Evaporation Channel as a Tool to Study Fission Dynamics

The dynamics of the fission process is expected to affect the evaporation residue cross section because of the fission hindrance due to the nuclear viscosity. Systems of intermediate fissility constitute a suitable environment for testing such hypothesis, since they are characterized by evaporation residue cross sections comparable or larger than the fission ones. Observables related to emitted charged particle, due to their relatively high emission probability, can be used to put stringent constraints on models describing the excited nucleus decay and to recognize the effects of fission dynamics. In this work model simulations are compared with the experimental data collected via the ^{32}S + ^{100}Mo reaction at E_{lab}= 200 MeV. By comparing an extended set of evaporation channel observables the limits of the statistical model and the large improvement coming by using a dynamical model are evidenced. The importance of using a large angular covering apparatus to extract the observable is stressed. The opportunity to measure more sensitive observables by a new detection device in operation at LNL are also discussed.Comment: v1: 7 pages, 6 figure

Fragmentation of spherical radioactive heavy nuclei as a novel probe of transient effects in fission

Peripheral collisions with radioactive heavy-ion beams at relativistic energies are discussed as an innovative approach for probing the transient regime experienced by fissile systems evolving towards quasi-equilibrium. A dedicated experiment using the advanced technical installations of GSI, Darmstadt, permitted to realize ideal conditions for the investigation of relaxation effects in the meta-stable well. Combined with a highly sensitive experimental signature, it provides a measure of the transient effects with respect to the flux over the fission barrier. Within a two-step reaction process, 45 proton-rich unstable spherical isotopes produced by projectile-fragmentation of a stable 238U beam have been used as secondary projectiles. The fragmentation of the radioactive projectiles on lead results in nearly spherical compound nuclei which span a wide range in excitation energy and fissility. The decay of these excited systems by fission is studied with a dedicated set-up which permits the detection of both fission products in coincidence and the determination of their atomic numbers with high resolution. The width of the fission-fragment nuclear charge distribution is shown to be specifically sensitive to pre-saddle transient effects and is used to establish a clock for the passage of the saddle point. The comparison of the experimental results with model calculations points to a fission delay of (3.3+/-0.7).10-21s for initially spherical compound nuclei, independent of excitation energy and fissility. This value suggests a nuclear dissipation strength at small deformation of (4.5+/-0.5).1021s-1. The very specific combination of the physics and technical equipment exploited in this work sheds light on previous controversial conclusions.Comment: 38 pages, 15 figure

Sequential fissions of heavy nuclear systems

In Xe+Sn central collisions from 12 to 20 MeV/A measured with the INDRA 4$\pi$ multidetector, the three-fragment exit channel occurs with a significant cross section. In this contribution, we show that these fragments arise from two successive binary splittings of a heavy composite system. Strong Coulomb proximity effects are observed in the three-fragment final state. By comparison with Coulomb trajectory calculations, we show that the time scale between the consecutive break-ups decreases with increasing bombarding energy, becoming compatible with quasi-simultaneous multifragmentation above 18 MeV/A.Comment: 6 pages, 5 figures, contribution to conference proceedings of the Fifth International Workshop on Nuclear fission and Fission-Product Spectroscop

Examination of isospin effects in multi-dimensional Langevin fission dynamics

Abstract One-dimensional and three-dimensional dynamical fission calculations based on Langevin equations are performed for the compound nuclei 194 Pb, 200 Pb, 206 Pb, 182 Hg, and 204 Hg to investigate the influence of the compound nucleus isospin on the prescission particle multiplicities and on the fission fragment mass–energy distribution. It is found that the prescission neutron, proton, and alpha particle multiplicities have approximately the same sensitivity to the dissipation strength for a given nucleus. This is at variance with conclusions of recent papers. The sensitivity of the calculated prescission particle multiplicities to the dissipation strength becomes higher with decreasing isospin of fissioning compound nucleus, and the increase of prescission particle multiplicities could reach 200%, when the reduction coefficient of one-body viscosity k s increases from 0.1 to 1, for the most neutron deficient nuclei considered. The variances of fission fragment mass and kinetic energy distributions are less sensitive to the change of dissipation strength than the prescission light particle multiplicities. A comparison to experimental data concerning 200 Pb nucleus is also presented

Clustering effects in 48Cr composite nuclei produced via 24Mg + 24Mg reaction

In the framework of studying clustering effects in N=Z light nuclei, an experiment was carried out to get information on the properties of the 48 Cr composite nuclei produced via the 24 Mg +24 Mg reaction. In particular, the study regards the 48 Cr at 60 MeV of excitation energy where a resonance with a narrow width (170 KeV) has been found by measuring the elastic and anelastic channels. To determine the deformation of this state, evaporative Light Charged Particles (LCP) are measured and compared to the Statistical Model (SM) predictions, which are very sensitive to nuclear deformation. The experiment was performed at LNL using the 8ĒLP apparatus to select LCPs and a Parallel Plate Avalanche Counter (PPAC) system to detect the Evaporation Residues (ER). Preliminary results on the measurements of ER – LCP and LCP – LCP angular correlations are presented which indicate the presence of a very large deformation.The analysis will proceed with the extraction of the LCP energy spectra and with the angular correlations for high multiplicity channels to determine the deformation

First experiment on fission transients in highly fissile spherical nuclei produced by fragmentation of radioactive beams

We report on a novel experimental approach for studying the dissipative spreading of collective motion in a meta-stable nuclear system, using, for the first time, highly fissile nuclei with spherical shape. This was achieved by fragmentation of 45 radioactive heavy-ion beams at GSI, Darmstadt. The use of inverse kinematics and a dedicated experimental set-up allowed for the identification in atomic number of both fission fragments. From the width of their charge distributions, a transient time of (3.3 +/- 0.7) 10-21 s is deduced for initially spherical nuclei.Comment: 7 pages, 4 figures, background information at http://www-win.gsi.de/charms

Coulomb chronometry to probe the decay mechanism of hot nuclei

In 129 Xe+ nat Sn central collisions from 8 to 25 MeV/A, the three-fragment exit channel occurs with a significant cross section. We show that these fragments arise from two successive binary splittings of a heavy composite system. The sequence of fragment production is determined. Strong Coulomb proximity effects are observed in the three-fragment final state. A comparison with Coulomb trajec-tory calculations shows that the time scale between the consecutive break-ups decreases with increasing bombarding energy, becoming quasi-simultaneous above excitation energy E * = 4.0$\pm$0.5 MeV/A. This transition from sequential to simultaneous break-up was interpreted as the signature of the onset of multifragmentation for the three-fragment exit channel in this system.Comment: 12 pages; 13 Figures; 4 Table; Accepted for publication in Physical Review