(2+1) resonant enhanced multiphoton ionization of H_2 via the E, F^(1)Σ^+_g state

In this paper, we report the results of ab initio calculations of photoelectron angular distributions and vibrational branching ratios for the (2+1) REMPI of H_2 via the E, F^(1)Σ^+_g state, and compare these with the experimental data of Anderson et al. [Chem. Phys. Lett. 105, 22 (1984)]. These results show that the observed non‐Franck–Condon behavior is predominantly due to the R dependence of the transition matrix elements, and to a lesser degree to the energy dependence. This work presents the first molecular REMPI study employing a correlated wave function to describe the Rydberg–valence mixing in the resonant intermediate state

Highly indistinguishable and strongly entangled photons from symmetric GaAs quantum dots

The development of scalable sources of non-classical light is fundamental to unlocking thetechnological potential of quantum photonics. Semiconductor quantum dots are emerging asnear-optimal sources of indistinguishable single photons. However, their performance assources of entangled-photon pairs are still modest compared to parametric down converters.Photons emitted from conventional Stranski–Krastanov InGaAs quantum dots have shownnon-optimal levels of entanglement and indistinguishability. For quantum networks, bothcriteria must be met simultaneously. Here, we show that this is possible with a system thathas received limited attention so far: GaAs quantum dots. They can emit triggered polar-ization-entangled photons with high purity (g(2)(0) = 0.002±0.002), high indistinguish-ability (0.93±0.07 for 2 ns pulse separation) and high entanglement fidelity(0.94±0.01). Our results show that GaAs might be the material of choice for quantum-dotentanglement sources in future quantum technologie

Nano-engineered hierarchical natural fibre composites with localised cellulose nanocrystals and tailored interphase for improved mechanical properties

Natural fibre composites have been utilised in many applications such as automotive and buildings, thanks to their high specific properties and environmentally friendly nature. However, the incompatibility between hydrophilic natural fibres and hydrophobic polymer resins remains a longstanding issue in natural fibre composites. Inspired by nature's hierarchical structures and tailored functionalities, a nano-engineered hierarchical natural fibre composite has been developed in this study, utilising cellulose nanocrystals (CNCs) as localised nano-reinforcements at flax surfaces in a flax/bio-epoxy system. A simple and versatile spray coating technique was used to deposit CNCs on unmodified flax fibres, without using any chemical solvents. With the increased surface roughness and hence improved epoxy wetting on nano-engineered flax surfaces (3 wt% CNC loading), mechanical properties of the hierarchical composites have been significantly improved, with a 60 % increase in interlaminar shear strength, indicating an enhanced interfacial load transfer between flax and epoxy, alongside improved flexural modulus (14 %) and strength (23 %). This green approach without using any chemicals provides a scalable and sustainable way to develop tailored interfaces for natural fibre composites with enhanced resin wetting and mechanical properties

Corrigendum to "Assessment of China's virtual air pollution transport embodied in trade by using a consumption-based emission inventory" published in Atmos. Chem. Phys., 15, 5443-5456, 2015

No abstract available

Assessment of China's virtual air pollution transport embodied in trade by using a consumption-based emission inventory

Substantial anthropogenic emissions from China have resulted in serious air pollution, and this has generated considerable academic and public concern. The physical transport of air pollutants in the atmosphere has been extensively investigated; however, understanding the mechanisms how the pollutant was transferred through economic and trade activities remains a challenge. For the first time, we quantified and tracked China's air pollutant emission flows embodied in interprovincial trade, using a multiregional input - output model framework. Trade relative emissions for four key air pollutants (primary fine particle matter, sulfur dioxide, nitrogen oxides and non-methane volatile organic compounds) were assessed for 2007 in each Chinese province. We found that emissions were significantly redistributed among provinces owing to interprovincial trade. Large amounts of emissions were embodied in the imports of eastern regions from northern and central regions, and these were determined by differences in regional economic status and environmental policy. It is suggested that measures should be introduced to reduce air pollution by integrating cross-regional consumers and producers within national agreements to encourage efficiency improvement in the supply chain and optimize consumption structure internationally. The consumption-based air pollutant emission inventory developed in this work can be further used to attribute pollution to various economic activities and final demand types with the aid of air quality models

Conductance fluctuations at the integer quantum Hall plateau transition

We study numerically conductance fluctuations near the integer quantum Hall effect plateau transition. The system is presumed to be in a mesoscopic regime, with phase coherence length comparable to the system size. We focus on a two-terminal conductance G for square samples, considering both periodic and open boundary conditions transverse to the current. At the plateau transition, G is broadly distributed, with a distribution function close to uniform on the interval between zero and one in units of e^2/h. Our results are consistent with a recent experiment by Cobden and Kogan on a mesoscopic quantum Hall effect sample.Comment: minor changes, 5 pages LaTex, 7 postscript figures included using epsf; to be published Phys. Rev. B 55 (1997

Universality in an integer Quantum Hall transition

An integer Quantum Hall effect transition is studied in a modulation doped p-SiGe sample. In contrast to most examples of such transitions the longitudinal and Hall conductivities at the critical point are close to 0.5 and 1.5 (e^2/h), the theoretically expected values. This allows the extraction of a scattering parameter, describing both conductivity components, which depends exponentially on filling factor. The strong similarity of this functional form to those observed for transitions into the Hall insulating state and for the B=0 metal- insulator transition implies a universal quantum critical behaviour for the transitions. The observation of this behaviour in the integer Quantum Hall effect, for this particular sample, is attributed to the short-ranged character of the potential associated with the dominant scatterers

Disappearance of integer quantum Hall effect

The disappearance of integer quantum Hall effect (IQHE) at strong disorder and weak magnetic field is studied in a lattice model. A generic sequence by which the IQHE plateaus disappear is revealed: higher IQHE plateaus always vanish earlier than lower ones, and extended levels between those plateaus do not float up in energy but keep merging together after the destruction of plateaus. All of these features remain to be true in the weak-field limit as shown by the thermodynamic-localization-length calculation. Topological characterization in terms of Chern integers provides a simple physical explanation and suggests a qualitative difference between the lattice and continuum models.Comment: Revtex, four pages; four figures, postscript fil

Approximating the monomer-dimer constants through matrix permanent

The monomer-dimer model is fundamental in statistical mechanics. However, it is #P-complete in computation, even for two dimensional problems. A formulation in matrix permanent for the partition function of the monomer-dimer model is proposed in this paper, by transforming the number of all matchings of a bipartite graph into the number of perfect matchings of an extended bipartite graph, which can be given by a matrix permanent. Sequential importance sampling algorithm is applied to compute the permanents. For two-dimensional lattice with periodic condition, we obtain $0.6627\pm0.0002$, where the exact value is $h_2=0.662798972834$. For three-dimensional lattice with periodic condition, our numerical result is $0.7847\pm0.0014$, {which agrees with the best known bound $0.7653 \leq h_3 \leq 0.7862$.}Comment: 6 pages, 2 figure

Network Models of Quantum Percolation and Their Field-Theory Representations

We obtain the field-theory representations of several network models that are relevant to 2D transport in high magnetic fields. Among them, the simplest one, which is relevant to the plateau transition in the quantum Hall effect, is equivalent to a particular representation of an antiferromagnetic SU(2N) ($N\to 0$) spin chain. Since the later can be mapped onto a $\theta\ne 0$, $U(2N)/U(N)\times U(N)$ sigma model, and since recent numerical analyses of the corresponding network give a delocalization transition with $\nu\approx 2.3$, we conclude that the same exponent is applicable to the sigma model