2,213 research outputs found
Coherent Modulation of the YBa2Cu3O6+x Atomic Structure by Displacive Stimulated Ionic Raman Scattering
We discuss the mechanism of coherent phonon generation by Stimulated Ionic
Raman Scattering, a process different from conventional excitation with near
visible optical pulses. Ionic Raman scattering is driven by anharmonic coupling
between a directly excited infrared-active phonon mode and other Raman modes.
We experimentally study the response of YBa2Cu3O6+x to the resonant excitation
of apical oxygen motions at 20 THz by mid-infrared pulses, which has been shown
in the past to enhance the interlayer superconducting coupling. We find
coherent oscillations of four totally symmetric (Ag) Raman modes and make a
critical assessment of the role of these oscillatory motions in the enhancement
of superconductivity.Comment: 12 pages, 4 figure
Evaluation of soil moisture downscaling using a simple thermal-based proxy - the REMEDHUS network (Spain) example
Soil moisture retrieved from satellite microwave remote sensing normally has spatial resolution on the order of tens of kilometers, which are too coarse for many regional hydrological applications such as agriculture monitoring and drought prediction. Therefore, various downscaling methods have been proposed to enhance the spatial resolution of satellite soil moisture products. The aim of this study is to investigate the validity and robustness of the simple vegetation temperature condition index (VTCI) downscaling scheme over a dense soil moisture observational network (REMEDHUS) in Spain. First, the optimized VTCI was determined through sensitivity analyses of VTCI to surface temperature, vegetation index, cloud, topography, and land cover heterogeneity, using data from Moderate Resolution Imaging Spectroradiometer∼(MODIS) and MSG SEVIRI (METEOSAT Second Generation-Spinning Enhanced Visible and Infrared Imager). Then the downscaling scheme was applied to improve the spatial resolution of the European Space Agency's Water Cycle Multi-mission Observation Strategy and Climate Change Initiative (ESA CCI) soil moisture, which is a merged product based on both active and passive microwave observations. The results from direct validation against soil moisture observations, spatial pattern comparison, as well as seasonal and land use analyses show that the downscaling method can significantly improve the spatial details of CCI soil moisture while maintaining the accuracy of CCI soil moisture. The accuracy level is comparable to other downscaling methods that were also validated against the REMEDHUS network. Furthermore, slightly better performance of MSG SEVIRI over MODIS was observed, which suggests the high potential of applying a geostationary satellite for downscaling soil moisture in the future. Overall, considering the simplicity, limited data requirements and comparable accuracy level to other complex methods, the VTCI downscaling method can facilitate relevant hydrological applications that require high spatial and temporal resolution soil moisture. © 2015 Author(s)
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Do we (need to) care about canopy radiation schemes in DGVMs? Caveats and potential impacts
Dynamic global vegetation models (DGVMs) are an essential part of current state-of-the-art Earth system models. In recent years, the complexity of DGVMs has increased by incorporating new important processes like, e.g., nutrient cycling and land cover dynamics, while biogeophysical processes like surface radiation have not been developed much further. Canopy radiation models are however very important for the estimation of absorption and reflected fluxes and are essential for a proper estimation of surface carbon, energy and water fluxes.
The present study provides an overview of current implementations of canopy radiation schemes in a couple of state-of-the-art DGVMs and assesses their accuracy in simulating canopy absorption and reflection for a variety of different surface conditions. Systematic deviations in surface albedo and fractions of absorbed photosynthetic active radiation (faPAR) are identified and potential impacts are assessed.
The results show clear deviations for both, absorbed and reflected, surface solar radiation fluxes. FaPAR is typically underestimated, which results in an underestimation of gross primary productivity (GPP) for the investigated cases. The deviation can be as large as 25% in extreme cases. Deviations in surface albedo range between −0.15 ≤ Δα ≤ 0.36, with a slight positive bias on the order of Δα ≈ 0.04. Potential radiative forcing caused by albedo deviations is estimated at −1.25 ≤ RF ≤ −0.8 (W m−2), caused by neglect of the diurnal cycle of surface albedo.
The present study is the first one that provides an assessment of canopy RT schemes in different currently used DGVMs together with an assessment of the potential impact of the identified deviations. The paper illustrates that there is a general need to improve the canopy radiation schemes in DGVMs and provides different perspectives for their improvement
Pump frequency resonances for light-induced incipient superconductivity in YBaCuO
Optical excitation in the cuprates has been shown to induce transient
superconducting correlations above the thermodynamic transition temperature,
, as evidenced by the terahertz frequency optical properties in the
non-equilibrium state. In YBaCuO this phenomenon has so far
been associated with the nonlinear excitation of certain lattice modes and the
creation of new crystal structures. In other compounds, like
LaBaCuO, similar effects were reported also for excitation at
near infrared frequencies, and were interpreted as a signature of the melting
of competing orders. However, to date it has not been possible to
systematically tune the pump frequency widely in any one compound, to
comprehensively compare the frequency dependent photo-susceptibility for this
phenomenon. Here, we make use of a newly developed optical parametric
amplifier, which generates widely tunable high intensity femtosecond pulses, to
excite YBaCuO throughout the entire optical spectrum (3 - 750
THz). In the far-infrared region (3 - 25 THz), signatures of non-equilibrium
superconductivity are induced only for excitation of the 16.4 THz and 19.2 THz
vibrational modes that drive -axis apical oxygen atomic positions. For
higher driving frequencies (25 - 750 THz), a second resonance is observed
around the charge transfer band edge at ~350 THz. These observations highlight
the importance of coupling to the electronic structure of the CuO planes,
either mediated by a phonon or by charge transfer.Comment: 47 pages, 21 figures, 2 table
Influence of Monolayer-Monolayer Coupling on the Phase Behavior of a Fluid Lipid Bilayer
AbstractWe suggest a minimal model for the coupling of the lateral phase behavior in an asymmetric lipid membrane across its two monolayers. Our model employs one single order parameter for each monolayer leaflet, namely its composition. Regular solution theory on the mean-field level is used to describe the free energy in each individual leaflet. Coupling between monolayers entails an energy penalty for any local compositional differences across the membrane. We calculate and analyze the phase behavior of this model. It predicts a range of possible scenarios. A monolayer with a propensity for phase separation is able to induce phase separation in the apposed monolayer. Conversely, a monolayer without this propensity is able to prevent phase separation in the apposed monolayer. If there is phase separation in the membrane, it may lead to either complete or partial registration of the monolayer domains across the membrane. The latter case which corresponds to a three-phase coexistence is only found below a critical coupling strength. We calculate that critical coupling strength. Above the critical coupling strength, the membrane adopts a uniform compositional difference between its two monolayers everywhere in the membrane, implying phase coexistence between only two phases and thus perfect spatial registration of all domains on the apposed membrane leafs. We use the lattice Boltzmann simulation method to also study the morphologies that form during phase separation within the three-phase coexistence region. Generally, domains in one monolayer diffuse but remain fully enclosed within domains in the other monolayer
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