22 research outputs found

    Analysis of the Nuclear Structure of Rhenium-186 Using Neutron-Induced Reactions

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    Evaluated nuclear data for 186Re identify the majority of spin-parity assignments as tentative, with approximate values for the energies of several levels and transitions. In particular, the absence of known transitions that feed the J = 8+ isomer 186mRe motivates their discovery. This isomer, which has a half-life of 2 105 years, has a potential application in an isomer power source. Additionally, the isomer s role in certain nucleosynthesis processes is not well understood, so measured cross sections for transitions that feed the isomer would have astrophysical implications. Using the GErmanium Array for Neutron Induced Excitations (GEANIE) spectrometer at the Los Alamos Neutron Science Center (LANSCE), (n,2n ) and (n,n ) reactions in a 99.52% enriched 187Re target were used to obtain -ray spectra from 186Re and 187Re, respectively. The experimental data reveal 5 new transitions in186Re and 4 new transitions in 187Re. Similarities between the level schemes of 184Re and 186Re suggest that one of the newly-observed transitions in 186Re feeds the isomer from a level at 414.9 keV. The -ray energy measured for this transition implies an isomer energy of 148.2(5) keV, which is a significant improvement over the adopted value of 149(7) keV

    Nuclear Structure of \u3csup\u3e186\u3c/sup\u3eRe

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    The unstable odd-Z, odd-N isotope 186Re exists in a mid-shell deformed region of the chart of the nuclides where long-lived nuclear isomers are common. 186Re (ground-state half-life T1/2 = 3.7186 d) has an isomer with a half-life of ~2.0 x105 y. The 186mRe isomer is a candidate energy-storage medium for a radioisotope power source of military importance that would operate on the principle of isomer depletion. Data about levels and transitions above the 186mRe isomer, absent from the adopted level scheme for 186Re, are needed to identify a means of depleting the isomer. Four experiments were performed to investigate the 186Re level structure, which involved three different reactions..

    New transitions and feeding of the J\u3csup\u3eπ\u3c/sup\u3e=(8\u3csup\u3e+\u3c/sup\u3e) isomer in \u3csup\u3e186\u3c/sup\u3eRe

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    The spallation neutron source at the Los Alamos Neutron Science Center Weapons Neutron Research facility was used to populate excited states in 186Re via (n,2nγ) reactions on an enriched 187Re target. Gamma rays were detected with the GErmanium Array for Neutron Induced Excitations spectrometer, a Compton-suppressed array of 18 HPGe detectors. Incident neutron energies were determined by the time-of-flight technique and used to obtain γ-ray excitation functions for the purpose of identifying γ rays by reaction channel. Analysis of the singles γ-ray spectrum gated on the neutron energy range 10≤En≤25MeV resulted in five transitions and one level added to the 186Re level scheme. The additions include the placement of three γ rays at 266.7, 381.2, and 647.7 keV which have been identified as feeding the 2.0×105yr, Jπ=(8+) isomer and yield an improved value of 148.2(5)keV for the isomer energy. These transitions may have astrophysical implications related to the use of the Re-Os cosmochronometer. Abstract © APS

    Investigation of \u3csup\u3e186\u3c/sup\u3eRe via radiative thermal-neutron capture on \u3csup\u3e185\u3c/sup\u3eRe

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    Partial -ray production cross sections and the total radiative thermal-neutron capture cross section for the 185Re(n,)186Re reaction were measured using the Prompt Gamma Activation Analysis facility at the Budapest Research Reactor with an enriched 185Re target. The 186Re cross sections were standardized using well-known 35Cl(n,)36Cl cross sections from irradiation of a stoichiometric natReCl3 target. The resulting cross sections for transitions feeding the 186Re ground state from low-lying levels below a cutoff energy of Ec=746keV were combined with a modeled probability of ground-state feeding from levels above Ec to arrive at a total cross section of σ0=111(6)b for radiative thermal-neutron capture on 185Re. A comparison of modeled discrete-level populations with measured transition intensities led to proposed revisions for seven tentative spin-parity assignments in the adopted level scheme for 186Re. Additionally, 102 primary rays were measured, including 50 previously unknown. A neutron-separation energy of Sn=6179.59(5)keV was determined from a global least-squares fit of the measured -ray energies to the known 186Re decay scheme. The total capture cross section and separation energy results are comparable to earlier measurements of these values

    Developments in Capture- γ Libraries for Nonproliferation Applications

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    The neutron-capture reaction is fundamental for identifying and analyzing the γ-ray spectrum from an unknown assembly because it provides unambiguous information on the neutron-absorbing isotopes. Nondestructive-assay applications may exploit this phenomenon passively, for example, in the presence of spontaneous-fission neutrons, or actively where an external neutron source is used as a probe. There are known gaps in the Evaluated Nuclear Data File libraries corresponding to neutron-capture γ-ray data that otherwise limit transport-modeling applications. In this work, we describe how new thermal neutron-capture data are being used to improve information in the neutron-data libraries for isotopes relevant to nonproliferation applications. We address this problem by providing new experimentally-deduced partial and total neutron-capture reaction cross sections and then evaluate these data by comparison with statistical-model calculations

    INSPIRE (INvestigating Social and PractIcal suppoRts at the End of life): Pilot randomised trial of a community social and practical support intervention for adults with life-limiting illness

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    YesBACKGROUND: For most people, home is the preferred place of care and death. Despite the development of specialist palliative care and primary care models of community based service delivery, people who are dying, and their families/carers, can experience isolation, feel excluded from social circles and distanced from their communities. Loneliness and social isolation can have a detrimental impact on both health and quality of life. Internationally, models of social and practical support at the end of life are gaining momentum as a result of the Compassionate Communities movement. These models have not yet been subjected to rigorous evaluation. The aims of the study described in this protocol are: (1) to evaluate the feasibility, acceptability and potential effectiveness of The Good Neighbour Partnership (GNP), a new volunteer-led model of social and practical care/support for community dwelling adults in Ireland who are living with advanced life-limiting illness; and (2) to pilot the method for a Phase III Randomised Controlled Trial (RCT). DESIGN: The INSPIRE study will be conducted within the Medical Research Council (MRC) Framework for the Evaluation of Complex Interventions (Phases 0-2) and includes an exploratory two-arm delayed intervention randomised controlled trial. Eighty patients and/or their carers will be randomly allocated to one of two groups: (I) Intervention: GNP in addition to standard care or (II) Control: Standard Care. Recipients of the GNP will be asked for their views on participating in both the study and the intervention. Quantitative and qualitative data will be gathered from both groups over eight weeks through face-to-face interviews which will be conducted before, during and after the intervention. The primary outcome is the effect of the intervention on social and practical need. Secondary outcomes are quality of life, loneliness, social support, social capital, unscheduled health service utilisation, caregiver burden, adverse impacts, and satisfaction with intervention. Volunteers engaged in the GNP will also be assessed in terms of their death anxiety, death self efficacy, self-reported knowledge and confidence with eleven skills considered necessary to be effective GNP volunteers. DISCUSSION: The INSPIRE study addresses an important knowledge gap, providing evidence on the efficacy, utility and acceptability of a unique model of social and practical support for people living at home, with advanced life-limiting illness. The findings will be important in informing the development (and evaluation) of similar service models and policy elsewhere both nationally and internationally. TRIAL REGISTRATION: ISRCTN18400594 18(th) February 2015

    In-beam γ-ray Spectroscopy Studies of Medium-spin States in the Odd-odd Nucleus \u3csup\u3e186\u3c/sup\u3eRe

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    Excited states in 186Re with spins up to J=12ℏ were investigated in two separate experiments using 186W(d,2n) reactions at beam energies of 12.5 and 14.5 MeV. Two- and threefold γ-ray coincidence data were collected using the CAESAR and CAGRA spectrometers, respectively, each composed of Compton-suppressed high-purity germanium detectors. Analysis of the data revealed rotational bands built on several two-quasiparticle intrinsic states, including a long-lived Kπ=(8+) isomer. Configuration assignments were supported by an analysis of in-band properties, such as |gK−gR| values. The excitation energies of the observed intrinsic states were compared with results from multi-quasiparticle blocking calculations, based on the Lipkin-Nogami pairing approach, that included contributions from the residual proton-neutron interactions. Abstract ©2017 American Physical Societ

    Discourse, justification and critique: towards a legitimate digital copyright regime?

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    Digitization and the internet have posed an acute economic challenge to rights holders in the cultural industries. Faced with a threat to their form of capital accumulation from copyright infringement, rights holders have used discourse strategically in order to try and legitimate and strengthen their position in the digital copyright debate with governments and media users. In so doing, they have appealed to general justificatory principles – about what is good, right, and just – that provide some scope for opposition and critique, as other groups contest their interpretation of these principles and the evidence used to support them. In this article, we address the relative lack of academic attention paid to the role of discourse in copyright debates by analysing user-directed marketing campaigns and submissions to UK government policy consultations. We show how legitimacy claims are justified and critiqued, and conclude that amid these debates rests some hope of achieving a more legitimate policy resolution to the copyright wars – or at least the possibility of beginning a more constructive dialogue

    Suppression and azimuthal anisotropy of prompt and nonprompt J/psi production in PbPb collisions at root S-NN=2.76 TeV

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    The nuclear modification factor RAA and the azimuthal anisotropy coefficient v2 of prompt and nonprompt (i.e. those from decays of b hadrons) J/ψ mesons, measured from PbPb and pp collisions at sNN−−−√=2.76 TeV at the LHC, are reported. The results are presented in several event centrality intervals and several kinematic regions, for transverse momenta pT>6.5 GeV/c and rapidity |y|<2.4 , extending down to pT=3 GeV/c in the 1.6<|y|<2.4 range. The v2 of prompt J/ψ is found to be nonzero, but with no strong dependence on centrality, rapidity, or pT over the full kinematic range studied. The measured v2 of nonprompt J/ψ is consistent with zero. The RAA of prompt J/ψ exhibits a suppression that increases from peripheral to central collisions but does not vary strongly as a function of either y or pT in the fiducial range. The nonprompt J/ψ RAA shows a suppression which becomes stronger as rapidity or pT increases. The v2 and RAA of open and hidden charm, and of open charm and beauty, are compared
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