Laser Wake Field Collider

Recently NAno-Plasmonic, Laser Inertial Fusion Experiments (NAPLIFE) were proposed, as an improved way to achieve laser driven fusion. The improvement is the combination of two basic research discoveries: (i) the possibility of detonations on space-time hyper-surfaces with time-like normal (i.e. simultaneous detonation in a whole volume) and (ii) to increase this volume to the whole target, by regulating the laser light absorption using nanoshells or nanorods as antennas. These principles can be realized in a one dimensional configuration, in the simplest way with two opposing laser beams as in particle colliders. Such, opposing laser beam experiments were also performed recently. Here we study the consequences of the Laser Wake Field Acceleration (LWFA) if we experience it in a colliding laser beam set-up. These studies can be applied to laser driven fusion, but also to other rapid phase transition, combustion, or ignition studies in other materials.publishedVersio

The Effect of Femtosecond Laser Irradiation and Plasmon Field on the Degree of Conversion of a UDMA-TEGDMA Copolymer Nanocomposite Doped with Gold Nanorods

In this work, the effects of femtosecond laser irradiation and doping with plasmonic gold nanorods on the degree of conversion (DC) of a urethane dimethacrylate (UDMA)–triethylene glycol dimethacrylate (TEGDMA) nanocomposite were investigated. The UDMA-TEGDMA photopolymer was prepared in a 3:1 weight ratio and doped with dodecanethiol- (DDT) capped gold nanorods of 25 × 75 or 25 × 85 nm nominal diameter and length. It was found that the presence of the gold nanorods alone (without direct plasmonic excitation) can increase the DC of the photopolymer by 6–15%. This increase was found to be similar to what could be achieved with a control heat treatment of 30 min at 180 °C. It was also shown that femtosecond laser impulses (795 nm, 5 mJ pulse energy, 50 fs pulse length, 2.83 Jcm−2 fluence), applied after the photopolymerization under a standard dental curing lamp, can cause a 2–7% increase in the DC of undoped samples, even after thermal pre-treatment. The best DC values (12–15% increase) were obtained with combined nanorod doping and subsequent laser irradiation close to the plasmon resonance peak of the nanorods (760–800 nm), which proves that the excited plasmon field can directly facilitate double bond breakage (without thermoplasmonic effects due to the short pulse length) and increase the crosslink density independently from the initial photopolymerization process

Pulsed laser intensity dependence of crater formation and light reflection in the UDMA-TEGDMA copolymer nanocomposite, doped with resonant plasmonic gold nanorods

Plasmonic nanoparticles embedded into a solid matrix could play crucial role in laser-matter interactions. In this study, excess energy creation was observed during the single-shot irradiation of a polymer matrix containing plasmonic gold nanorods, resonant to the laser wavelength, with a high intensity femtosecond laser pulse. This effect was manifested in a 7-fold rise in the crater volume for a 1.7-fold increase of the laser intensity, and was absent in the pure polymer without the gold doping. It occurred at laser intensities > 1.5 x 1017 W/cm2, being the vanishing threshold of plasma mirror formation, resulting in a more than 80% increase of the amount of laser light entering the target. This threshold was found to be critical for the plasmonic effect of gold nanoantennas tuned to the wavelength of the laser on the crater formation