Analyzing Fragmentation of Simple Fluids with Percolation Theory

We show that the size distributions of fragments created by high energy nuclear collisions are remarkably well reproduced within the framework of a parameter free percolation model. We discuss two possible scenarios to explain this agreement and suggest that percolation could be an universal mechanism to explain the fragmentation of simple fluids.Comment: 12 pages, 11 figure

Viscosity and viscosity anomalies of model silicates and magmas: a numerical investigation

We present results for transport properties (diffusion and viscosity) using computer simulations. Focus is made on a densified binary sodium disilicate 2SiO$_2$-Na$_2$O (NS2) liquid and on multicomponent magmatic liquids (MORB, basalt). In the NS2 liquid, results show that a certain number of anomalies appear when the system is densified: the usual diffusivity maxima/minima is found for the network-forming ions (Si,O) whereas the sodium atom displays three distinct r\'egimes for diffusion. Some of these features can be correlated with the obtained viscosity anomaly under pressure, the latter being be fairly well reproduced from the simulated diffusion constant. In model magmas (MORB liquid), we find a plateau followed by a continuous increase of the viscosity with pressure. Finally, having computed both diffusion and viscosity independently, we can discuss the validity of the Eyring equation for viscosity which relates diffusion and viscosity. It is shown that it can be considered as valid in melts with a high viscosity. On the overall, these results highlight the difficulty of establishing a firm relationship between dynamics, structure and thermodynamics in complex liquids.Comment: 13 pages, 8 figure

Partial energies fluctuations and negative heat capacities

We proceed to a critical examination of the method used in nuclear fragmentation to exhibit signals of negative heat capacity. We show that this method leads to unsatisfactory results when applied to a simple and well controlled model. Discrepancies are due to incomplete evaluation of potential energies.Comment: Modified figures 3 and

A Little Big Bang scenario of fragmentation

We suggest a multifragmentation scenario in which fragments are produced at an early, high temperature and high density, stage of the reaction. In this scenario, self-bound clusters of particles in the hot and dense fluid are the precursors of the observed fragments. This solves a number of recurrent problems concerning the kinetic energies and the temperature of the fragments, encountered with the standard low density fragmentation picture. The possibility to recover the initial thermodynamic parameters from the inspection of the asymptotic fragment size and kinetic energy distributions is discussed

A "Little Big Bang" Scenario of Multifragmentation

We suggest a multifragmentation scenario in which fragments are produced at an early, high temperature and high density, stage of the reaction. In this scenario, self-bound clusters of particles in the hot and dense fluid are the precursors of the observed fragments. This solves a number of recurrent problems concerning the kinetic energies and the temperature of the fragments, encountered with the standard low density fragmentation picture. The possibility to recover the initial thermodynamic parameters from the inspection of the asymptotic fragment size and kinetic energy distributions is discussed.Comment: 15 pages, 12 figure

Percolation line of stable clusters in supercritical fluids

We predict that self-bound clusters of particles exist in the supercritical phase of simple fluids. These clusters, whose internal temperature is lower than the global temperature of the system, define a percolation line that starts at the critical point. This line should be physically observable. Possible experiments showing the validity of these predictions are discussed.Comment: 5 pages, 3 figures, corrected some typo