985 research outputs found

    The structure of superheavy elements newly discovered in the reaction of 86^{86}Kr with 208^{208}Pb

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    The structure of superheavy elements newly discovered in the 208^{208}Pb(86^{86}Kr,n) reaction at Berkeley is systematically studied in the Relativistic Mean Field (RMF) approach. It is shown that various usually employed RMF forces, which give fair description of normal stable nuclei, give quite different predictions for superheavy elements. Among the effective forces we tested, TM1 is found to be the good candidate to describe superheavy elements. The binding energies of the 293^{293}118 nucleus and its α−\alpha-decay daughter nuclei obtained using TM1 agree with those of FRDM within 2 MeV. Similar conclusion that TM1 is the good interaction is also drawn from the calculated binding energies for Pb isotopes with the Relativistic Continuum Hartree Bogoliubov (RCHB) theory. Using the pairing gaps obtained from RCHB, RMF calculations with pairing and deformation are carried out for the structure of superheavy elements. The binding energy, shape, single particle levels, and the Q values of the α−\alpha-decay QαQ_{\alpha} are discussed, and it is shown that both pairing correlation and deformation are essential to properly understand the structure of superheavy elements. A good agreement is obtained with experimental data on QαQ_{\alpha}. %Especially, the atomic number %dependence of QαQ_{\alpha} %seems to match with the experimental observationComment: 19 pages, 5 figure

    Phenolic Compound Profiles in Grape Skins of Cabernet Sauvignon, Merlot, Syrah and Marselan Cultivated in the Shacheng Area (China)

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    The phenolic compounds in the grape skins of Cabernet Sauvignon (CS), Merlot (ML), Syrah (SY) and Marselan (MS) from Shacheng, in China, were compared using HPLC-MS/MS. The results showed that the types and levels of phenolic compounds varied greatly with cultivars. Malvidin derivatives were the main anthocyanins. CS and ML showed a higher content of malvidin-3-O-(6-O-acetyl)-glucoside than malvidin-3-O-(trans-6-O- coumaryl)-glucoside, while SY and MS differed from CS and ML. ML had higher delphinidin and cyanidin derivatives, SY had higher peonidin derivatives, while malvidin and petunidin were higher in MS. The total content of flavonols, flavan-3-ols, phenolic acids and stilbenes in grape skins showed no difference among CS, ML and MS. Isorhamnetin-3-O-glucoside (CS, ML, MY), quercetin-3O-glucoside (SY), procyanidin trimer (SY, MS), procyanidin dimer (CS, ML), syringetin-3-O-glucoside, trans-cinnamic acid and resveratrol were the most abundant non-anthocyanin phenolic compounds. Cluster analysis showed that CS and ML, and SY and MS had similar phenolic profiles

    A Raman Study of Morphotropic Phase Boundary in PbZr1-xTixO3 at low temperatures

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    Raman spectra of PbZr1-xTixO3 ceramics with titanium concentration varying between 0.40 and 0.60 were measured at 7 K. By observing the concentration-frequency dependence of vibrational modes, we identified the boundaries among rhombohedral, monoclinic, and tetragonal ferroelectric phases. The analysis of the spectra was made in the view of theory group analysis making possible the assignment of some modes for the monoclinic phase.Comment: 5 pages, 4 figure

    Nuclear Skins and Halos in the Mean-Field Theory

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    Nuclei with large neutron-to-proton ratios have neutron skins, which manifest themselves in an excess of neutrons at distances greater than the radius of the proton distribution. In addition, some drip-line nuclei develop very extended halo structures. The neutron halo is a threshold effect; it appears when the valence neutrons occupy weakly bound orbits. In this study, nuclear skins and halos are analyzed within the self-consistent Skyrme-Hartree-Fock-Bogoliubov and relativistic Hartree-Bogoliubov theories for spherical shapes. It is demonstrated that skins, halos, and surface thickness can be analyzed in a model-independent way in terms of nucleonic density form factors. Such an analysis allows for defining a quantitative measure of the halo size. The systematic behavior of skins, halos, and surface thickness in even-even nuclei is discussed.Comment: 22 RevTeX pages, 22 EPS figures included, submitted to Physical Review

    A Measurement of Psi(2S) Resonance Parameters

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    Cross sections for e+e- to hadons, pi+pi- J/Psi, and mu+mu- have been measured in the vicinity of the Psi(2S) resonance using the BESII detector operated at the BEPC. The Psi(2S) total width; partial widths to hadrons, pi+pi- J/Psi, muons; and corresponding branching fractions have been determined to be Gamma(total)= (264+-27) keV; Gamma(hadron)= (258+-26) keV, Gamma(mu)= (2.44+-0.21) keV, and Gamma(pi+pi- J/Psi)= (85+-8.7) keV; and Br(hadron)= (97.79+-0.15)%, Br(pi+pi- J/Psi)= (32+-1.4)%, Br(mu)= (0.93+-0.08)%, respectively.Comment: 8 pages, 6 figure

    Measurements of the Mass and Full-Width of the ηc\eta_c Meson

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    In a sample of 58 million J/ψJ/\psi events collected with the BES II detector, the process J/Ïˆâ†’ÎłÎ·c\psi\to\gamma\eta_c is observed in five different decay channels: ÎłK+K−π+π−\gamma K^+K^-\pi^+\pi^-, ÎłÏ€+π−π+π−\gamma\pi^+\pi^-\pi^+\pi^-, ÎłK±KS0π∓\gamma K^\pm K^0_S \pi^\mp (with KS0→π+π−K^0_S\to\pi^+\pi^-), ÎłÏ•Ï•\gamma \phi\phi (with ϕ→K+K−\phi\to K^+K^-) and Îłppˉ\gamma p\bar{p}. From a combined fit of all five channels, we determine the mass and full-width of ηc\eta_c to be mηc=2977.5±1.0(stat.)±1.2(syst.)m_{\eta_c}=2977.5\pm1.0 ({stat.})\pm1.2 ({syst.}) MeV/c2c^2 and Γηc=17.0±3.7(stat.)±7.4(syst.)\Gamma_{\eta_c} = 17.0\pm3.7 ({stat.})\pm7.4 ({syst.}) MeV/c2c^2.Comment: 9 pages, 2 figures and 4 table. Submitted to Phys. Lett.

    Catalysts based on Co-Birnessite and Co-Todorokite for the efficient production of hydrogen by ethanol steam reforming

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    [EN] Two structured manganese oxides (Birnessite and Todorokite) containing Co have been studied in the steam reforming of ethanol. It has been found that both materials are active in the hydrogen production, exhibiting high values of conversion of ethanol and selectivities to hydrogen (100% and 70%, respectively). The best results have been obtained with the catalyst based on Todorokite material. Characterization by DRX, BET area, TPR and TEM has allowed to find that the excellent performance exhibited by this material could be attributed to the lower size of the Co metallic particles present in this sample (6 nm vs 12 nm in Birnessite). This lower size could be related to the especial microporous structure of Todorokite precursor, which could provide high-quality positions for the stabilization of the Co metal particles during calcination and reduction steps. Catalytic deactivation has also been considered. Deactivation was found higher for Todorokite-based catalyst, which presented the largest amount of deposited carbon (26.2 wt% for Co-TOD vs 10.6 wt% for Co-BIR). On the other hand, the degree of metal sintering was found similar in both catalysts. Therefore, the deactivation of the catalysts has been attributed primarily to the deposition of coke. The results presented here show that it is possible to prepare new catalysts based on manganese oxides with Birnessite and Todorokite structure and promoted with Co with high catalytic performance in the steam reforming of ethanol. (C) 2017 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.The doctor Javier Francisco Da Costa Serra acknowledges the CSIC for granted the scholarship predoctoral-JAE-CSIC. Moreover, Electronic Microscopy Service of UPV for TEM images.Da Costa Serra, JF.; Chica, A. (2018). Catalysts based on Co-Birnessite and Co-Todorokite for the efficient production of hydrogen by ethanol steam reforming. International Journal of Hydrogen Energy. 43(35):16859-16865. https://doi.org/10.1016/j.ijhydene.2017.12.114S1685916865433

    Partial Wave Analysis of J/Ïˆâ†’Îł(K+K−π+π−)J/\psi \to \gamma (K^+K^-\pi^+\pi^-)

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    BES data on J/Ïˆâ†’Îł(K+K−π+π−)J/\psi \to \gamma (K^+K^-\pi^+\pi^-) are presented. The K∗Kˉ∗K^*\bar K^* contribution peaks strongly near threshold. It is fitted with a broad 0−+0^{-+} resonance with mass M=1800±100M = 1800 \pm 100 MeV, width Γ=500±200\Gamma = 500 \pm 200 MeV. A broad 2++2^{++} resonance peaking at 2020 MeV is also required with width ∌500\sim 500 MeV. There is further evidence for a 2−+2^{-+} component peaking at 2.55 GeV. The non-K∗Kˉ∗K^*\bar K^* contribution is close to phase space; it peaks at 2.6 GeV and is very different from K∗K∗ˉK^{*}\bar{K^{*}}.Comment: 15 pages, 6 figures, 1 table, Submitted to PL
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