We present the first evidence of magnetic order in the quasi-one-dimensional
spin 1/2 molecular chain compound, copper pyrazine dinitrate Cu(C4H4N2)(NO3)2}.
Zero field muon-spin relaxation measurements made at dilution refrigerator
temperatures show oscillations in the measured asymmetry, characteristic of a
quasistatic magnetic field at the muon sites. Our measurements provide
convincing evidence for long range magnetic order below a temperature
T_N=107(1) mK. This leads to an estimate of the interchain coupling constant of
|J'|/k_B=0.046 K and to a ratio |J'/J| = 4.4 x 10^-3.Comment: 4 pages, 3 figures. Submitted to Physical Review Letter