2,672 research outputs found
Isotope effect in quasi-two-dimensional metal-organic antiferromagnets
Although the isotope effect in superconducting materials is well-documented,
changes in the magnetic properties of antiferromagnets due to isotopic
substitution are seldom discussed and remain poorly understood. This is perhaps
surprising given the possible link between the quasi-two-dimensional (Q2D)
antiferromagnetic and superconducting phases of the layered cuprates. Here we
report the experimental observation of shifts in the N\'{e}el temperature and
critical magnetic fields (; ) in a Q2D organic molecular antiferromagnets on
substitution of hydrogen for deuterium. These compounds are characterized by
strong hydrogen bonds through which the dominant superexchange is mediated. We
evaluate how the in-plane and inter-plane exchange energies evolve as the
hydrogens on different ligands are substituted, and suggest a possible
mechanism for this effect in terms of the relative exchange efficiency of
hydrogen and deuterium bonds
Photon Echoes Produced by Switching Electric Fields
We demonstrate photon echoes in Eu:YSiO by controlling the
inhomogeneous broadening of the Eu
FD optical transition. This transition has
a linear Stark shift and we induce inhomogeneous broadening by applying an
external electric field gradient. After optical excitation, reversing the
polarity of the field rephases the ensemble, resulting in a photon echo. This
is the first demonstration of such a photon echo and its application as a
quantum memory is discussed.Comment: improved introduction, including theoretical outline of the relvant
quantum memory proposa
Magnetic order in the quasi-one-dimensional spin 1/2 chain, copper pyrazine dinitrate
We present the first evidence of magnetic order in the quasi-one-dimensional
spin 1/2 molecular chain compound, copper pyrazine dinitrate Cu(C4H4N2)(NO3)2}.
Zero field muon-spin relaxation measurements made at dilution refrigerator
temperatures show oscillations in the measured asymmetry, characteristic of a
quasistatic magnetic field at the muon sites. Our measurements provide
convincing evidence for long range magnetic order below a temperature
T_N=107(1) mK. This leads to an estimate of the interchain coupling constant of
|J'|/k_B=0.046 K and to a ratio |J'/J| = 4.4 x 10^-3.Comment: 4 pages, 3 figures. Submitted to Physical Review Letter
Barriers and facilitators to palliative care education in nursing and residential homes: a rapid review
Background:
There is insufficient high-quality evidence to suggest that palliative care education can impact care home settings.
Aims:
To identify, appraise and synthesise all available evidence on the barriers and facilitators to providing palliative care education in residential and nursing care homes and to generate recommendations to increase the effectiveness of future palliative care education programmes in care homes.
Methods:
A rapid review searching CINAHL, Medline and ProQuest. One author screened full-text articles for inclusion. Any uncertainties were discussed with a second author.
Findings:
Twenty-two articles were included in the full review. Analysis of the included articles revealed the following overlapping themes: structural systems; cultural and personal issues; and knowledge translation issues with interaction.
Conclusion:
Addressing the barriers and facilitators when designing palliative care education programmes for care homes will lead to more successful outcomes
Muon-fluorine entangled states in molecular magnets
The information accessible from a muon-spin relaxation experiment is often
limited since we lack knowledge of the precise muon stopping site. We
demonstrate here the possibility of localizing a spin polarized muon in a known
stopping state in a molecular material containing fluorine. The muon-spin
precession that results from the entangled nature of the muon-spin and
surrounding nuclear spins is sensitive to the nature of the stopping site and
we use this property to identify three classes of site. We are also able to
describe the extent to which the muon distorts its surroundings.Comment: 4 pages, 3 figure
Method of extending hyperfine coherence times in Pr^3+:Y_2SiO_5
In this letter we present a method for increasing the coherence time of
praseodymium hyperfine ground state transitions in Pr^3+:Y_2SiO_5 by the
application of a specific external magnetic field. The magnitude and angle of
the external field is applied such that the Zeeman splitting of a hyperfine
transition is at a critical point in three dimensions, making the first order
Zeeman shift vanishingly small for the transition. This reduces the influence
of the magnetic interactions between the praseodymium ions and the spins in the
host lattice on the transition frequency. Using this method a phase memory time
of 82ms was observed, a value two orders of magnitude greater than previously
reported. It is shown that the residual dephasing is amenable quantum error
correction
Empirical wind model for the middle and lower atmosphere. Part 1: Local time average
The HWM90 thermospheric wind model was revised in the lower thermosphere and extended into the mesosphere and lower atmosphere to provide a single analytic model for calculating zonal and meridional wind profiles representative of the climatological average for various geophysical conditions. Gradient winds from CIRA-86 plus rocket soundings, incoherent scatter radar, MF radar, and meteor radar provide the data base and are supplemented by previous data driven model summaries. Low-order spherical harmonics and Fourier series are used to describe the major variations throughout the atmosphere including latitude, annual, semiannual, and longitude (stationary wave 1). The model represents a smoothed compromise between the data sources. Although agreement between various data sources is generally good, some systematic differences are noted, particularly near the mesopause. Root mean square differences between data and model are on the order of 15 m/s in the mesosphere and 10 m/s in the stratosphere for zonal wind, and 10 m/s and 4 m/s, respectively, for meridional wind
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Relationship between adiposity and admixture in African-American and Hispanic-American women.
ObjectiveThe objective of this study was to investigate whether differences in admixture in African-American (AFA) and Hispanic-American (HA) adult women are associated with adiposity and adipose distribution.DesignThe proportion of European, sub-Saharan African and Amerindian admixture was estimated for AFA and HA women in the Women's Heath Initiative using 92 ancestry informative markers. Analyses assessed the relationship between admixture and adiposity indices.SubjectsThe subjects included 11 712 AFA and 5088 HA self-identified post-menopausal women.ResultsThere was a significant positive association between body mass index (BMI) and African admixture when BMI was considered as a continuous variable, and age, education, physical activity, parity, family income and smoking were included covariates (P<10(-4)). A dichotomous model (upper and lower BMI quartiles) showed that African admixture was associated with a high odds ratio (OR=3.27 (for 100% admixture compared with 0% admixture), 95% confidence interval 2.08-5.15). For HA, there was no association between BMI and admixture. In contrast, when waist-to-hip ratio (WHR) was used as a measure of adipose distribution, there was no significant association between WHR and admixture in AFA but there was a strong association in HA (P<10(-4); OR Amerindian admixture=5.93, confidence interval=3.52-9.97).ConclusionThese studies show that: (1) African admixture is associated with BMI in AFA women; (2) Amerindian admixture is associated with WHR but not BMI in HA women; and (3) it may be important to consider different measurements of adiposity and adipose distribution in different ethnic population groups
Magnetic properties of the quasi-two-dimensional S = 1/2 Heisenberg antiferromagnet [Cu(pyz)2(HF2)]PF6
We report on high-field magnetization, specific-heat and electron spin
resonance (ESR) studies of the quasi-two-dimensional spin-1/2 Heisenberg
antiferromagnet [Cu(pyz)2(HF2)]PF6. The frequency-field diagram of ESR modes
below TN = 4.38 K is described in the frame of the meanfield theory, confirming
a collinear magnetic structure with an easy-plane anisotropy. The obtained
results allowed us to determine the anisotropy/exchange interaction ratio, A/J
= 0.003, and the upper limit for the inter/intra-plane exchange-interaction
ratio, J'/J = 1/16. It is argued that despite the onset of 3D long-range
magnetic ordering the magnetic properties of this material (including
high-magnetic-field magnetization and non-monotonic field dependence of the
Neel temperature) are strongly affected by two-dimensional spin correlations.Comment: 5 pages, 7 figure
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