872 research outputs found
Size Distribution of Superparamagnetic Particles Determined by Magnetic Sedimentation
We report on the use of magnetic sedimentation as a means to determine the
size distribution of dispersed magnetic particles. The particles investigated
here are i) single anionic and cationic nanoparticles of diameter D = 7 nm and
ii) nanoparticle clusters resulting from electrostatic complexation with
polyelectrolytes and polyelectrolyte-neutral copolymers. A theoretical
expression of the sedimentation concentration profiles at the steady state is
proposed and it is found to describe accurately the experimental data. When
compared to dynamic light scattering, vibrating sample magnetometry and
cryogenic transmission electron microscopy, magnetic sedimentation exhibits a
unique property : it provides the core size and core size distribution of
nanoparticle aggregates.Comment: 9 pages - templated ACS - 7 figures - 1 tabl
Temperature Dependent Magnon-Phonon Coupling in bcc Fe from Theory and Experiment
An ab initio based framework for quantitatively assessing the phonon contribution due to magnon-phonon interactions and lattice expansion is developed. The theoretical results for bcc Fe are in very good agreement with high-quality phonon frequency measurements. For some phonon branches, the magnon-phonon interaction is an order of magnitude larger than the phonon shift due to lattice expansion, demonstrating the strong impact of magnetic short-range order even significantly above the Curie temperature. The framework closes the previous simulation gap between the ferro- and paramagnetic limits
Mass resolution optimization in a large isotopic composition experiment
A range-energy experiment was built to measure the isotopic composition of galactic cosmic rays. An enrichment of neutron rich isotopes, 22Ne and (25Mg + 26Mg) in particular, when compared to the solar composition is shown. A rich statistics measurement of these and other neutron-rich isotopes in the galactic flux yields information to the source of these particles. A computer simulation of the experiment was used to estimate the instrument resolution. The Cherenkov detector light collection efficiency, was calculated. Absorption of light in the radiator was considered to determine the optimum Cherenkov medium thickness. The experiment will determine the isotopic composition for the elements neon through argon in the energy range 300 to 800 MeV per nucleon
Dynamics of iron atoms across the pressure-induced Invar transition in Pd_3Fe
The ^(57)Fe phonon partial density of states (PDOS) in L1_2-ordered Pd_3Fe was studied at high pressures by nuclear resonant inelastic x-ray scattering (NRIXS) measurements and density functional theory (DFT) calculations. The NRIXS spectra showed that the stiffening of the ^(57)Fe PDOS with decreasing volume was slower from 12 to 24 GPa owing to the pressure-induced Invar transition in Pd_3Fe, with a change from a high-moment ferromagnetic (FM) state to a low-moment (LM) state observed by nuclear forward scattering. Force constants obtained from fitting to a Born–von Kármán model showed a relative softening of the first-nearest-neighbor (1NN) Fe-Pd longitudinal force constants at the magnetic transition. For the FM low-pressure state, the DFT calculations gave a PDOS and 1NN longitudinal force constants in good agreement with experiment, but discrepancies for the high-pressure LM state suggest the presence of short-range magnetic order
Spin Glass Ordering in Diluted Magnetic Semiconductors: a Monte Carlo Study
We study the temperature-dilution phase diagram of a site-diluted Heisenberg
antiferromagnet on a fcc lattice, with and without the Dzyaloshinskii-Moriya
anisotropic term, fixed to realistic microscopic parameters for (IIB=Cd, Hg, Zn). We show that the dipolar Dzyaloshinskii-Moriya anisotropy
induces a finite-temperature phase transition to a spin glass phase, at
dilutions larger than 80%. The resulting probability distribution of the order
parameter P(q) is similar to the one found in the cubic lattice
Edwards-Anderson Ising model. The critical exponents undergo large finite size
corrections, but tend to values similar to the ones of the
Edwards-Anderson-Ising model.Comment: 4 pages plus 3 postscript figure
Measurement of the electric dipole moments for transitions to rubidium Rydberg states via Autler-Townes splitting
We present the direct measurements of electric-dipole moments for
transitions with for Rubidium atoms. The
measurements were performed in an ultracold sample via observation of the
Autler-Townes splitting in a three-level ladder scheme, commonly used for
2-photon excitation of Rydberg states. To the best of our knowledge, this is
the first systematic measurement of the electric dipole moments for transitions
from low excited states of rubidium to Rydberg states. Due to its simplicity
and versatility, this method can be easily extended to other transitions and
other atomic species with little constraints. Good agreement of the
experimental results with theory proves the reliability of the measurement
method.Comment: 12 pages, 6 figures; figure 6 replaced with correct versio
Thermally Driven Electronic Topological Transition in FeTi
Ab initio molecular dynamics, supported by inelastic neutron scattering and nuclear resonant inelastic x-ray scattering, showed an anomalous thermal softening of the M^−_5 phonon mode in B2-ordered FeTi that could not be explained by phonon-phonon interactions or electron-phonon interactions calculated at low temperatures. A computational investigation showed that the Fermi surface undergoes a novel thermally driven electronic topological transition, in which new features of the Fermi surface arise at elevated temperatures. The thermally induced electronic topological transition causes an increased electronic screening for the atom displacements in the M^−_5 phonon mode and an adiabatic electron-phonon interaction with an unusual temperature dependence
Magnetic susceptibility of EuTe/PbTe Heisenberg superlattices: experimental and theoretical studies
We report results on the temperature dependence of the susceptibilities of a
set of MBE-grown short-period EuTe/PbTe antiferromagnetic superlattices having
different EuTe layer thicknesses. In-plane and orthogonal susceptibilities have
been measured and display a strong anisotropy at low temperature, confirming
the occurrence of a magnetic phase transition in the thicker samples, as seen
also in neutron diffraction studies. We suggest that dipolar interactions
stabilize antiferromagnetic long-range order in an otherwise isotropic system
and we present numerical and analytical results for the low-temperature
orthogonal susceptibility.Comment: 30 pages, 8 ps figures, RevTe
Paul trapping of radioactive 6He+ions and direct observation of their beta-decay
We demonstrate that abundant quantities of short-lived beta unstable ions can
be trapped in a novel transparent Paul trap and that their decay products can
directly be detected in coincidence. Low energy 6He+ (807 ms half-life) ions
were extracted from the SPIRAL source at GANIL, then decelerated, cooled and
bunched by means of the buffer gas cooling technique. More than 10^8 ions have
been stored over a measuring period of six days and about 10^5 decay
coincidences between the beta particles and the 6Li^{++} recoiling ions have
been recorded. The technique can be extended to other short-lived species,
opening new possibilities for trap assisted decay experiments.Comment: 4 pages, 4 figures, submitted to Phys.Rev.Let
Epitaxial and layer-by-layer growth of EuO thin films on yttria-stabilized cubic zirconia (001) using MBE distillation
We have succeeded in growing epitaxial and highly stoichiometric films of EuO
on yttria-stabilized cubic zirconia (YSZ) (001). The use of the Eu-distillation
process during the molecular beam epitaxy assisted growth enables the
consistent achievement of stoichiometry. We have also succeeded in growing the
films in a layer-by-layer fashion by fine tuning the Eu vs. oxygen deposition
rates. The initial stages of growth involve the limited supply of oxygen from
the YSZ substrate, but the EuO stoichiometry can still be well maintained. The
films grown were sufficiently smooth so that the capping with a thin layer of
aluminum was leak tight and enabled ex situ experiments free from trivalent Eu
species. The findings were used to obtain recipes for better epitaxial growth
of EuO on MgO (001).Comment: 10 pages, 15 figure
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