BiTeCl and BiTeBr: a comparative high-pressure optical study
We here report a detailed high-pressure infrared transmission study of BiTeCl
and BiTeBr. We follow the evolution of two band transitions: the optical
excitation between two Rashba-split conduction bands, and the
absorption across the band gap. In the low pressure range, ~GPa,
for both compounds is approximately constant with pressure and
decreases, in agreement with band structure calculations. In BiTeCl, a clear
pressure-induced phase transition at 6~GPa leads to a different ground state.
For BiTeBr, the pressure evolution is more subtle, and we discuss the
possibility of closing and reopening of the band gap. Our data is consistent
with a Weyl phase in BiTeBr at 56~GPa, followed by the onset of a structural
phase transition at 7~GPa.Comment: are welcom
Experimentally Engineering the Edge Termination of Graphene Nanoribbons
The edges of graphene nanoribbons (GNRs) have attracted much interest due to
their potentially strong influence on GNR electronic and magnetic properties.
Here we report the ability to engineer the microscopic edge termination of high
quality GNRs via hydrogen plasma etching. Using a combination of
high-resolution scanning tunneling microscopy and first-principles
calculations, we have determined the exact atomic structure of plasma-etched
GNR edges and established the chemical nature of terminating functional groups
for zigzag, armchair and chiral edge orientations. We find that the edges of
hydrogen-plasma-etched GNRs are generally flat, free of structural
reconstructions and are terminated by hydrogen atoms with no rehybridization of
the outermost carbon edge atoms. Both zigzag and chiral edges show the presence
of edge states.Comment: 16+9 pages, 3+4 figure
Magnetic excitations and electronic interactions in SrCuTeO: a spin-1/2 square lattice Heisenberg antiferromagnet
SrCuTeO presents an opportunity for exploring low-dimensional
magnetism on a square lattice of Cu ions. We employ ab initio
multi-reference configuration interaction calculations to unravel the Cu
electronic structure and to evaluate exchange interactions in SrCuTeO.
The latter results are validated by inelastic neutron scattering using linear
spin-wave theory and series-expansion corrections for quantum effects to
extract true coupling parameters. Using this methodology, which is quite
general, we demonstrate that SrCuTeO is an almost realization of a
nearest-neighbor Heisenberg antiferromagnet but with relatively weak coupling
of 7.18(5) meV.Comment: 10 pages, 7 figure
Density functional investigations of defect induced mid-gap states in graphane
We have carried out ab initio electronic structure calculations on graphane
(hydrogenated graphene) with single and double vacancy defects. Our analysis of
the density of states reveal that such vacancies induce the mid gap states and
modify the band gap. The induced states are due to the unpaired electrons on
carbon atoms. Interestingly the placement and the number of such states is
found to be sensitive to the distance between the vacancies. Furthermore we
also found that in most of the cases the vacancies induce a local magnetic
moment.Comment: 15 page
Universal Magnetic Properties of sp-type Defects in Covalently Functionalized Graphene
Using density-functional calculations, we study the effect of sp-type
defects created by different covalent functionalizations on the electronic and
magnetic properties of graphene. We find that the induced magnetic properties
are {\it universal}, in the sense that they are largely independent on the
particular adsorbates considered. When a weakly-polar single covalent bond is
established with the layer, a local spin-moment of 1.0 always appears
in graphene. This effect is similar to that of H adsorption, which saturates
one orbital in the carbon layer. The magnetic couplings between the
adsorbates show a strong dependence on the graphene sublattice of
chemisorption. Molecules adsorbed at the same sublattice couple
ferromagnetically, with an exchange interaction that decays very slowly with
distance, while no magnetism is found for adsorbates at opposite sublattices.
Similar magnetic properties are obtained if several orbitals are
saturated simultaneously by the adsorption of a large molecule. These results
might open new routes to engineer the magnetic properties of graphene
derivatives by chemical means
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