Quantum-enhanced capture of photons using optical ratchet states

Natural and artificial light harvesting systems often operate in a regime where the flux of photons is relatively low. Besides absorbing as many photons as possible it is therefore paramount to prevent excitons from annihilation via photon re-emission until they have undergone an irreversible energy conversion process. Taking inspiration from photosynthetic antenna structures, we here consider ring-like systems and introduce a class of states we call ratchets: excited states capable of absorbing but not emitting light. This allows our antennae to absorb further photons whilst retaining the excitations from those that have already been captured. Simulations for a ring of four sites reveal a peak power enhancement by up to a factor of 35 under ambient conditions owing to a combination of ratcheting and the prevention of emission through dark-state population. In the slow extraction limit the achievable power enhancement due to ratcheting alone exceeds 20%.Comment: major revision with improved model (all data and figures updated

Entanglement distribution for a practical quantum-dot-based quantum processor architecture

We propose a quantum dot (QD) architecture for enabling universal quantum information processing. Quantum registers, consisting of arrays of vertically stacked self-assembled semiconductor QDs, are connected by chains of in-plane self-assembled dots. We propose an entanglement distributor, a device for producing and distributing maximally entangled qubits on demand, communicated through in-plane dot chains. This enables the transmission of entanglement to spatially separated register stacks, providing a resource for the realization of a sizeable quantum processor built from coupled register stacks of practical size. Our entanglement distributor could be integrated into many of the present proposals for self-assembled QD-based quantum computation (QC). Our device exploits the properties of simple, relatively short, spin-chains and does not require microcavities. Utilizing the properties of self-assembled QDs, after distribution the entanglement can be mapped into relatively long-lived spin qubits and purified, providing a flexible, distributed, off-line resource. © IOP Publishing Ltd and Deutsche Physikalische Gesellschaft

Selective spin coupling through a single exciton

We present a novel scheme for performing a conditional phase gate between two spin qubits in adjacent semiconductor quantum dots through delocalized single exciton states, formed through the inter-dot Foerster interaction. We consider two resonant quantum dots, each containing a single excess conduction band electron whose spin embodies the qubit. We demonstrate that both the two-qubit gate, and arbitrary single-qubit rotations, may be realized to a high fidelity with current semiconductor and laser technology.Comment: 5 pages, 3 figures; published version, equation formatting improved, references adde

Bath induced coherence and the secular approximation

Finding efficient descriptions of how an environment affects a collection of discrete quantum systems would lead to new insights into many areas of modern physics. Markovian, or time-local, methods work well for individual systems, but for groups a question arises: does system-bath or inter-system coupling dominate the dissipative dynamics? The answer has profound consequences for the long-time quantum correlations within the system. We consider two bosonic modes coupled to a bath. By comparing an exact solution to different Markovian master equations, we find that a smooth crossover of the equations-of-motion between dominant inter-system and system-bath coupling exists - but requires a non-secular master equation. We predict a singular behaviour of the dynamics, and show that the ultimate failure of non-secular equations of motion is essentially a failure of the Markov approximation. Our findings justify the use of time-local theories throughout the crossover between system-bath dominated and inter-system-coupling dominated dynamics.PostprintPeer reviewe

Overcoming phonon-induced dephasing for indistinguishable photon sources

Reliable single photon sources constitute the basis of schemes for quantum communication and measurement based quantum computing. Solid state single photon sources based on quantum dots are convenient and versatile but the electronic transitions that generate the photons are subject to interactions with lattice vibrations. Using a microscopic model of electron-phonon interactions and a quantum master equation, we here examine phonon-induced decoherence and assess its impact on the rate of production, and indistinguishability, of single photons emitted from an optically driven quantum dot system. We find that, above a certain threshold of desired indistinguishability, it is possible to mitigate the deleterious effects of phonons by exploiting a three-level Raman process for photon production

Public opinion on energy crops in the landscape: considerations for the expansion of renewable energy from biomass

Public attitudes were assessed towards two dedicated biomass crops – Miscanthus and Short Rotation Coppice (SRC), particularly regarding their visual impacts in the landscape. Results are based on responses to photographic and computer-generated images as the crops are still relatively scarce in the landscape. A questionnaire survey indicated little public concern about potential landscape aesthetics but more concern about attendant built infrastructure. Focus group meetings and interviews indicated support for biomass end uses that bring direct benefits to local communities. Questions arise as to how well the imagery used was able to portray the true nature of these tall, dense, perennial plants but based on the responses obtained and given the caveat that there was limited personal experience of the crops, it appears unlikely that wide-scale planting of biomass crops will give rise to substantial public concern in relation to their visual impact in the landscape

Supercooled vortex liquid and quantitative theory of melting of the flux line lattice in type II superconductors

A metastable homogeneous state exists down to zero temperature in systems of repelling objects. Zero ''fluctuation temperature'' liquid state therefore serves as a (pseudo) ''fixed point'' controlling the properties of vortex liquid below and even around melting point. There exists Madelung constant for the liquid in the limit of zero temperature which is higher than that of the solid by an amount approximately equal to the latent heat of melting. This picture is supported by an exactly solvable large $N$ Ginzburg - Landau model in magnetic field. Based on this understanding we apply Borel - Pade resummation technique to develop a theory of the vortex liquid in type II superconductors. Applicability of the effective lowest Landau level model is discussed and corrections due to higher levels is calculated. Combined with previous quantitative description of the vortex solid the melting line is located. Magnetization, entropy and specific heat jumps along it are calculated. The magnetization of liquid is larger than that of solid by $1.8$ irrespective of the melting temperature. We compare the result with experiments on high $T_{c}$ cuprates $YBa_{2}Cu_{3}O_{7}$, $DyBCO$, low $T_{c}$ material $(K,Ba)BiO_{3}$ and with Monte Carlo simulations.Comment: 28 pages and 4 figures. Enlarged version of paper cond-mat/0107281 with many new content

A Robust Cross-Linking Strategy for Block Copolymer Worms Prepared via Polymerization-Induced Self-Assembly

A poly(glycerol monomethacrylate) (PGMA) chain transfer agent is chain-extended by reversible addition-fragmentation chain transfer (RAFT) statistical copolymerization of 2-hydroxypropyl methacrylate (HPMA) with glycidyl methacrylate (GlyMA) in concentrated aqueous solution via polymerization-induced self-assembly (PISA). A series of five free-standing worm gels is prepared by fixing the overall degree of polymerization of the core-forming block at 144 while varying its GlyMA content from 0 to 20 mol %. 1H NMR kinetics indicated that GlyMA is consumed much faster than HPMA, producing a GlyMA-rich sequence close to the PGMA stabilizer block. Temperature-dependent oscillatory rheological studies indicate that increasing the GlyMA content leads to progressively less thermoresponsive worm gels, with no degelation on cooling being observed for worms containing 20 mol % GlyMA. The epoxy groups in the GlyMA residues can be ring-opened using 3-aminopropyltriethoxysilane (APTES) in order to prepare core cross-linked worms via hydrolysis-condensation with the siloxane groups and/or hydroxyl groups on the HPMA residues. Perhaps surprisingly, 1H NMR analysis indicates that the epoxy-amine reaction and the intermolecular cross-linking occur on similar time scales. Cross-linking leads to stiffer worm gels that do not undergo degelation upon cooling. Dynamic light scattering studies and TEM analyses conducted on linear worms exposed to either methanol (a good solvent for both blocks) or anionic surfactant result in immediate worm dissociation. In contrast, cross-linked worms remain intact under such conditions, provided that the worm cores comprise at least 10 mol % GlyMA

Spin Star as Switch for Quantum Networks

Quantum state transfer is an important task in quantum information processing. It is known that one can engineer the couplings of a one-dimensional spin chain to achieve the goal of perfect state transfer. To leverage the value of these spin chains, a spin star is potentially useful for connecting different parts of a quantum network. In this work, we extend the spin-chain engineering problem to the problems with a topology of a star network. We show that a permanently coupled spin star can function as a network switch for transferring quantum states selectively from one node to another by varying the local potentials only. Together with one-dimensional chains, this result allows applications of quantum state transfer be applied to more general quantum networks.Comment: 10 pages, 2 figur