12 research outputs found
Characterizing noise correlation and enhancing coherence via qubit motion
The identification of spacial noise correlation is of critical importance in developing error-corrected quantum devices, but it has barely been studied so far. In this work, we utilize an effective method called qubit motion, to efficiently determine the noise correlations between any pair of qubits in a 7-qubit superconducting quantum system. The noise correlations between the same pairs of qubits are also investigated when the qubits are at distinct operating frequencies. What’s more, in this multi-qubit system with the presence of noise correlations, we demonstrate the enhancing effect of qubit motion on the coherence of logic qubits, and we propose a Motion-CPMG operation sequence to more efficiently protect the logic state from decoherence, which is experimentally demonstrated to extend the coherence time of logic qubits by nearly one order of magnitude
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Mutual modulation between surface chemistry and bulk microstructure within secondary particles of nickel-rich layered oxides.
Surface lattice reconstruction is commonly observed in nickel-rich layered oxide battery cathode materials, causing unsatisfactory high-voltage cycling performance. However, the interplay of the surface chemistry and the bulk microstructure remains largely unexplored due to the intrinsic structural complexity and the lack of integrated diagnostic tools for a thorough investigation at complementary length scales. Herein, by combining nano-resolution X-ray probes in both soft and hard X-ray regimes, we demonstrate correlative surface chemical mapping and bulk microstructure imaging over a single charged LiNi0.8Mn0.1Co0.1O2 (NMC811) secondary particle. We reveal that the sub-particle regions with more micro cracks are associated with more severe surface degradation. A mechanism of mutual modulation between the surface chemistry and the bulk microstructure is formulated based on our experimental observations and finite element modeling. Such a surface-to-bulk reaction coupling effect is fundamentally important for the design of the next generation battery cathode materials
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Mutual modulation between surface chemistry and bulk microstructure within secondary particles of nickel-rich layered oxides.
Surface lattice reconstruction is commonly observed in nickel-rich layered oxide battery cathode materials, causing unsatisfactory high-voltage cycling performance. However, the interplay of the surface chemistry and the bulk microstructure remains largely unexplored due to the intrinsic structural complexity and the lack of integrated diagnostic tools for a thorough investigation at complementary length scales. Herein, by combining nano-resolution X-ray probes in both soft and hard X-ray regimes, we demonstrate correlative surface chemical mapping and bulk microstructure imaging over a single charged LiNi0.8Mn0.1Co0.1O2 (NMC811) secondary particle. We reveal that the sub-particle regions with more micro cracks are associated with more severe surface degradation. A mechanism of mutual modulation between the surface chemistry and the bulk microstructure is formulated based on our experimental observations and finite element modeling. Such a surface-to-bulk reaction coupling effect is fundamentally important for the design of the next generation battery cathode materials