Semiclassical two-step model for ionization of hydrogen molecule by strong laser field

We extend the semiclassical two-step model for strong-field ionization that describes quantum interference and accounts for the Coulomb potential beyond the semiclassical perturbation theory to the hydrogen molecule. In the simplest case of the molecule oriented along the polarization direction of a linearly polarized laser field, we predict significant deviations of the two-dimensional photoelectron momentum distributions and the energy spectra from the case of atomic hydrogen. Specifically, for the hydrogen molecule the electron energy spectrum falls off slower with increasing energy, and the holographic interference fringes are more pronounced than for the hydrogen atom at the same parameters of the laser pulse.Comment: 9 pages, 6 figure

Semiclassical two-step model for strong-field ionization

We present a semiclassical two-step model for strong-field ionization that accounts for path interferences of tunnel-ionized electrons in the ionic potential beyond perturbation theory. Within the framework of a classical trajectory Monte-Carlo representation of the phase-space dynamics, the model employs the semiclassical approximation to the phase of the full quantum propagator in the exit channel. By comparison with the exact numerical solution of the time-dependent Schr\"odinger equation for strong-field ionization of hydrogen, we show that for suitable choices of the momentum distribution after the first tunneling step, the model yields good quantitative agreement with the full quantum simulation. The two-dimensional photoelectron momentum distributions, the energy spectra, and the angular distributions are found to be in good agreement with the corresponding quantum results. Specifically, the model quantitatively reproduces the fan-like interference patterns in the low-energy part of the two-dimensional momentum distributions as well as the modulations in the photoelectron angular distributions.Comment: 31 pages, 7 figure

Capture into Rydberg states and momentum distributions of ionized electrons

The yield of neutral excited atoms and low-energy photoelectrons generated by the electron dynamics in the combined Coulomb and laser field after tunneling is investigated. We present results of Monte-Carlo simulations built on the two-step semiclassical model, as well as analytic estimates and scaling relations for the population trapping into the Rydberg states. It is shown that mainly those electrons are captured into bound states of the neutral atom that due to their initial conditions (i) have moderate drift momentum imparted by the laser field and (ii) avoid strong interaction ("hard" collision) with the ion. In addition, it is demonstrated that the channel of capture, when accounted for in semiclassical calculations, has a pronounced effect on the momentum distribution of electrons with small positive energy. For the parameters that we investigated its presence leads to a dip at zero momentum in the longitudinal momentum distribution of the ionized electrons.Comment: 9 pages, 8 figures in one zip-archiv

Steady state solutions of hydrodynamic traffic models

We investigate steady state solutions of hydrodynamic traffic models in the absence of any intrinsic inhomogeneity on roads such as on-ramps. It is shown that typical hydrodynamic models possess seven different types of inhomogeneous steady state solutions. The seven solutions include those that have been reported previously only for microscopic models. The characteristic properties of wide jam such as moving velocity of its spatiotemporal pattern and/or out-flux from wide jam are shown to be uniquely determined and thus independent of initial conditions of dynamic evolution. Topological considerations suggest that all of the solutions should be common to a wide class of traffic models. The results are discussed in connection with the universality conjecture for traffic models. Also the prevalence of the limit-cycle solution in a recent study of a microscopic model is explained in this approach.Comment: 9 pages, 6 figure

Reconstruction of a single-active-electron potential from electron momentum distribution produced by strong-field ionization using optimization technique

We present a method for retrieving of single-active electron potential in an atom or molecule from a given momentum distribution of photoelectrons ionized by a strong laser field. In this method the potential varying within certain limits is found as the result of the optimization procedure aimed at reproducing the given momentum distribution. The optimization using numerical solution of the time-dependent Schrodinger equation for ionization of a model one-dimensional atom shows the good accuracy of the potential reconstruction method. This applies to different ways used for representing of the potential under reconstruction, including a parametrization and determination of the potential by specifying its values on a spatial grid.Comment: 18 pages, 6 figure

Long-lived states in synchronized traffic flow. Empirical prompt and dynamical trap model

The present paper proposes a novel interpretation of the widely scattered states (called synchronized traffic) stimulated by Kerner's hypotheses about the existence of a multitude of metastable states in the fundamental diagram. Using single vehicle data collected at the German highway A1, temporal velocity patterns have been analyzed to show a collection of certain fragments with approximately constant velocities and sharp jumps between them. The particular velocity values in these fragments vary in a wide range. In contrast, the flow rate is more or less constant because its fluctuations are mainly due to the discreteness of traffic flow. Subsequently, we develop a model for synchronized traffic that can explain these characteristics. Following previous work (I.A.Lubashevsky, R.Mahnke, Phys. Rev. E v. 62, p. 6082, 2000) the vehicle flow is specified by car density, mean velocity, and additional order parameters $h$ and $a$ that are due to the many-particle effects of the vehicle interaction. The parameter $h$ describes the multilane correlations in the vehicle motion. Together with the car density it determines directly the mean velocity. The parameter $a$, in contrast, controls the evolution of $h$ only. The model assumes that $a$ fluctuates randomly around the value corresponding to the car configuration optimal for lane changing. When it deviates from this value the lane change is depressed for all cars forming a local cluster. Since exactly the overtaking manoeuvres of these cars cause the order parameter $a$ to vary, the evolution of the car arrangement becomes frozen for a certain time. In other words, the evolution equations form certain dynamical traps responsible for the long-time correlations in the synchronized mode.Comment: 16 pages, 10 figures, RevTeX

Macroscopic Dynamics of Multi-Lane Traffic

We present a macroscopic model of mixed multi-lane freeway traffic that can be easily calibrated to empirical traffic data, as is shown for Dutch highway data. The model is derived from a gas-kinetic level of description, including effects of vehicular space requirements and velocity correlations between successive vehicles. We also give a derivation of the lane-changing rates. The resulting dynamic velocity equations contain non-local and anisotropic interaction terms which allow a robust and efficient numerical simulation of multi-lane traffic. As demonstrated by various examples, this facilitates the investigation of synchronization patterns among lanes and effects of on-ramps, off-ramps, lane closures, or accidents.Comment: For related work see http://www.theo2.physik.uni-stuttgart.de/helbing.htm

Interpreting Attoclock Measurements of Tunnelling Times

Resolving in time the dynamics of light absorption by atoms and molecules, and the electronic rearrangement this induces, is among the most challenging goals of attosecond spectroscopy. The attoclock is an elegant approach to this problem, which encodes ionization times in the strong-field regime. However, the accurate reconstruction of these times from experimental data presents a formidable theoretical challenge. Here, we solve this problem by combining analytical theory with ab-initio numerical simulations. We apply our theory to numerical attoclock experiments on the hydrogen atom to extract ionization time delays and analyse their nature. Strong field ionization is often viewed as optical tunnelling through the barrier created by the field and the core potential. We show that, in the hydrogen atom, optical tunnelling is instantaneous. By calibrating the attoclock using the hydrogen atom, our method opens the way to identify possible delays associated with multielectron dynamics during strong-field ionization.Comment: 33 pages, 10 figures, 3 appendixe

Transfer learning, alternative approaches, and visualization of a convolutional neural network for retrieval of the internuclear distance in a molecule from photoelectron momentum distributions

We investigate the application of deep learning to the retrieval of the internuclear distance in the two-dimensional H$_2^{+}$ molecule from the momentum distribution of photoelectrons produced by strong-field ionization. We study the effect of the carrier-envelope phase on the prediction of the internuclear distance with a convolutional neural network. We apply the transfer learning technique to make our convolutional neural network applicable to distributions obtained for parameters outside the ranges of the training data. The convolutional neural network is compared with alternative approaches to this problem, including the direct comparison of momentum distributions, support-vector machines, and decision trees. These alternative methods are found to possess very limited transferability. Finally, we use the occlusion-sensitivity technique to extract the features that allow a neural network to take its decisions.Comment: 28 pages, 7 figures, 1 tabl