Description of the Fission Process: Nuclear Models for Fission Dynamics

Nuclear fission is the splitting of a heavy nucleus into two or more fragments, a process that releases a substantial amount of energy. It is ubiquitous in modern applications, critical for national security, energy generation and reactor safeguards. Fission also plays an important role in understanding the astrophysical formation of elements in the universe. Eighty years after the discovery of the fission process, its theoretical understanding from first principles remains a great challenge. In this paper, we present promising new approaches to make more accurate predictions of fission observables

Collective enhancement in the exciton model

International audienceThe pre-equilibrium reaction mechanism is considered in the context of the exciton model. A modification to the one-particle one-hole state density is studied which can be interpreted as a collective enhancement. The magnitude of the collective enhancement is set by simulating the Lawrence Livermore National Laboratory (LLNL) pulsed-spheres neutron-leakage spectra. The impact of the collective enhancement is explored in the context of the highly deformed actinide, 239-Pu. A consequence of this enhancement is the removal of fictitious levels in the Distorted-Wave Born Approximation often used in modern nuclear reaction codes

Direct Mass Measurements to Inform the Behavior of <math display="inline"><mrow><mmultiscripts><mrow><mi>Sb</mi></mrow><mprescripts/><none/><mrow><mn>128</mn><mi mathvariant="normal">m</mi></mrow></mmultiscripts></mrow></math> in Nucleosynthetic Environments

International audienceNuclear isomer effects are pivotal in understanding nuclear astrophysics, particularly in the rapid neutron-capture process where the population of metastable isomers can alter the radioactive decay paths of nuclei produced during astrophysical events. The β-decaying isomer Sb128m was identified as potentially impactful since the β-decay pathway along the A=128 isobar funnels into this state bypassing the ground state. We report the first direct mass measurements of the Sb128 isomer and ground state using the Canadian Penning Trap mass spectrometer at Argonne National Laboratory. We find mass excesses of -84564.8(25)  keV and -84608.8(21)  keV, respectively, resulting in an excitation energy for the isomer of 43.9(33) keV. These results provide the first key nuclear data input for understanding the role of Sb128m in nucleosynthesis, and we show that it will influence the flow of the rapid neutron-capture process

69,71Co β-decay strength distributions from total absorption spectroscopy

Background: The rapid neutron capture process is one of the main nucleosynthesis processes of elements heavier than Fe. Uncertainties in nuclear properties, such as masses, half-lives, and β -delayed neutron probabilities can cause orders of magnitude of variation within astrophysical r-process simulations. Presently, theoretical models are used to make global predictions of various nuclear properties for the thousands of nuclei required for these simulations, and measurements are required to benchmark these models, especially far from stability. Purpose: β -decay strength distributions can be used to not only inform astrophysical r-process simulations, but also to provide a stringent test for theoretical calculations. The aim of this work is to provide accurate strength distributions for 69 , 71 Co β decay. Method: The technique of total absorption spectroscopy was used to measure the β decay of 69 , 71 Co for the first time at the National Superconducting Cyclotron Laboratory. The ions were implanted in a double-sided silicon strip detector at the center of the Summing NaI(Tl) detector and identified using standard particle identification methods. The response of the detection system to the β -decay electron and subsequent γ -ray radiation was fit to the observed experimental data using a χ 2 -minimization technique. Results: β -feeding intensities and Gamow-Teller strength distributions were extracted from the fits of the experimental data. The β -decay intensities show that there is a large percentage of feeding to levels above 2 MeV, which have not been observed in previous studies. The resultant β -feeding intensities and Gamow-Teller strength distributions were compared to shell model and quasiparticle random phase approximation (QRPA) calculations. Conclusions: Comparing experimentally determined β -decay strength distributions provides a test of models, which are commonly used for global β -decay properties for astrophysical calculations. This work highlights the importance of performing detailed comparisons of models to experimental data, particularly far from stability and as close to the r-process path as possible

β\beta-Decay Half-Lives of 55 Neutron-Rich Isotopes beyond the N=82 Shell Gap

International audienceThe $\beta$-decay half-lives of 55 neutron-rich nuclei $^{134-139}$Sn, $^{134-142}$Sb, $^{137-144}$Te, $^{140-146}$I, $^{142-148}$Xe, $^{145-151}$Cs, $^{148-153}$Ba, $^{151-155}$La were measured at the Radioactive Isotope Beam Factory (RIBF) employing the projectile fission fragments of $^{238}$U. The nuclear level structure, which relates to deformation, has a large effect on the half-lives. The impact of newly-measured half-lives on modeling the astrophysical origin of the heavy elements is studied in the context of $r$ process nucleosynthesis. For a wide variety of astrophysical conditions, including those in which fission recycling occurs, the half-lives have an important local impact on the second ($A$ $\approx$ 130) peak