Spin correlations among the charge carriers in an ordered stripe phase

We have observed a diffuse component to the low-energy magnetic excitation spectrum of stripe-ordered La5/3Sr1/3NiO4 probed by neutron inelastic scattering. The diffuse scattering forms a square pattern with sides parallel and perpendicular to the stripe directions. The signal is dispersive, with a maximum energy of ~10 meV. Probed at 2 meV the scattering decreases in strength with increasing temperature, and is barely visible at 100 K. We argue that the signal originates from dynamic, quasi- one-dimensional, antiferromagnetic correlations among the stripe electrons.Comment: 4 pages, 4 figures. To be published in Physical Review Letter

Electronic structure and magnetic properties of the spin-1/2 Heisenberg system CuSe2O5

A microscopic magnetic model for the spin-1/2 Heisenberg chain compound CuSe2O5 is developed based on the results of a joint experimental and theoretical study. Magnetic susceptibility and specific heat data give evidence for quasi-1D magnetism with leading antiferromagnetic (AFM) couplings and an AFM ordering temperature of 17 K. For microscopic insight, full-potential DFT calculations within the local density approximation (LDA) were performed. Using the resulting band structure, a consistent set of transfer integrals for an effective one-band tight-binding model was obtained. Electronic correlations were treated on a mean-field level starting from LDA (LSDA+U method) and on a model level (Hubbard model). In excellent agreement of experiment and theory, we find that only two couplings in CuSe2O5 are relevant: the nearest-neighbour intra-chain interaction of 165 K and a non-frustrated inter-chain coupling of 20 K. From a comparison with structurally related systems (Sr2Cu(PO4)2, Bi2CuO4), general implications for a magnetic ordering in presence of inter-chain frustration are made.Comment: 20 pages, 8 figures, 3 table

The strength of frustration and quantum fluctuations in LiVCuO4

For the 1D-frustrated ferromagnetic J_1-J_2 model with interchain coupling added, we analyze the dynamical and static structure factor S(k,omega), the pitch angle phi of the magnetic structure, the magnetization curve of edge-shared chain cuprates, and focus on LiCuVO4 for which neither a perturbed spinon nor a spin wave approach can be applied. phi is found to be most sensitive to the interplay of frustration and quantum fluctuations. For LiVCuO4 the obtained exchange parameters J are in accord with the results for a realistic 5-band extended Hubbard model and LSDA + U predictions yielding alpha=J_2/|J_1| about 0.75 in contrast to 5.5 > alpha > 1.42 suggested in the literature. The alpha-regime of the empirical phi-values in NaCu2O2 and linarite are considered, too.Comment: 7 pages, 7 figures, (1 figure added), improved text including also the abstract (the present second version has been submitted to EPL 26.10.2011, so far with one missing first referee report

Dominant ferromagnetism in the spin-1/2 half-twist ladder 334 compounds, Ba3Cu3In4O12 and Ba3Cu3Sc4O12

The magnetic properties of polycrystalline samples of Ba3Cu3In4O12 (In-334) and Ba3Cu3Sc4O12 (Sc-334) are reported. Both 334 phases have a structure derived from perovskite, with CuO4 squares interconnected to form half-twist ladders along the c-axis. The Cu-O-Cu angles, ~ 90o, and the positive Weiss temperatures indicate the presence of significant ferromagnetic (FM) interactions along the Cu ladders. At low temperatures, T < 20 K, sharp transitions in the magnetic susceptibility and heat capacity measurements indicate three-dimensional (3D) antiferromagnetic (AFM) ordering at TN. TN is suppressed on application of a field and a complex magnetic phase diagram with three distinct magnetic regimes below the upper critical field can be inferred from our measurements. The magnetic interactions are discussed in relation to a modified spin-1/2 FM-AFM model and the 334 half-twist ladder is compared to other 2-rung ladder spin-1/2 systems.Comment: 20 pages, 7 figure

NMR relaxation rate in the field-induced octupolar liquid phase of spin-1/2 J1-J2 frustrated chains

In the spin-1/2 frustrated chain with nearest-neighbor ferromagnetic exchange J1 and next-nearest-neighbor antiferromagnetic exchange J2 under magnetic field, magnetic multipolar-liquid (quadrupolar, octupolar, and hexadecapolar) phases are widely expanded from the saturation down to a low-field regime. Recently, we have clarified characteristic temperature and field dependence of the NMR relaxation rate 1/T_1 in the quadrupolar phase. In this paper, we examine those of 1/T_1 in the octupolar phase combining field theoretical method with numerical data. The relevance of the results to quasi one-dimensional J1-J2 magnets such as PbCuSO4(OH)2, Rb2Cu2Mo3O12 and Li2ZrCuO4 is shortly discussed.Comment: 6 pages (1 column), 3 figure

Population level effectiveness of implementing collaborative care management for depression

AbstractObjectiveCare management is feasible to deploy in routine care, and the depression outcomes of patients reached by this evidence-based practice are similar to those observed in randomized controlled trials. However, no studies have estimated the population level effectiveness of care management when deployed in routine care. Population level effectiveness depends on both reach into the target population and the clinical effectiveness for those reached.MethodThis multisite hybrid Type 3 effectiveness–implementation study employed a pre-post, quasi-experimental design. The study was conducted at 22 Veterans Affairs community-based outpatient clinics. Evidence-based quality improvement was used as the facilitation strategy to promote adoption. Medication possession ratios (MPRs) were calculated for 1558 patients with an active antidepressant prescription. Differences in treatment response rates at implementation and control sites were estimated from observed differences in MPR.ResultsReach into the target population at implementation sites was 10.3%. Patients at implementation sites had a significantly higher probability of having MPR≥0.9 than patients at control sites [odds ratio=1.38, confidence interval95=(1.07, 1.78), P=.01]. This increase in MPR was estimated to yield a 1% point increase in response rates.ConclusionsWhile depression care management improves outcomes for patients receiving services, low levels of reach can reduce overall population level effectiveness

Jahn-Teller versus quantum effects in the spin-orbital material LuVO3

We report on combined neutron and resonant x-ray scattering results, identifying the nature of the spin-orbital ground state and magnetic excitations in LuVO3 as driven by the orbital parameter. In particular, we distinguish between models based on orbital Peierls dimerization, taken as a signature of quantum effects in orbitals, and Jahn-Teller distortions, in favor of the latter. In order to solve this long-standing puzzle, polarized neutron beams were employed as a prerequisite in order to solve details of the magnetic structure, which allowed quantitative intensity-analysis of extended magnetic excitation data sets. The results of this detailed study enabled us to draw definite conclusions about classical vs quantum behavior of orbitals in this system and to discard the previous claims about quantum effects dominating the orbital physics of LuVO3 and similar systems.Comment: Phys. Rev. B 91, 161104(R) (2015