41 research outputs found

    Nonlinear order parameter oscillations and lattice coupling in strongly-driven charge-density-wave systems

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    The anharmonic response of charge-density wave (CDW) order to strong laser-pulse perturbations in 1T-TaS_2 and TbTe_3 is investigated by means of a multiple-pump-pulse time-resolved femtosecond optical spectroscopy. We observe remarkable anharmonic effects hitherto undetected in the systems exhibiting collective charge ordering. The efficiency for additional excitation of the amplitude mode by a laser pulse becomes periodically modulated after the mode is strongly excited into a coherently oscillating state. A similar effect is observed also for some other phonons, where the cross-modulation at the amplitude-mode frequency indicates anharmonic interaction of those phonons with the amplitude mode. By analyzing the observed phenomena in the framework of time-dependent Ginzburg-Landau theory we attribute the effects to the anharmonicity of the mode potentials inherent to the broken symmetry state of the CDW systems

    Tracking Cooper Pairs in a Cuprate Superconductor by Ultrafast Angle-Resolved Photoemission

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    In high-temperature superconductivity, the process that leads to the formation of Cooper pairs, the fundamental charge carriers in any superconductor, remains mysterious. We use a femtosecond laser pump pulse to perturb superconducting Bi2Sr2CaCu2O8+{\delta}, and study subsequent dynamics using time- and angle-resolved photoemission and infrared reflectivity probes. Gap and quasiparticle population dynamics reveal marked dependencies on both excitation density and crystal momentum. Close to the d-wave nodes, the superconducting gap is sensitive to the pump intensity and Cooper pairs recombine slowly. Far from the nodes pumping affects the gap only weakly and recombination processes are faster. These results demonstrate a new window into the dynamical processes that govern quasiparticle recombination and gap formation in cuprates.Comment: 22 pages, 9 figure

    Relaxation Dynamics of Photoinduced Changes in the Superfluid Weight of High-Tc Superconductors

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    In the transient state of d-wave superconductors, we investigate the temporal variation of photoinduced changes in the superfluid weight. We derive the formula that relates the nonlinear response function to the nonequilibrium distribution function. The latter qunatity is obtained by solving the kinetic equation with the electron-electron and the electron-phonon interaction included. By numerical calculations, a nonexponential decay is found at low temperatures in contrast to the usual exponential decay at high temperatures. The nonexponential decay originates from the nonmonotonous temporal variation of the nonequilibrium distribution function at low energies. The main physical process that causes this behavior is not the recombination of quasiparticles as previous phenomenological studies suggested, but the absorption of phonons.Comment: 18 pages, 12 figures; to be published in J. Phys. Soc. Jpn. Vol. 80, No.

    Nodal quasiparticle meltdown in ultra-high resolution pump-probe angle-resolved photoemission

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    High-TcT_c cuprate superconductors are characterized by a strong momentum-dependent anisotropy between the low energy excitations along the Brillouin zone diagonal (nodal direction) and those along the Brillouin zone face (antinodal direction). Most obvious is the d-wave superconducting gap, with the largest magnitude found in the antinodal direction and no gap in the nodal direction. Additionally, while antinodal quasiparticle excitations appear only below TcT_c, superconductivity is thought to be indifferent to nodal excitations as they are regarded robust and insensitive to TcT_c. Here we reveal an unexpected tie between nodal quasiparticles and superconductivity using high resolution time- and angle-resolved photoemission on optimally doped Bi2_2Sr2_2CaCu2_2O8+δ_{8+\delta}. We observe a suppression of the nodal quasiparticle spectral weight following pump laser excitation and measure its recovery dynamics. This suppression is dramatically enhanced in the superconducting state. These results reduce the nodal-antinodal dichotomy and challenge the conventional view of nodal excitation neutrality in superconductivity.Comment: 7 pages, 3 figure. To be published in Nature Physic

    Froehlich Polaron and Bipolaron: Recent Developments

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    It is remarkable how the Froehlich polaron, one of the simplest examples of a Quantum Field Theoretical problem, as it basically consists of a single fermion interacting with a scalar Bose field of ion displacements, has resisted full analytical or numerical solution at all coupling since 1950, when its Hamiltonian was first written. The field has been a testing ground for analytical, semi-analytical, and numerical techniques, such as path integrals, strong-coupling perturbation expansion, advanced variational, exact diagonalisation (ED), and quantum Monte Carlo (QMC) techniques. This article reviews recent developments in the field of continuum and discrete (lattice) Froehlich (bi)polarons starting with the basics and covering a number of active directions of research.Comment: 131 pages, 17 figures, 409 references, appear in Reports on Progress in Physic

    Effect of organic, conventional and mixed cultivation practices on soil microbial community structure and nematode abundance in a cultivated onion crop

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    pre-print, non-peer-reviewedBACKGROUND: Responses of the soil microbial and nematode community to organic and conventional agricultural practices were studied using the Teagasc Kinsealy Systems Comparison trial as the experimental system. The trial is a long term field experiment which divides conventional and organic agriculture into component pest-control and soil treatment practices. We hypothesised that management practices would affect soil ecology and used community level physiological profiles (CLPP), microbial and nematode counts, and denaturing gradient gel electrophoresis (DGGE) to characterise soil microbial communities in plots used for onion (Allium cepa L.) cultivation. RESULTS: Microbial activity and culturable bacterial counts were significantly higher under fully organic management. Culturable fungi, actinomycete and nematode counts showed a consistent trend towards higher numbers under fully organic management but these data were not statistically significant. No differences were found in the fungal/bacterial ratio. DGGE banding patterns and sequencing of excised bands showed clear differences between treatments. Putative onion fungal pathogens were predominantly sequenced under conventional soil treatment practices whilst putative soil suppressive bacterial species were predominantly sequenced from the organic pest-control treatment plots. CONCLUSION: Organic management increased microbial activity and diversity. Sequence data was indicative of differences in functional groups and warrants further investigation.Irish Research Council for Science, Engineering and TechnologyOGTThe Irish Department of Agriculture, Fisheries and Food (FIRM 06/NITARFC6) is gratefully acknowledged for financial support. TLL thanks IRCSET and OGT for financial support
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