Including nonlocality in exchange-correlation kernel from time-dependent current density functional theory: Application to the stopping power of electron liquids

We develop a scheme for building the scalar exchange-correlation (xc) kernel of time-dependent density functional theory (TDDFT) from the tensorial kernel of time-dependent {\em current} density functional theory (TDCDFT) and the Kohn-Sham current density response function. Resorting to the local approximation to the kernel of TDCDFT results in a nonlocal approximation to the kernel of TDDFT, which is free of the contradictions that plague the standard local density approximation (LDA) to TDDFT. As an application of this general scheme, we calculate the dynamical xc contribution to the stopping power of electron liquids for slow ions to find that our results are in considerably better agreement with experiment than those obtained using TDDFT in the conventional LDA.Comment: 6 pages, 3 figures, accepted to Phys. Rev.

Time-Dependent Quasiparticle Current Density Functional Theory of X-Ray Nonlinear Response Functions

A real-space representation of the current response of many-electron systems with possible applications to x-ray nonlinear spectroscopy and magnetic susceptibilities is developed. Closed expressions for the linear, quadratic and third-order response functions are derived by solving the adiabatic Time Dependent Current Density Functional (TDCDFT) equations for the single-electron density matrix in Liouville space.Comment: 11 page

Exact exchange-correlation potential for a time-dependent two electron system

We obtain an exact solution of the time-dependent Schroedinger equation for a two-electron system confined to a plane by an isotropic parabolic potential whose curvature is periodically modulated in time. From this solution we compute the exact time-dependent exchange correlation potential v_xc which enters the Kohn-Sham equation of time-dependent density functional theory. Our exact result provides a benchmark against which various approximate forms for v_xc can be compared. Finally v_xc is separated in an adiabatic and a pure dynamical part and it is shown that, for the particular system studied, the dynamical part is negligible.Comment: 23 pages, 6 figure

Magnetic susceptibility of insulators from first principles

We present an {\it ab initio} approach for the computation of the magnetic susceptibility $\chi$ of insulators. The approach is applied to compute $\chi$ in diamond and in solid neon using density functional theory in the local density approximation, obtaining good agreement with experimental data. In solid neon, we predict an observable dependence of $\chi$ upon pressure.Comment: Revtex, to appear in Physical Review Lette

Gilbert damping and spin Coulomb drag in a magnetized electron liquid with spin-orbit interaction

We present a microscopic calculation of the Gilbert damping constant for the magnetization of a two-dimensional spin-polarized electron liquid in the presence of intrinsic spin-orbit interaction. First we show that the Gilbert constant can be expressed in terms of the auto-correlation function of the spin-orbit induced torque. Then we specialize to the case of the Rashba spin-orbit interaction and we show that the Gilbert constant in this model is related to the spin-channel conductivity. This allows us to study the Gilbert damping constant in different physical regimes, characterized by different orderings of the relevant energy scales -- spin-orbit coupling, Zeeman coupling, momentum relaxation rate, spin-momentum relaxation rate, spin precession frequency -- and to discuss its behavior in various limits. Particular attention is paid to electron-electron interaction effects,which enter the spin conductivity and hence the Gilbert damping constant via the spin Coulomb drag coefficient.Comment: 18 pages, 8 figure

Spin transport in a unitary Fermi gas close to the BCS transition

We consider spin transport in a two-component ultracold Fermi gas with attractive interspecies interactions close to the BCS pairing transition. In particular, we consider the spin-transport relaxation rate and the spin-diffusion constant. Upon approaching the transition, the scattering amplitude is enhanced by pairing fluctuations. However, as the system approaches the transition, the spectral weight for excitations close to the Fermi level is decreased by the formation of a pseudogap. To study the consequence of these two competing effects, we determine the spin-transport relaxation rate and the spin-diffusion constant using both a Boltzmann approach and a diagrammatic approach. The former ignores pseudogap physics and finite lifetime effects. In the latter, we incorporate the full pseudogap physics and lifetime effects, but we ignore vertex corrections, so that we effectively calculate single-particle relaxation rates instead of transport relaxation rates. We find that there is qualitative agreement between these two approaches although the results for the transport coefficients differ quantitatively.Comment: 9 pages, 10 figure

Lorentz shear modulus of fractional quantum Hall states

We show that the Lorentz shear modulus of macroscopically homogeneous electronic states in the lowest Landau level is proportional to the bulk modulus of an equivalent system of interacting classical particles in the thermodynamic limit. Making use of this correspondence we calculate the Lorentz shear modulus of Laughlin's fractional quantum Hall states at filling factor $\nu=1/m$ ($m$ an odd integer) and find that it is equal to $\pm \hbar mn/4$, where $n$ is the density of particles and the sign depends on the direction of magnetic field. This is in agreement with the recent result obtained by Read in arXiv:0805.2507 and corrects our previous result published in Phys. Rev. B {\bf 76}, 161305 (R) (2007).Comment: 8 pages, 3 figure

Collective charge-density excitations of non-circular quantum dots in a magnetic field

Recent photoabsorption measurements have revealed a rich fine structure in the collective charge-density excitation spectrum of few-electron quantum dots in the presence of magnetic fields. We have performed systematic computational studies of the far-infrared density response of quantum dots, using time-dependent density-functional theory in the linear regime and treating the dots as two-dimensional disks. It turns out that the main characteristics observed in the experiment can be understood in terms of the electronic shell structure of the quantum dots. However, new features arise if a breaking of the circular symmetry of the dots is allowed, leading to an improved description of the experimental results.Comment: 18 pages, 5 figures, submitted to Phys. Rev.

Continuum elasticity theory of edge excitations in a two-dimensional electron liquid with finite range interactions

We make use of continuum elasticity theory to investigate the collective modes that propagate along the edge of a two-dimensional electron liquid or crystal in a magnetic field. An exact solution of the equations of motion is obtained with the following simplifying assumptions: (i) The system is {\it macroscopically} homogeneous and isotropic in the half-plane delimited by the edge (ii) The electron-electron interaction is of finite range due to screening by external electrodes (iii) The system is nearly incompressible. At sufficiently small wave vector $q$ we find a universal dispersion curve $\omega \sim q$ independent of the shear modulus. At larger wave vectors the dispersion can change its form in a manner dependent on the comparison of various length scales. We obtain analytical formulas for the dispersion and damping of the modes in various physical regimes.Comment: 3 figure