1,132 research outputs found
Spin fluctuations with two-dimensional XY behavior in a frustrated S = 1/2 square-lattice ferromagnet
The spin dynamics of the layered square-lattice vanadate Pb2VO(PO4)2 is
investigated by electron spin resonance at various magnetic fields and at
temperatures above magnetic ordering. The linewidth divergence towards low
temperatures seems to agree with isotropic Heisenberg-type spin exchange
suggesting that the spin relaxation in this quasi-two dimensional compound is
governed by low-dimensional quantum fluctuations. However, a weak easy- plane
anisotropy of the g factor points to the presence of a planar XY type of
exchange. Indeed, we found that the linewidth divergence is described best by
XY-like spin fluctuations which requires a single parameter only. Therefore,
ESR-probed spin dynamics could establish Pb2VO(PO4)2 as the first frustrated
square lattice system with XY-inherent spin topological fluctuations.Comment: 5 pages, 3 figure
Anisotropic ferromagnetism in carbon doped zinc oxide from first-principles studies
A density functional theory study of substitutional carbon impurities in ZnO
has been performed, using both the generalized gradient approximation (GGA) and
a hybrid functional (HSE06) as exchange-correlation functional. It is found
that the non-spinpolarized C impurity is under almost all
conditions thermodynamically more stable than the C impurity which
has a magnetic moment of , with the exception of very O-poor
and C-rich conditions. This explains the experimental difficulties in sample
preparation in order to realize -ferromagnetism in C-doped ZnO. From GGA
calculations with large 96-atom supercells, we conclude that two
C-C impurities in ZnO interact ferromagnetically, but
the interaction is found to be short-ranged and anisotropic, much stronger
within the hexagonal -plane of wurtzite ZnO than along the c-axis. This
layered ferromagnetism is attributed to the anisotropy of the dispersion of
carbon impurity bands near the Fermi level for C impurities in
ZnO. From the calculated results, we derive that a C
concentration between 2% and 6% should be optimal to achieve
-ferromagnetism in C-doped ZnO.Comment: 9 pages, 7 figure
Topographical characterization and microstructural interface analysis of vacuum-plasma-sprayed titanium and hydroxyapatite coatings on carbon fibre-reinforced poly(etheretherketone)
In the present study, topographical characterization and microstructural interface analysis of vacuum-plasma-sprayed titanium and hydroxyapatite (HA) coatings on carbon fibre-reinforced polyetheretherketone (CF/PEEK) was performed. VPS-Ti coatings with high roughness values (Ra=28.29±3.07 μm, Rz=145.35±9.88 μm) were obtained. On this titanium, intermediate layer HA coatings of various thicknesses were produced. With increasing coating thickness, roughness values of the HA coatings decreased. A high increase of profile length ratio, Lr, of the VPS-Ti coatings (Lr=1.45) compared to the grit-blasted CF/PEEK substrate (Lr=1.08) was observed. Increasing the HA coating thickness resulted in a reduction of the Lr values similar to the roughness values. Fractal analysis of the obtained roughness profiles revealed that the VPS-Ti coatings showed the highest fractal dimension of D=1.34±0.02. Fractal dimension dropped to a value of 1.23-1.25 for all HA coatings. No physical deterioration of the CF/PEEK substrate was observed, indicating that substrate drying and the used VPS process parameter led to the desired coatings on the composite material. Cross-section analysis revealed a good interlocking between the titanium intermediate layer and the PEEK substrate. It is therefore assumed that this interlocking results in suitable mechanical adhesive strength. From the results obtained in this study it is concluded that VPS is a suitable method for manufacturing HA coatings on carbon fibre-reinforced PEEK implant material
Pressure Induced Topological Phase Transitions in Membranes
Some highly unusual features of a lipid-water liquid crystal are revealed by
high pressure x-ray diffraction, light scattering and dilatometric studies of
the lamellar (bilayer ) to nonlamellar inverse hexagonal ()
phase transition. (i) The size of the unit cell of the phase increases
with increasing pressure. (ii) The transition volume, ,
decreases and appears to vanish as the pressure is increased. (iii) The
intensity of scattered light increases as decreases. Data are
presented which suggest that this increase is due to the formation of an
intermediate cubic phase, as predicted by recent theoretical suggestions of the
underlying universal phase sequence.Comment: 12 pages, typed using REVTEX 2.
Striped instability of a holographic Fermi-like liquid
We consider a holographic description of a system of strongly-coupled
fermions in 2+1 dimensions based on a D7-brane probe in the background of
D3-branes. The black hole embedding represents a Fermi-like liquid. We study
the excitations of the Fermi liquid system. Above a critical density which
depends on the temperature, the system becomes unstable towards an
inhomogeneous modulated phase which is similar to a charge density and spin
wave state. The essence of this instability can be effectively described by a
Maxwell-axion theory with a background electric field. We also consider the
fate of zero sound at non-zero temperature.Comment: 16 pages, 9 figures; v2: added discussion and one figure. Typos
correcte
Instability of the rhodium magnetic moment as origin of the metamagnetic phase transition in alpha-FeRh
Based on ab initio total energy calculations we show that two magnetic states
of rhodium atoms together with competing ferromagnetic and antiferromagnetic
exchange interactions are responsible for a temperature induced metamagnetic
phase transition, which experimentally is observed for stoichiometric
alpha-FeRh. A first-principle spin-based model allows to reproduce this
first-order metamagnetic transition by means of Monte Carlo simulations.
Further inclusion of spacial variation of exchange parameters leads to a
realistic description of the experimental magneto-volume effects in alpha-FeRh.Comment: 10 pages, 13 figures, accepted for publication in Phys. Rev.
Field-induced metal-insulator transition and switching phenomenon in correlated insulators
We study the nonequilibrium switching phenomenon associated with the
metal-insulator transition under electric field E in correlated insulator by a
gauge-covariant Keldysh formalism. Due to the feedback effect of the resistive
current I, this occurs as a first-order transition with a hysteresis of I-V
characteristics having a lower threshold electric field (\sim 10^4 Vcm^{-1})
much weaker than that for the Zener breakdown. It is also found that the
localized mid-gap states introduced by impurities and defects act as hot spots
across which the resonant tunneling occurs selectively, which leads to the
conductive filamentary paths and reduces the energy cost of the switching
function.Comment: 5 pages, 3 figures. A study on the metal-insulator transition in
correlated insulators was adde
Magnetic properties of small Pt-capped Fe, Co and Ni clusters: A density functional theory study
Theoretical studies on M (M = Fe, Co, Ni) and MPt (for
= 3, 4, 5, 20) clusters including the spin-orbit coupling are done using
density functional theory. The magnetic anisotropy energy (MAE) along with the
spin and orbital moments are calculated for M icosahedral clusters. The
angle-dependent energy differences are modelled using an extended classical
Heisenberg model with local anisotropies. From our studies, the MAE for
Jahn-Teller distorted Fe, Mackay distorted Fe and nearly
undistorted Co clusters are found to be 322, 60 and 5 eV/atom,
respectively, and are large relative to the corresponding bulk values, (which
are 1.4 and 1.3 eV/atom for bcc Fe and fcc Co, respectively.) However, for
Ni (which practically does not show relaxation tendencies), the
calculated value of MAE is found to be 0.64 eV/atom, which is
approximately four times smaller compared to the bulk fcc Ni (2.7
eV/atom). In addition, MAE of the capped cluster (FePt) is
enhanced compared to the uncapped Jahn-Teller distorted Fe cluster
Three-dimensional quantization of the electromagnetic field in dispersive and absorbing inhomogeneous dielectrics
A quantization scheme for the phenomenological Maxwell theory of the full
electromagnetic field in an inhomogeneous three-dimensional, dispersive and
absorbing dielectric medium is developed. The classical Maxwell equations with
spatially varying and Kramers-Kronig consistent permittivity are regarded as
operator-valued field equations, introducing additional current- and
charge-density operator fields in order to take into account the noise
associated with the dissipation in the medium. It is shown that the equal-time
commutation relations between the fundamental electromagnetic fields
and and the potentials and in the Coulomb gauge
can be expressed in terms of the Green tensor of the classical problem. From
the Green tensors for bulk material and an inhomogeneous medium consisting of
two bulk dielectrics with a common planar interface it is explicitly proven
that the well-known equal-time commutation relations of QED are preserved
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