Magnetic Soret effect: Application of the ferrofluid dynamics theory

The ferrofluid dynamics theory is applied to thermodiffusive problems in magnetic fluids in the presence of magnetic fields. The analytical form for the magnetic part of the chemical potential and the most general expression of the mass flux are given. By employing these results to experiments, global Soret coefficients in agreement with measurements are determined. Also an estimate for a hitherto unknown transport coefficient is made.Comment: 7 pages, 2 figure

Controlling anomalous stresses in soft field-responsive systems

We report a new phenomenon occurring in field-responsive suspensions: shear-induced anomalous stresses. Competition between a rotating field and a shear flow originates a multiplicity of anomalous stress behaviors in suspensions of bounded dimers constituted by induced dipoles. The great variety of stress regimes includes non-monotonous behaviors, multi-resonances, negative viscosity effect and blockades. The reversibility of the transitions between the different regimes and the self-similarity of the stresses make this phenomenon controllable and therefore applicable to modify macroscopic properties of soft condensed matter phasesComment: 5 pages, 6 figures, submitted to PR

Suppressing the Rayleigh-Taylor instability with a rotating magnetic field

The Rayleigh-Taylor instability of a magnetic fluid superimposed on a non-magnetic liquid of lower density may be suppressed with the help of a spatially homogeneous magnetic field rotating in the plane of the undisturbed interface. Starting from the complete set of Navier-Stokes equations for both liquids a Floquet analysis is performed which consistently takes into account the viscosities of the fluids. Using experimentally relevant values of the parameters we suggest to use this stabilization mechanism to provide controlled initial conditions for an experimental investigation of the Rayleigh-Taylor instability

Double Rosensweig instability in a ferrofluid sandwich structure

We consider a horizontal ferrofluid layer sandwiched between two layers of immiscible non-magnetic fluids. In a sufficiently strong vertical magnetic field the flat interfaces between magnetic and non-magnetic fluids become unstable to the formation of peaks. We theoretically investigate the interplay between these two instabilities for different combinations of the parameters of the fluids and analyze the evolving interfacial patterns. We also estimate the critical magnetic field strength at which thin layers disintegrate into an ordered array of individual drops

Phase Coexistence of a Stockmayer Fluid in an Applied Field

We examine two aspects of Stockmayer fluids which consists of point dipoles that additionally interact via an attractive Lennard-Jones potential. We perform Monte Carlo simulations to examine the effect of an applied field on the liquid-gas phase coexistence and show that a magnetic fluid phase does exist in the absence of an applied field. As part of the search for the magnetic fluid phase, we perform Gibbs ensemble simulations to determine phase coexistence curves at large dipole moments, $\mu$. The critical temperature is found to depend linearly on $\mu^2$ for intermediate values of $\mu$ beyond the initial nonlinear behavior near $\mu=0$ and less than the $\mu$ where no liquid-gas phase coexistence has been found. For phase coexistence in an applied field, the critical temperatures as a function of the applied field for two different $\mu$ are mapped onto a single curve. The critical densities hardly change as a function of applied field. We also verify that in an applied field the liquid droplets within the two phase coexistence region become elongated in the direction of the field.Comment: 23 pages, ReVTeX, 7 figure

Ferroplasmas: Magnetic Dust Dynamics in a Conducting Fluid

We consider a dusty plasma, in which the dust particles have a magnetic dipole moment. A Hall-MHD type of model, generalized to account for the intrinsic magnetization, is derived. The model is shown to be energy conserving, and the energy density and flux is derived. The general dispersion relation is then derived, and we show that kinetic Alfv\'en waves exhibit an instability for a low temperature and high density plasma. We discuss the implication of our results.Comment: 6 pages, 1 figur

Magnetization of polydisperse colloidal ferrofluids: Effect of magnetostriction

We exploit magnetostriction in polydisperse ferrofluids in order to generate nonlinear responses, and apply a thermodynamical method to derive the desired nonlinear magnetic susceptibility. For an ideal gas, this method has been demonstrated to be in excellent agreement with a statistical method. In the presence of a sinusoidal ac magnetic field, the magnetization of the polydisperse ferrofluid contains higher-order harmonics, which can be extracted analytically by using a perturbation approach. We find that the harmonics are sensitive to the particle distribution and the degree of field-induced anisotropy of the system. In addition, we find that the magnetization is higher in the polydisperse system than in the monodisperse one, as also found by a recent Monte Carlo simulation. Thus, it seems possible to detect the size distribution in a polydisperse ferrofluid by measuring the harmonics of the magnetization under the influence of magnetostriction.Comment: 23 pages, 4 figures. To be accepted for publication in Phys. Rev.

Parametric Forcing of Waves with Non-Monotonic Dispersion Relation: Domain Structures in Ferrofluids?

Surface waves on ferrofluids exposed to a dc-magnetic field exhibit a non-monotonic dispersion relation. The effect of a parametric driving on such waves is studied within suitable coupled Ginzburg-Landau equations. Due to the non-monotonicity the neutral curve for the excitation of standing waves can have up to three minima. The stability of the waves with respect to long-wave perturbations is determined $via$ a phase-diffusion equation. It shows that the band of stable wave numbers can split up into two or three sub-bands. The resulting competition between the wave numbers corresponding to the respective sub-bands leads quite naturally to patterns consisting of multiple domains of standing waves which differ in their wave number. The coarsening dynamics of such domain structures is addressed.Comment: 23 pages, 6 postscript figures, composed using RevTeX. Submitted to PR

A ferrofluid based neural network: design of an analogue associative memory

We analyse an associative memory based on a ferrofluid, consisting of a system of magnetic nano-particles suspended in a carrier fluid of variable viscosity subject to patterns of magnetic fields from an array of input and output magnetic pads. The association relies on forming patterns in the ferrofluid during a trainingdphase, in which the magnetic dipoles are free to move and rotate to minimize the total energy of the system. Once equilibrated in energy for a given input-output magnetic field pattern-pair the particles are fully or partially immobilized by cooling the carrier liquid. Thus produced particle distributions control the memory states, which are read out magnetically using spin-valve sensors incorporated in the output pads. The actual memory consists of spin distributions that is dynamic in nature, realized only in response to the input patterns that the system has been trained for. Two training algorithms for storing multiple patterns are investigated. Using Monte Carlo simulations of the physical system we demonstrate that the device is capable of storing and recalling two sets of images, each with an accuracy approaching 100%.Comment: submitted to Neural Network

Rotating Hele-Shaw cells with ferrofluids

We investigate the flow of two immiscible, viscous fluids in a rotating Hele-Shaw cell, when one of the fluids is a ferrofluid and an external magnetic field is applied. The interplay between centrifugal and magnetic forces in determining the instability of the fluid-fluid interface is analyzed. The linear stability analysis of the problem shows that a non-uniform, azimuthal magnetic field, applied tangential to the cell, tends to stabilize the interface. We verify that maximum growth rate selection of initial patterns is influenced by the applied field, which tends to decrease the number of interface ripples. We contrast these results with the situation in which a uniform magnetic field is applied normally to the plane defined by the rotating Hele-Shaw cell.Comment: 12 pages, 3 ps figures, RevTe