1,006 research outputs found
Field-Induced Magnetic and Structural Domain Alignment in PrO2
We present a neutron diffraction study of the magnetic structure of single
crystal PrO2 under applied fields of 0-6 T. As the field is increased, changes
are observed in the magnetic Bragg intensities. These changes are found to be
irreversible when the field is reduced, but the original intensities can be
recovered by heating to T > 122 K, then re-cooling in zero field. The
antiferromagnetic ordering temperature TN = 13.5 K and the magnetic periodicity
are unaffected by the applied field. We also report measurements of the
magnetic susceptibility of single crystal PrO2 under applied fields of 0-7 T.
These show strong anisotropy, as well as an anomaly at T = 122 +/- 2 K which
coincides with the temperature TD = 120 +/- 2 K at which a structural
distortion occurs. For fields applied along the [100] direction the
susceptibility increases irreversibly with field in the temperature range TN <
T < TD. However, for fields along [110] the susceptibility is independent of
field in this range. We propose structural domain alignment, which strongly
influences the formation of magnetic domains below TN, as the mechanism behind
these changes.Comment: 11 pages, 13 figures, 5 tables. Minor typographical changes in v
Cooperative Jahn-Teller Distortion in PrO2
We report neutron diffraction data on single crystal PrO2 which reveal a
cooperative Jahn-Teller distortion at TD = 120 +/- 2 K. Below this temperature
an internal distortion of the oxygen sublattice causes the unit cell of the
crystallographic structure to become doubled along one crystal axis. We discuss
several possible models for this structure. The antiferromagnetic structure
below TN = 13.5 K is found to consist of two components, one of which shares
the same doubled unit cell as the distorted crystallographic structure. We also
present measurements of the magnetic susceptibility, the specific heat capacity
and the electrical conductivity of PrO2. The susceptibility data show an
anomaly at a temperature close to TD. From the specific heat capacity data we
deduce that the ground state is doubly degenerate, consistent with a distortion
of the cubic local symmetry. We discuss possible mechanisms for this. The
conductivity shows an activated behaviour with an activation energy Ea = 0.262
+/- 0.003 eV.Comment: 12 pages, 14 figures, 2 tables. Additional suggested structure in v
Phonon Dispersion Relations in PrBa2Cu3O6+x (x ~ 0.2)
We report measurements of the phonon dispersion relations in
non-superconducting, oxygen-deficient PrBa2Cu3O6+x (x ~ 0.2) by inelastic
neutron scattering. The data are compared with a model of the lattice dynamics
based on a common interaction potential. Good agreement is achieved for all but
two phonon branches, which are significantly softer than predicted. These modes
are found to arise predominantly from motion of the oxygen ions in the CuO2
planes. Analogous modes in YBa2Cu3O6 are well described by the common
interaction potential model.Comment: 4 pages, 3 figures. Minor changes following referees' comment
Spin resonance in the superconducting state of LiFeODFeSe observed by neutron spectroscopy
We have performed inelastic neutron scattering measurements on a powder
sample of the superconductor lithium iron selenide hydroxide
LiFeODFeSe (, \,K). The spectrum shows an enhanced intensity below over an
energy range , where is the
superconducting gap, with maxima at the wave vectors \,\AA and \,\AA. The behavior of this
feature is consistent with the spin resonance mode found in other
unconventional superconductors, and strongly resembles the spin resonance
observed in the spectrum of the molecular-intercalated iron selenide,
Li(ND)(ND)FeSe. The signal can
be described with a characteristic two-dimensional wave vector
in the Brillouin zone of the iron square lattice, consistent with the nesting
vector between electron Fermi sheets
Influence of static Jahn-Teller distortion on the magnetic excitation spectrum of PrO2: A synchrotron x-ray and neutron inelastic scattering study
A synchrotron x-ray diffraction study of the crystallographic structure of
PrO2 in the Jahn-Teller distorted phase is reported. The distortion of the
oxygen sublattice, which was previously ambiguous, is shown to be a chiral
structure in which neighbouring oxygen chains have opposite chiralities. A
temperature dependent study of the magnetic excitation spectrum, probed by
neutron inelastic scattering, is also reported. Changes in the energies and
relative intensities of the crystal field transitions provide an insight into
the interplay between the static and dynamic Jahn-Teller effects.Comment: 7 pages, 6 figure
Magnetic impurity coupled to interacting conduction electrons
We consider a magnetic impurity which interacts by hybridization with a
system of weakly correlated electrons and determine the energy of the ground
state by means of an 1/N_f expansion. The correlations among the conduction
electrons are described by a Hubbard Hamiltonian and are treated to lowest
order in the interaction strength. We find that their effect on the Kondo
temperature, T_K, in the Kondo limit is twofold: First, the position of the
impurity level is shifted due to the reduction of charge fluctuations, which
reduces T_K. Secondly, the bare Kondo exchange coupling is enhanced as spin
fluctuations are enlarged. In total, T_K increases. Both corrections require
intermediate states beyond the standard Varma-Yafet ansatz. This shows that the
Hubbard interaction does not just provide quasiparticles, which hybridize with
the impurity, but also renormalizes the Kondo coupling.Comment: ReVTeX 19 pages, 3 uuenconded postscript figure
Rights Myopia in Child Welfare
For decades, legal scholars have debated the proper balance of parents\u27 rights and children\u27s rights in the child welfare system. This Article argues that the debate mistakenly privileges rights. Neither parents\u27 rights nor children\u27s rights serve families well because, as implemented, a solely rights-based model of child welfare does not protect the interests of parents or children. Additionally, even if well-implemented, the model still would not serve parents or children because it obscures the important role of poverty in child abuse and neglect and fosters conflict rather than collaboration between the state and families. In lieu of a solely rights-based model, this Article proposes a problem-solving model for child welfare and explores one embodiment of such a model, family group conferencing. This Article concludes that a problem-solving model holds significant potential to address many of the profound theoretical and practical shortcomings of the current child welfare system
The importance of XY anisotropy in Sr2IrO4 revealed by magnetic critical scattering experiments
The magnetic critical scattering in SrIrO has been characterized
using X-ray resonant magnetic scattering (XRMS) both below and above the 3D
antiferromagnetic ordering temperature, T. The order parameter
critical exponent below T is found to be \beta=0.195(4), in the
range of the 2D XYh universality class. Over an extended temperature range
above T, the amplitude and correlation length of the intrinsic
critical fluctuations are well described by the 2D Heisenberg model with XY
anisotropy. This contrasts with an earlier study of the critical scattering
over a more limited range of temperature which found agreement with the theory
of the isotropic 2D Heisenberg quantum antiferromagnet, developed to describe
the critical fluctuations of the conventional Mott insulator LaCuO and
related systems. Our study therefore establishes the importance of XY
anisotropy in the low-energy effective Hamiltonian of SrIrO, the
prototypical spin-orbit Mott insulator.Comment: 6 pages, 4 figure
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