590 research outputs found
Collective Singlet Excitations and Evolution of Raman Spectral Weights in the 2D Spin Dimer Compound SrCu2(BO3)2
We present a Raman light scattering study of the two-dimensional quantum spin
system SrCu2(BO3)2 and show that the magnetic excitation spectrum has a rich
structure, including several well-defined bound state modes at low temperature,
and a scattering continuum and quasielastic light scattering contributions at
high temperature. The key to the understanding of the unique features of
SrCu2(BO3)2 is the presence of strong interactions between well-localized
triplet excitations in the network of orthogonal spin dimers realized in this
compound. Based on our analysis of the Heisenberg model relevant for this
material, we argue that the collective excitations involving two and
three-particle singlet bound states have large binding energies and are
observed as well-defined peaks in the Raman spectrum.Comment: 5 pages, 2 figures. Revised version, to appear in Phys. Rev. Lett.
(2000
Longitudinal magnon in the tetrahedral spin system Cu2Te2O5Br2 near quantum criticality
We present a comprehensive study of the coupled tetrahedra-compound
Cu2Te2O5Br2 by theory and experiments in external magnetic fields. We report
the observation of a longitudinal magnon in Raman scattering in the ordered
state close to quantum criticality. We show that the excited
tetrahedral-singlet sets the energy scale for the magnetic ordering temperature
T_N. This energy is determined experimentally. The ordering temperature T_N has
an inverse-log dependence on the coupling parameters near quantum criticality
Ground state order and spin-lattice coupling in tetrahedral spin systems Cu2Te2O5X2
High-resolution ac susceptibility and thermal conductivity measurement on
Cu2Te2O5X2(X=Br,Cl) single crystals are reported. For Br-sample, sample
dependence prevents to distinguish between possibilities of magnetically
ordered and spin-singlet ground states. In Cl-sample a three-dimensional
transition at 18.5 K is accompanied by almost isotropic behavior of
susceptibility and almost switching behavior of thermal conductivity. Thermal
conductivity studies suggest the presence of a tremendous spin-lattice coupling
characterizing Cl- but not Br-sample. Below the transition Cl-sample is in a
complex magnetic state involving AF order but also the elements consistent with
the presence of a gap in the excitation spectrum.Comment: version accepted for publication in Phys.Rev.B-Rapid Communicatio
Magnetism of a tetrahedral cluster spin-chain
We discuss the magnetic properties of a dimerized and completely frustrated
tetrahedral spin-1/2 chain. Using a combination of exact diagonalization and
bond-operator theory the quantum phase diagram is shown to incorporate a
singlet-product, a dimer, and a Haldane phase. In addition we consider one-,
and two-triplet excitations in the dimer phase and evaluate the magnetic Raman
cross section which is found to be strongly renormalized by the presence of a
two-triplet bound state. The link to a novel tellurate materials is clarified.Comment: 8 pages, 8 figure
Density of a gas of spin polarized fermions in a magnetic field
For a fermion gas with equally spaced energy levels that is subjected to a
magnetic field, the particle density is calculated. The derivation is based on
the path integral approach for identical particles, in combination with the
inversion techniques for the generating function of the static response
functions. Explicit results are presented for the ground state density as a
function of the magnetic field with a number of particles ranging from 1 to 45.Comment: 9 pages, 8 figures; To appear in Phys. Rev. E on December 1, 2000;
e-mail addresses: [email protected], [email protected],
[email protected], [email protected]
Structural and magnetic dimers in the spin-gapped system CuTe2O5
We investigated the magnetic properties of the system CuTe2O5 by
susceptibility and electron spin resonance measurements. The anisotropy of the
effective g-factors and the ESR linewidth indicates that the anticipated
structural dimer does not correspond to the singlet-forming magnetic dimer.
Moreover, the spin susceptibility of CuTe2O5 can only be described by taking
into account interdimer interactions of the same order of magnitude than the
intradimer coupling. Analyzing the exchange couplings in the system we identify
the strongest magnetic coupling between two Cu ions to be mediated by
super-super exchange interaction via a bridging Te ligand, while the
superexchange coupling between the Cu ions of the structural dimer only results
in the second strongest coupling
Effects of climate warming and declining species richness in grassland model ecosystems: acclimation of CO2 fluxes
To study the effects of warming and declining species richness on the carbon balance of grassland communities, model ecosystems containing one, three or nine species were exposed to ambient and elevated (ambient +3°C) air temperature. In this paper, we analyze measured ecosystem CO2 fluxes to test whether ecosystem photosynthesis and respiration had acclimated to warming after 28 months of continuous heating, and whether the degree of acclimation depended on species richness. In order to test whether acclimation occurred, short term temperature response curves were established for all communities in both treatments. At similar temperatures, lower flux rates in the heated communities as compared to the unheated communities would indicate thermal acclimation. Because plant cover was significantly higher in the heated treatment, we normalized the data for plant cover. Subsequently, down-regulation of both photosynthesis and respiration was observed. Although CO2 fluxes were larger in communities with higher species richness, species richness did not affect the degree of acclimation to warming. These results imply that models need to take thermal acclimation into account to simulate photosynthesis and respiration in a warmer world.This research was funded by the Fund for
Scientific Research – Flanders (Belgium) as project “effects of biodiversity loss and climate warming on carbon sequestration
mechanisms in terrestrial ecosystems”, contract #G.0434.03N. H. J. De Boeck holds a grant from the Institute for the Promotion
of Innovation by science and Technology in Flanders. P. Serrano-Ortiz benefits from a pre-doctoral grant from the Junta
de Andalucía
Dopant-Bound Spinons in Cu_(1-x)Zn_xGeO_3
Polarized inelastic light scattering experiments on Cu_(1-x)Zn_xGeO_3 (0<= x
0 a new distinct mode at nearly half the
energy of the singlet response below the spin-Peierls transition. The
temperature, magnetic field, polarization, and doping dependencies of this mode
are similar to those of the singlet bound state. The data are interpreted in
terms of a spinon-assisted light scattering process. Position and form of the
peak provide strong evidence for the presence of dopant-bound spinons in
Cu_(1-x)Zn_xGeO_3.Comment: 4 pages, Latex with 3 figures, including EPL style files, Eur. Phys.
Lett. in pres
Spin gap behavior and charge ordering in \alpha^{\prime}-NaV_2O_5 probed by light scattering
We present a detailed analysis of light scattering experiments performed on
the quarter-filled spin ladder compound -NaVO for
the temperature range 5 KT300 K. This system undergoes a phase
transition into a singlet ground state at T=34 K accompanied by the formation
of a super structure. For T34 K several new modes were detected. Three of
these modes are identified as magnetic bound states. Experimental evidence for
charge ordering on the V sites is detected as an anomalous shift and splitting
of a V-O vibration at 422 cm for temperatures above 34 K. The smooth and
crossover-like onset of this ordering at T= 80 K is accompanied by
pretransitional fluctuations both in magnetic and phononic Raman scattering. It
resembles the effect of stripe order on the super structure intensities in
LaNiO.Comment: 36 pages, 11 figures, accepted for publication in PRB (sept.99
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