5,302 research outputs found
Reconsideration of Second Harmonic Generation from neat Air/Water Interface: Broken of Kleinman Symmetry from Dipolar Contribution
It has been generally accepted that there are significant quadrupolar and
bulk contributions to the second harmonic generation (SHG) reflected from the
neat air/water interface, as well as common liquid interfaces. Because there
has been no general methodology to determine the quadrupolar and bulk
contributions to the SHG signal from a liquid interface, this conclusion was
reached based on the following two experimental phenomena. Namely, the broken
of the macroscopic Kleinman symmetry, and the significant temperature
dependence of the SHG signal from the neat air/water interface. However,
because sum frequency generation vibrational spectroscopy (SFG-VS) measurement
of the neat air/water interface observed no apparent temperature dependence,
the temperature dependence in the SHG measurement has been reexamined and
proven to be an experimental artifact. Here we present a complete microscopic
analysis of the susceptibility tensors of the air/water interface, and show
that dipolar contribution alone can be used to address the issue of broken of
the macroscopic Kleinman symmetry at the neat air/water interface. Using this
analysis, the orientation of the water molecules at the interface can be
obtained, and it is consistent with the measurement from SFG-VS. Therefore, the
key rationales to conclude significantly quadrupolar and bulk contributions to
the SHG signal of the neat air/water interface can no longer be considered as
valid as before. This new understanding of the air/water interface can shed
light on our understanding of the nonlinear optical responses from other
molecular interfaces as well
On the indistinguishability of Raman photons
We provide a theoretical framework to study the effect of dephasing on the
quantum indistinguishability of single photons emitted from a coherently driven
cavity QED -system. We show that with a large excited-state detuning,
the photon indistinguishability can be drastically improved provided that the
fluctuation rate of the noise source affecting the excited state is fast
compared with the photon emission rate. In some cases a spectral filter is
required to realize this improvement, but the cost in efficiency can be made
small.Comment: 18 pages, 3 figures, final versio
An Empirical Approach to the Bond Additivity Model in Quantitative Interpretation of Sum Frequency Generation Vibrational Spectra
A complete empirical approach from known Raman and IR spectra is used to make
corrections to the bond additivity model for quantitative interpretation of Sum
Frequency generation Vibrational Spectra (SFG-VS) from molecular interfaces.
This empirical correction successfully addresses the failures of the simple
bond additivity model. This empirical approach not only provides new
understandings of the effectiveness and limitations of the bond additivity
model, but also provides a practical roadmap for its application in SFG-VS
studies of molecular interfaces
Oscillating magnetoresistance in diluted magnetic semiconductor barrier structures
Ballistic spin polarized transport through diluted magnetic semiconductor
(DMS) single and double barrier structures is investigated theoretically using
a two-component model. The tunneling magnetoresistance (TMR) of the system
exhibits oscillating behavior when the magnetic field are varied. An
interesting beat pattern in the TMR and spin polarization is found for
different NMS/DMS double barrier structures which arises from an interplay
between the spin-up and spin-down electron channels which are splitted by the
s-d exchange interaction.Comment: 4 pages, 6 figures, submitted to Phys. Rev.
Dynamics of fermions coupling to a U(1) gauge field in the limit
We study in this paper the properties of a gas of fermions coupling to a U(1)
gauge field at wavevectors at dimensions larger than one,
where is a high momentum cutoff and is the fermi wave
vector. In particular, we shall consider the limit where charge
and current fluctuations at wave vectors are forbidden. Within a
bosonization approximation, effective actions describing the low energy physics
of the system are constructed, where we show that the system can be described
as a fermion liquid formed by chargeless quasi-particles which has vanishing
wavefunction overlap with the bare fermions in the system.Comment: 25 page
Coexistence of hexatic and isotropic phases in two-dimensional Yukawa systems
We have performed Brownian dynamics simulations on melting of two-dimensional
colloidal crystal in which particles interact with Yukawa potential. The pair
correlation function and bond-orientational correlation function was calculated
in the Yukawa system. An algebraic decay of the bond orientational correlation
function was observed. By ruling out the coexistence region, only a unstable
hexatic phase was found in the Yukawa systems. But our work shows that the
melting of the Yukawa systems is a two-stage melting not consist with the KTHNY
theory and the isotropic liquid and the hexatic phase coexistence region was
found. Also we have studied point defects in two-dimensional Yukawa systems.Comment: 9 pages, 8 figures. any comments are welcom
The TIANSHAN Radio Experiment for Neutrino Detection
An antenna array devoted to the autonomous radio-detection of high energy
cosmic rays is being deployed on the site of the 21 cm array radio telescope in
XinJiang, China. Thanks in particular to the very good electromagnetic
environment of this remote experimental site, self-triggering on extensive air
showers induced by cosmic rays has been achieved with a small scale prototype
of the foreseen antenna array. We give here a detailed description of the
detector and present the first detection of extensive air showers with this
prototype.Comment: 37 pages, 15 figures. Astroparticle Physics (in press
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