1,546 research outputs found

    Determination of spin and orbital magnetization in the ferromagnetic superconductor UCoGe

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    International audienceThe magnetism in the ferromagnetic superconductor UCoGe has been studied using a combination of magnetic Compton scattering, bulk magnetization, X-ray magnetic circular dichroism and electronic structure calculations, in order to determine the spin and orbital moments. The experimentally observed total spin moment, Ms, was found to be-0.24 ± 0.05 ”B at 5 T. By comparison with the total moment of 0.16 ± 0.01 ”B, the orbital moment, M l , was determined to be 0.40 ± 0.05 ”B. The U and Co spin moments were determined to be antiparallel. We find that the U 5f electrons carry a spin moment of Us ≈-0.30 ”B and that there is a Co spin moment of Cos ≈ 0.06 ”B induced via hybridization. The ratio U l /Us, of −1.3 ± 0.3, shows the U moment to be itinerant. In order to ensure an accurate description of the properties of 5f systems, and to provide a critical test of the theoretical approaches, it is clearly necessary to obtain experimental data for both the spin and orbital moments, rather than just the total magnetic moment. This can be achieved simply by measuring the spin moment with magnetic Compton scattering and comparing this to the total moment from bulk magnetizatio

    Global DNA methylation and cognitive and behavioral outcomes at 4 years of age: A cross‐sectional study

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    Background Accumulating evidence suggests that breastfeeding exclusivity and duration are positively associated with child cognition. This study investigated whether DNA methylation, an epigenetic mechanism modified by nutrient intake, may contribute to the link between breastfeeding and child cognition. The aim was to quantify the relationship between global DNA methylation and cognition and behavior at 4 years of age. Methods Child behavior and cognition were measured at age 4 years using the Wechsler Preschool and Primary Scale of Intelligence, third version (WPPSI‐III), and Child Behavior Checklist (CBC). Global DNA methylation (%5‐methylcytosines (%5mC)) was measured in buccal cells at age 4 years, using an enzyme‐linked immunosorbent assay (ELISA) commercial kit. Linear regression models were used to quantify the statistical relationships. Results Data were collected from 73 children recruited from the Women and Their Children's Health (WATCH) study. No statistically significant associations were found between global DNA methylation levels and child cognition or behavior (p > .05), though the estimates of effect were consistently negative. Global DNA methylation levels in males were significantly higher than in females (median %5mC: 1.82 vs. 1.03, males and females, respectively, (p < .05)). Conclusion No association was found between global DNA methylation and child cognition and behavior; however given the small sample, this study should be pooled with other cohorts in future meta‐analyses

    Screened Coulomb interactions in metallic alloys: II Screening beyond the single-site and atomic sphere approximations

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    A quantitative description of the configurational part of the total energy of metallic alloys with substantial atomic size difference cannot be achieved in the atomic sphere approximation: It needs to be corrected at least for the multipole moment interactions in the Madelung part of the one-electron potential and energy. In the case of a random alloy such interactions can be accounted for only by lifting the atomic sphere and single-site approximations, in order to include the polarization due to local environment effects. Nevertheless a simple parameterization of the screened Coulomb interactions for the ordinary single-site methods, including the generalized perturbation method, is still possible. We obtained such a parameterization for bulk and surface NiPt alloys, which allows one to obtain quantitatively accurate effective interactions in this system.Comment: 24 pages, 2 figure

    Grain coarsening behaviour of solution annealed Alloy 625 between 600–800°C

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    As with all alloys, the grain structure of the nickel-base superalloy 625 has a significant impact on its mechanical properties. Predictability of the grain structure evolution in this material is particularly pertinent because it is prone to inter-metallic precipitate formation both during manufacture and long term or high temperature service. To this end, analysis has been performed on the grain structure of Alloy 625 aged isothermally at temperatures between 600 and 800 °C for times up to 3000 h. Fits made according to the classical Arrhenius equation describing normal grain growth yield an average value for the activation energy of a somewhat inhomogeneous grain structure above 700 °C of 108.3±6.6 kJ mol−1 and 46.6±12.2 kJ mol−1 below 650 °C. Linear extrapolation between 650 and 700 °C produces a significantly higher value of 527.7±23.1 kJ mol−1. This result is ultimately a consequence of a high driving force, solute-impeded grain boundary migration process operating within the alloy. Comparison of the high and low temperature values with the activation energy for volume self-diffusion and grain boundary diffusion identifies the latter as the principle governing mechanism for grain growth in both instances. A decrease in the value of the time exponent (n) at higher temperatures despite a reduction in solute drag is attributable to the Zener pinning imposed by grain boundary M6C and M23C6 particles identified from Transmission Electron Microscopy (TEM) and Energy Dispersive X-ray Spectroscopy (EDXS) analysis. Vickers hardness results show the dominance of intermetallic intragranular precipitates in the governance of the mechanical properties of the material with grain coarsening being accompanied by a significant increase in hardness. Furthermore, the lack of any correlation with grain growth behaviour indicates these phases have no significant effect on the grain evolution of the material

    Long-Time Tails and Anomalous Slowing Down in the Relaxation of Spatially Inhomogeneous Excitations in Quantum Spin Chains

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    Exact analytic calculations in spin-1/2 XY chains, show the presence of long-time tails in the asymptotic dynamics of spatially inhomogeneous excitations. The decay of inhomogeneities, for t→∞t\to \infty , is given in the form of a power law (t/τQ)−ΜQ (t/\tau_{Q}) ^{-\nu_{Q}} where the relaxation time τQ\tau_{Q} and the exponent ÎœQ\nu_{Q} depend on the wave vector QQ, characterizing the spatial modulation of the initial excitation. We consider several variants of the XY model (dimerized, with staggered magnetic field, with bond alternation, and with isotropic and uniform interactions), that are grouped into two families, whether the energy spectrum has a gap or not. Once the initial condition is given, the non-equilibrium problem for the magnetization is solved in closed form, without any other assumption. The long-time behavior for t→∞t\to \infty can be obtained systematically in a form of an asymptotic series through the stationary phase method. We found that gapped models show critical behavior with respect to QQ, in the sense that there exist critical values QcQ_{c}, where the relaxation time τQ\tau_{Q} diverges and the exponent ÎœQ\nu_{Q} changes discontinuously. At those points, a slowing down of the relaxation process is induced, similarly to phenomena occurring near phase transitions. Long-lived excitations are identified as incommensurate spin density waves that emerge in systems undergoing the Peierls transition. In contrast, gapless models do not present the above anomalies as a function of the wave vector QQ.Comment: 25 pages, 2 postscript figures. Manuscript submitted to Physical Review

    Magnetoluminescence

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    Pulsar Wind Nebulae, Blazars, Gamma Ray Bursts and Magnetars all contain regions where the electromagnetic energy density greatly exceeds the plasma energy density. These sources exhibit dramatic flaring activity where the electromagnetic energy distributed over large volumes, appears to be converted efficiently into high energy particles and gamma-rays. We call this general process magnetoluminescence. Global requirements on the underlying, extreme particle acceleration processes are described and the likely importance of relativistic beaming in enhancing the observed radiation from a flare is emphasized. Recent research on fluid descriptions of unstable electromagnetic configurations are summarized and progress on the associated kinetic simulations that are needed to account for the acceleration and radiation is discussed. Future observational, simulation and experimental opportunities are briefly summarized.Comment: To appear in "Jets and Winds in Pulsar Wind Nebulae, Gamma-ray Bursts and Blazars: Physics of Extreme Energy Release" of the Space Science Reviews serie

    The electron heating rate and ion chemistry in the thermosphere above Wallops Island during the solar eclipse of 7 March 1970

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    An identical pair of thermosphere probes measured the N2 concentration and temperature, the ion composition and concentrations and the electron temperature up to 290 km about 30 min and 5 min before totality during the 7 March 1970 eclipse at Wallops Island. The rockets travelled similar trajectories thus permitting the purely temporal changes between nights to be resolved. The neutral temperature and N2 concentration changed little but the electron temperature decreased by as much as 20 per cent in the lower F-region. The ion concentration decreased by about 30 per cent in the F-region and about 50 per cent in the E-region, with little change in relative ion composition. The electron cooling rates decreased by a factor of 6 in the lower F-region, approximately in proportion to the change in visible solar disc. A smaller than expected decrease in the cooling rate below 150 km between the two flights indicates a hardening of the solar spectrum and suggests a significant heat contribution from the solar corona near totality. The ion composition measurements were consistent with solutions of the ion continuity equations. A proper fit required a factor of three enhancement of the flux below 200 A, an amount also consistent with the electron heat balance analysis. Reactions involving the minor ions N+ and N2+ were found to be important for the ion chemistry of the major ions O2+ and NO+, especially at the time of eclipse. The negligible response of the neutral atmosphere to the eclipse is reasonable considering the long time constants for the conductive and convective transport processes and the local nature of the disturbance.Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/34133/1/0000417.pd
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