Drastic annealing effects in transport properties of single crystals of the YbNi2B2C heavy fermion system

We report temperature dependent resistivity, specific heat, magnetic susceptibility and thermoelectric power measurements made on the heavy fermion system YbNi2B2C, for both as grown and annealed single crystals. Our results demonstrate a significant variation in the temperature dependent electrical resistivity and thermoelectric power between as grown crystals and crystals that have undergone optimal (150 hour, 950 C) annealing, whereas the thermodynamic properties: (c_p(T) and chi(T)) remain almost unchanged. We interpret these results in terms of redistributions of local Kondo temperatures associated with ligandal disorder for a small (~ 1%) fraction of the Yb sites.Comment: 5 pages, 4 figures, submitted to PR

Revealing the state space of turbulent pipe flow by symmetry reduction

Symmetry reduction by the method of slices is applied to pipe flow in order to quotient the stream-wise translation and azimuthal rotation symmetries of turbulent flow states. Within the symmetry-reduced state space, all travelling wave solutions reduce to equilibria, and all relative periodic orbits reduce to periodic orbits. Projections of these solutions and their unstable manifolds from their $\infty$-dimensional symmetry-reduced state space onto suitably chosen 2- or 3-dimensional subspaces reveal their interrelations and the role they play in organising turbulence in wall-bounded shear flows. Visualisations of the flow within the slice and its linearisation at equilibria enable us to trace out the unstable manifolds, determine close recurrences, identify connections between different travelling wave solutions, and find, for the first time for pipe flows, relative periodic orbits that are embedded within the chaotic attractor, which capture turbulent dynamics at transitional Reynolds numbers.Comment: 24 pages, 12 figure

Numerical investigation of high-speed droplet impact using a multiscale two-fluid approach

A single droplet impact onto solid surfaces remains a fundamental and challenging topic in both experimental and numerical studies with significant importance in a plethora of industrial applications, ranging from printing technologies to fuel injection in internal combustion engines. Under high-speed impact conditions, additional complexities arise as a result of the prompt droplet splashing and the subsequent violent fragmentation; thus, different flow regimes and a vast spectrum of sizes for the produced secondary flow structures coexist in the flow field. The present work introduces a numerical methodology to capture the multiscale processes involved with respect to local topological characteristics. The proposed methodology concerns a compressible Σ-Υ two-fluid model with dynamic interface sharpening based on an advanced flow topology detection algorithm. The model has been developed in OpenFOAM® and provides the flexibility of dealing with the multiscale character of droplet splashing, by switching between a sharp and a diffuse interface within the Eulerian-Eulerian framework in segregated and dispersed flow regions, respectively. An additional transport equation for the interface surface area density (Σ) introduces important information for the sub-grid scale phenomena, which is exploited in the dispersed flow regions to provide an insight into the extended cloud of secondary droplets after impact on the target. A high-speed water droplet impact case has been examined and evaluated against new experimental data; these refer to a millimetre size droplet impacting a solid dry smooth surface at velocity as high as 150m/s, which corresponds to a Weber number of ~7.6×10^5. At the investigated impact conditions compressibility effects dominate the early stages of droplet splashing. A strong shock wave forms and propagates inside the droplet, where transonic Mach numbers occur; local Mach numbers up to 2.5 are observed for the expelled surrounding gas outside the droplet. The proposed numerical approach is found to capture relatively accurately the phenomena and provide significant information regarding the produced flow structure dimensions, which is not available from the experiment

Direct observation of Fe spin reorientation in single crystalline YbFe6Ge6

We have grown single crystals of YbFe6Ge6 and LuFe6Ge6 and characterized their anisotropic behaviour through low field magnetic susceptibility, field-dependent magnetization, resistivity and heat capacity measurements. The Yb+3 valency is confirmed by LIII XANES measurements. YbFe6Ge6 crystals exhibit a field-dependent, sudden reorientation of the Fe spins at about 63 K, a unique effect in the RFe6Ge6 family (R = rare earths) where the Fe ions order anti-ferromagnetically with Neel temperatures above 450 K and the R ions' magnetism appears to behave independently. The possible origins of this unusual behaviour of the ordered Fe moments in this compound are discussed.Comment: 12 pages, 8 figures, accepted in J. Phys.: Cond. Matte

Anomalous infrared spectra of hybridized phonons in type-I clathrate Ba8_8Ga16_{16}Ge30_{30}

The optical conductivity spectra of the rattling phonons in the clathrate Ba$_8$Ga$_{16}$Ge$_{30}$ are investigated in detail by use of the terahertz time-domain spectroscopy. The experiment has revealed that the lowest-lying vibrational mode of a Ba(2)$^{2+}$ ion consists of a sharp Lorentzian peak at 1.2 THz superimposed on a broad tail weighted in the lower frequency regime around 1.0 THz. With decreasing temperature, an unexpected linewidth broadening of the phonon peak is observed, together with monotonic softening of the phonon peak and the enhancement of the tail structure. These observed anomalies are discussed in terms of impurity scattering effects on the hybridized phonon system of rattling and acoustic phonons.Comment: Submitted to JPS

Collapse of the Gd3+Gd^{3+} ESR fine structure throughout the coherent temperature of the Gd-doped Kondo Semiconductor CeFe4P12CeFe_{4}P_{12}

Experiments on the $Gd^{3+}$ Electron Spin Resonance (ESR) in the filled skutterudite $Ce_{1-x}Gd_{x}Fe_{4}P_{12}$ ($x \approx 0.001$), at temperatures where the host resistivity manifests a smooth insulator-metal crossover, provides evidence of the underlying Kondo physics associated with this system. At low temperatures (below $T \approx K$), $Ce_{1-x}Gd_{x}Fe_{4}P_{12}$ behaves as a Kondo-insulator with a relatively large hybridization gap, and the $Gd^{3+}$ ESR spectra displays a fine structure with lorentzian line shape, typical of insulating media. The electronic gap is attributed to the large hybridization present in the coherent regime of a Kondo lattice, when Ce 4f-electrons cooperate with band properties at half-filling. Mean-field calculations suggest that the electron-phonon interaction is fundamental at explaining the strong 4f-electron hybridization in this filled skutterudite. The resulting electronic structure is strongly temperature dependent, and at about $T^{*} \approx 160 K$ the system undergoes an insulator-to-metal transition induced by the withdrawal of 4f-electrons from the Fermi volume, the system becoming metallic and non-magnetic. The $Gd^{3+}$ ESR fine structure coalesces into a single dysonian resonance, as in metals. Still, our simulations suggest that exchange-narrowing via the usual Korringa mechanism, alone, is not capable of describing the thermal behavior of the ESR spectra in the entire temperature region ($4.2$ - $300$ K). We propose that temperature activated fluctuating-valence of the Ce ions is the missing ingredient that, added to the usual exchange-narrowing mechanism, fully describes this unique temperature dependence of the $Gd^{3+}$ ESR fine structure observed in $Ce_{1-x}Gd_{x}Fe_{4}P_{12}$.Comment: 19 pages, 6 figure

On the transient nature of localized pipe flow turbulence

International audienceThe onset of shear flow turbulence is characterized by turbulent patches bounded by regions of laminar flow. At low Reynolds numbers localized turbulence relaminarizes, raising the question of whether it is transient in nature or becomes sustained at a critical threshold. We present extensive numerical simulations and a detailed statistical analysis of the lifetime data, in order to shed light on the sources of the discrepancies present in the literature. The results are in excellent quantitative agreement with recent experiments and show that turbulent lifetimes increase super-exponentially with Reynolds number. In addition, we provide evidence for a lower bound below which there are no meta-stable characteristics of the transients, i.e. the relaminarization process is no longer memoryless. Copyright © Cambridge University Press 2010

Angular momentum distribution of hot gas and implications for disk galaxy formation

We study the angular momentum profiles both for dark matter and for gas within virialized halos, using a statistical sample of halos drawn from cosmological hydrodynamics simulations. Three simulations have been analyzed, one is the ``non-radiative'' simulation, and the other two have radiative cooling. We find that the gas component on average has a larger spin and contains a smaller fraction of mass with negative angular momentum than its dark matter counterpart in the non-radiative model. As to the cooling models, the gas component shares approximately the same spin parameter as its dark matter counterpart, but the hot gas has a higher spin and is more aligned in angular momentum than dark matter, while the opposite holds for the cold gas. After the mass of negative angular momentum is excluded, the angular momentum profile of the hot gas component approximately follows the universal function originally proposed by Bullock et al. for dark matter, though the shape parameter $\mu$ is much larger for hot gas and is comfortably in the range required by observations of disk galaxies. Since disk formation is related to the distribution of hot gas that will cool, our study may explain the fact that the disk component of observed galaxies contains a smaller fraction of low angular momentum material than dark matter in halos.Comment: 30 pages, 12 figures, 4 tables, accepted for publication in Ap