Experiments for electromagnetic levitation in microgravity

Containerless processing is a promising research tool for investigating the properties of undercooled melts and their solidification. For conducting samples RF-electromagnetic levitation offers the possibility to obtain large undercoolings by avoiding heterogeneous nucleation at container walls. On earth, however, strong magnetic fields are needed to compensate the gravitational force which imposes a lower limit on the available temperatures and on the accessible undercooling range. Under microgravity conditions the magnetic positioning fields can be minimized and hence, undercooling becomes feasible under ultra-high vacuum conditions and lower temperatures become accessible. In contrast to other undercooling and solidification techniques, electromagnetic levitation allows for diagnostic measurements during the early steps of nucleation and phase selection. Experiments cover a wide field of research topics: nucleation, directional solidification at high velocities, generation of metastable phases, evolution of microstructures, properties of undercooled liquids. Examples from these classes including experiments selected for the IML-2 mission are discussed with emphasis on technical requirements. An overview is given on the German TEMPUS (electromagnetic levitation facility) program

On the Shape of Liquid Metal Droplets in Electromagnetic Levitation Experiments

We present calculations and measurements on the shape of liquid metal droplets in electromagnetic levitation experiments. A normal stress balance model was developed to predict the shapes of liquid metal droplets that will be obtained in a microgravity experiment to measure the viscosity and surface tension of undercooled metals. This model was tested by calculating the droplet shapes in containerless experiments conducted to determine the surface tension of liquid metals. Inconsistencies associated with the results of a previous paper are elucidated. The computational results of the mathematical model are compared with the results of ground-based experiments for two different metals. The importance of the ratio of electromagnetic skin depth-to-droplet radius to the accuracy of the mathematical model is discussed. A planned alternate approach to modeling the shape by consideration of the entire droplet rather than only the surface is presented. As an example of an application. the influence of the shape on the splitting of the surface oscillation modes of levitated liquid metal droplets is discussed

TEMPUS: First results

The electromagnetic levitation facility, TEMPUS, developed by Dornier is designed to operate under microgravity conditions. Compared to terrestrial levitation, microgravity offers the possibility to melt and undercool in ultra high vacuum, thereby, providing an ultra clean environment. The technical concept of the TEMPUS facility was tested on two KC 135 flights and in the Texus 22 mission. Preparative investigations concerning the coil system and the heating and positioning efficiencies were carried out in the TEMPUS laboratory version. Furthermore, temperature-time profiles were determined under various boundary conditions. As a consequence of processing liquid metals under UHV, correct temperature measurement arises as the most critical problem. Experiences with experiments in the TEMPUS laboratory module show that due to the evaporation losses of the sample, the transmission of the CaF2 shielding windows changes drastically during the processing time. The investigation of the effect of contamination on pyrometry and the development of alternative evaporation shielding methods were initiated. During the second KC 135 flight, it was possible to heat up and melt an FeNi sample under He atmosphere. Oscillations of the molten sample, which were excited by switching out the magnetic heating field, could be detected and afterwards analyzed. From the frequency of these oscillations the surface tension of the sample material could be derived. The measurement of the surface tension and viscosity of an undercooled metal is proposed for TEMPUS on IML-2. This document is presented in view graph form

Mechanical vibrations of pendant liquid droplets

A simple optical deflection technique was used to monitor the vibrations of microlitre pendant droplets of deuterium oxide, formamide, and 1,1,2,2-tetrabromoethane. Droplets of different volumes of each liquid were suspended from the end of a microlitre pipette and vibrated using a small puff of nitrogen gas. A laser was passed through the droplets and the scattered light was collected using a photodiode. Vibration of the droplets resulted in the motion of the scattered beam and time-dependent intensity variations were recorded using the photodiode. These time- dependent variations were Fourier transformed and the frequencies and widths of the mechanical droplet resonances were extracted. A simple model of vibrations in pendant/sessile drops was used to relate these parameters to the surface tension, density and viscosity of the liquid droplets. The surface tension values obtained from this method were found to be in good agreement with results obtained using the standard pendant drop technique. Damping of capillary waves on pendant drops was shown to be similar to that observed for deep liquid baths and the kinematic viscosities obtained were in agreement with literature values for all three liquids studied

Measurement of thermophysical properties of liquid metallic alloys in a ground- and microgravity based research program. The Thermolab Project

An outline of the Thermolab Project is reported with the aim of informing on the wide range of properties which are becoming available for some industrial alloys. Selected examples of experiments and properties are provided

Metastable monotectic phase separation in Co–Cu alloys

The liquid phase separation behaviour of metastable monotectic Co–Cu alloys was investigated as a function of cooling rate using a 6.5 m drop-tube facility. A range of liquid phase separated morphologies were observed including stable two-layer core–shell, evolving core–shell and dendritic structures. It was found that in the core–shell structures the core was always in the higher melting point (Co-rich) phase, irrespective of the core and shell volume fraction. In Cu–50 at% Co alloy, high cooling rates were observed to yield two episodes of liquid phase separation, corresponding to binodal, followed by spinodal decomposition. The resulting structure comprised a core–shell structure in which the Co-rich core contained a very fine dispersion of Cu-rich particles with a Cu-rich shell which may, or may not, contain a similar dispersion of Co-rich particles