818 research outputs found
A 10B-based neutron detector with stacked Multiwire Proportional Counters and macrostructured cathodes
We present the results of the measurements of the detection efficiency for a
4.7 \r{A} neutron beam incident upon a detector incorporating a stack of up to
five MultiWire Proportional Counters (MWPC) with Boron-coated cathodes. The
cathodes were made of Aluminum and had a surface exhibiting millimeter-deep
V-shaped grooves of 45{\deg}, upon which the thin Boron film was deposited by
DC magnetron sputtering. The incident neutrons interacting with the converter
layer deposited on the sidewalls of the grooves have a higher capture
probability, owing to the larger effective absorption film thickness. This
leads to a higher overall detection efficiency for the grooved cathode when
compared to a cathode with a flat surface. Both the experimental results and
the predictions of the GEANT4 model suggests that a 5-counter detector stack
with coated grooved cathodes has the same efficiency as a 7-counter stack with
flat cathodes. The reduction in the number of counters in the stack without
altering the detection efficiency will prove highly beneficial for large-area
position-sensitive detectors for neutron scattering applications, for which the
cost-effective manufacturing of the detector and associated readout electronics
is an important objective. The proposed detector concept could be a
technological option for one of the new chopper spectrometers and other
instruments planned to be built at the future European Spallation Source in
Sweden. These results with macrostructured cathodes generally apply not just to
MWPCs but to other gaseous detectors as well.Comment: 14 pages, 9 figure
Electronic structure and chemical bonding in Ti4SiC3 investigated by soft x-ray emission spectroscopy and first principle theory
The electronic structure in the new transition metal carbide Ti4SiC3 has been
investigated by bulk-sensitive soft x-ray emission spectroscopy and compared to
the well-studied Ti3SiC2 and TiC systems. The measured high-resolution Ti L, C
K and Si L x-ray emission spectra are discussed with ab initio calculations
based on density-functional theory including core-to-valence dipole matrix
elements. The detailed investigations of the Ti-C and Ti-Si chemical bonds
provide increased understanding of the physical properties of these
nanolaminates. A strongly modified spectral shape is detected for the buried Si
monolayers due to Si 3p hybridization with the Ti 3d orbitals. As a result of
relaxation of the crystal structure and the charge-transfer from Ti (and Si) to
C, the strength of the Ti-C covalent bond is increased. The differences between
the electronic and crystal structures of Ti4SiC3 and Ti3SiC2 are discussed in
relation to the number of Si layers per Ti layer in the two systems and the
corresponding change of materials properties.Comment: 12 pages, 7 figures, 1 tabl
Bonding mechanism in the nitrides Ti2AlN and TiN: an experimental and theoretical investigation
The electronic structure of nanolaminate Ti2AlN and TiN thin films has been
investigated by bulk-sensitive soft x-ray emission spectroscopy. The measured
Ti L, N K, Al L1 and Al L2,3 emission spectra are compared with calculated
spectra using ab initio density-functional theory including dipole transition
matrix elements. Three different types of bond regions are identified; a
relatively weak Ti 3d - Al 3p bonding between -1 and -2 eV below the Fermi
level, and Ti 3d - N 2p and Ti 3d - N 2s bonding which are deeper in energy
observed at -4.8 eV and -15 eV below the Fermi level, respectively. A strongly
modified spectral shape of 3s states of Al L2,3 emission from Ti2AlN in
comparison to pure Al metal is found, which reflects the Ti 3d - Al 3p
hybridization observed in the Al L1 emission. The differences between the
electronic and crystal structures of Ti2AlN and TiN are discussed in relation
to the intercalated Al layers of the former compound and the change of the
materials properties in comparison to the isostructural carbides.Comment: 18 pages, 7 figures;
http://link.aps.org/doi/10.1103/PhysRevB.76.19512
Zero-bias anomalies of point contact resistance due to adiabatic electron renormalization of dynamical defects
We study effect of the adiabatic electron renormalization on the parameters
of the dynamical defects in the ballistic metallic point contact. The upper
energy states of the ``dressed'' defect are shown to give a smaller
contribution to a resistance of the contact than the lower energy ones. This
holds both for the "classical" renormalization related to defect coupling with
average local electron density and for the "mesoscopic" renormalization caused
by the mesoscopic fluctuations of electronic density the dynamical defects are
coupled with. In the case of mesoscopic renormalization one may treat the
dynamical defect as coupled with Friedel oscillations originated by the other
defects, both static and mobile. Such coupling lifts the energy degeneracy of
the states of the dynamical defects giving different mesoscopic contribution to
resistance, and provides a new model for the fluctuator as for the object
originated by the electronic mesoscopic disorder rather than by the structural
one. The correlation between the defect energy and the defect contribution to
the resistance leads to zero-temperature and zero-bias anomalies of the point
contact resistance.
A comparison of these anomalies with those predicted by the Two Channel Kondo
Model (TCKM) is made. It is shown, that although the proposed model is based on
a completely different from TCKM physical background, it leads to a zero-bias
anomalies of the point contact resistance, which are qualitatively similar to
TCKM predictions.Comment: 6 pages, to be published in Phys. Rev.
Electronic structure investigation of Ti3AlC2, Ti3SiC2, and Ti3GeC2 by soft-X-ray emission spectroscopy
The electronic structures of epitaxially grown films of Ti3AlC2, Ti3SiC2 and
Ti3GeC2 have been investigated by bulk-sensitive soft X-ray emission
spectroscopy. The measured high-resolution Ti L, C K, Al L, Si L and Ge M
emission spectra are compared with ab initio density-functional theory
including core-to-valence dipole matrix elements. A qualitative agreement
between experiment and theory is obtained. A weak covalent Ti-Al bond is
manifested by a pronounced shoulder in the Ti L-emission of Ti3AlC2. As Al is
replaced with Si or Ge, the shoulder disappears. For the buried Al and
Si-layers, strongly hybridized spectral shapes are detected in Ti3AlC2 and
Ti3SiC2, respectively. As a result of relaxation of the crystal structure and
the increased charge-transfer from Ti to C, the Ti-C bonding is strengthened.
The differences between the electronic structures are discussed in relation to
the bonding in the nanolaminates and the corresponding change of materials
properties.Comment: 15 pages, 8 figure
Spectroscopic ellipsometry study on the dielectric function of bulk Ti2AlN, Ti2AlC, Nb2AlC, (Ti0.5,Nb0.5)2AlC, and Ti3GeC2 MAX-phases
Molecular Hydrogen and Global Star Formation Relations in Galaxies
(ABRIDGED) We use hydrodynamical simulations of disk galaxies to study
relations between star formation and properties of the molecular interstellar
medium (ISM). We implement a model for the ISM that includes low-temperature
(T<10^4K) cooling, directly ties the star formation rate to the molecular gas
density, and accounts for the destruction of H2 by an interstellar radiation
field from young stars. We demonstrate that the ISM and star formation model
simultaneously produces a spatially-resolved molecular-gas surface density
Schmidt-Kennicutt relation of the form Sigma_SFR \propto Sigma_Hmol^n_mol with
n_mol~1.4 independent of galaxy mass, and a total gas surface density -- star
formation rate relation Sigma_SFR \propto Sigma_gas^n_tot with a power-law
index that steepens from n_tot~2 for large galaxies to n_tot>~4 for small dwarf
galaxies. We show that deviations from the disk-averaged Sigma_SFR \propto
Sigma_gas^1.4 correlation determined by Kennicutt (1998) owe primarily to
spatial trends in the molecular fraction f_H2 and may explain observed
deviations from the global Schmidt-Kennicutt relation.Comment: Version accepted by ApJ, high-res version available at
http://kicp.uchicago.edu/~brant/astro-ph/molecular_ism/rk2007.pd
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