2,542 research outputs found

    Electronic Orders Induced by Kondo Effect in Non-Kramers f-Electron Systems

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    This paper clarifies the microscopic nature of the staggered scalar order, which is specific to even number of f electrons per site. In such systems, crystalline electric field (CEF) can make a singlet ground state. As exchange interaction with conduction electrons increases, the CEF singlet at each site gives way to Kondo singlets. The collective Kondo singlets are identified with itinerant states that form energy bands. Near the boundary of itinerant and localized states, a new type of electronic order appears with staggered Kondo and CEF singlets. We present a phenomenological three-state model that qualitatively reproduces the characteristic phase diagram, which have been obtained numerically with use of the continuous-time quantum Monte Carlo combined with the dynamical mean-field theory. The scalar order observed in PrFe_4P_{12} is ascribed to this staggered order accompanying charge density wave (CDW) of conduction electrons. Accurate photoemission and tunneling spectroscopy should be able to probe sharp peaks below and above the Fermi level in the ordered phase.Comment: 7 pages, 8 figure

    Electron And Positron Scattering From 1,1- C2 H2 F2

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    1,1-difluoroethylene (1,1- C2 H2 F2) molecules have been studied for the first time experimentally and theoretically by electron and positron impact. 0.4-1000 eV electron and 0.2-1000 eV positron impact total cross sections (TCSs) were measured using a retarding potential time-of-flight apparatus. In order to probe the resonances observed in the electron TCSs, a crossed-beam method was used to investigate vibrational excitation cross sections over the energy range of 1.3-49 eV and scattering angles 90Ā° and 120Ā° for the two loss energies 0.115 and 0.381 eV corresponding to the dominant C-H (2 and 9) stretching and the combined C-F (3) stretching and C H2 (11) rocking vibrations, respectively. Electron impact elastic integral cross sections are also reported for calculations carried out using the Schwinger multichannel method with pseudopotentials for the energy range from 0.5 to 50 eV in the static-exchange approximation and from 0.5 to 20 eV in the static-exchange plus polarization approximation. Resonance peaks observed centered at about 2.3, 6.5, and 16 eV in the TCSs have been shown to be mainly due to the vibrational and elastic channels, and assigned to the B2, B1, and A1 symmetries, respectively. The Ļ€* resonance peak at 1.8 eV in C2 H4 is observed shifted to 2.3 eV in 1,1- C2 H2 F2 and to 2.5 eV in C2 F4; a phenomenon attributed to the decreasing CC bond length from C2 H4 to C2 F4. For positron impact a conspicuous peak is observed below the positronium formation threshold at about 1 eV, and other less pronounced ones centered at about 5 and 20 eV. Ā© 2007 American Institute of Physics.12616(1997) Kyoto Protocol to the United Nations Framework Convention on Climate Change, , http://www.cnn.com/SPECIALS/1997/global.warming/stories/treaty, DecemberMitsui, Y., Ohira, Y., Yonemura, T., Takaichi, T., Sekiya, A., Beppu, T., (2004) J. Electrochem. Soc., 151, p. 297Panajotovic, R., Kitajima, M., Tanaka, H., Jelisavic, M., Lower, J., Campbell, L., Brunger, M.J., Buckman, S.J., (2003) J. Phys. B, 36, p. 1615Szmytkowski, C., Kwitnewski, S., Ptasinska-Denga, E., (2003) Phys. Rev. A, 68, p. 032715Brescansin, L.M., MacHado, L.E., Lee, M.-T., (1998) Phys. Rev. A, 57, p. 3504Winstead, C., McKoy, V., (2002) J. Chem. Phys., 116, p. 1380. , 0021-9606 10.1063/1.1429649Winstead, C., McKoy, V., Bettega, M.H.F., (2005) Phys. Rev. A, 72, p. 042721Coggiola, M.J., Flicker, W.M., Mosher, O.A., Kuppermann, A., (1976) J. Chem. Phys., 65, p. 2655Edgell, W.F., Byrd, W.E., (1949) J. Chem. Phys., 17, p. 740Smith, D.C., Nielsen, J.R., Classen, H.H., (1950) J. Chem. Phys., 16, p. 326Joyner, P., Glockler, G., (1952) J. Chem. Phys., 20, p. 302Roberts, A., Edgell, W.F., (1949) J. Chem. Phys., 17, p. 742. , 0021-9606Roberts, A., Edgell, W.F., (1949) Phys. Rev., 76, p. 178Allan, M., Craig, N.C., McCarty, L.V., (2002) J. Phys. B, 35, p. 523Wahl, R.L., (2002) Principles and Practice of Positron Emission Tomography, , Lippincott, New York/ Williams and Wilkins, BaltimoreSchultz, P.J., Lynn, K.G., (1988) Rev. Mod. Phys., 60, p. 701Mitroy, J., Bromley, M.W.J., Ryzhikh, G.G., (2002) J. Phys. B, 35, p. 81Sueoka, O., Mori, S., Hamada, A., (1994) J. Phys. B, 27, p. 1452Kimura, M., Makochekanwa, C., Sueoka, O., (2004) J. Phys. B, 37, p. 1461Hoffman, K.R., Dababneh, M.S., Hsieh, Y.F., Kauppila, W.E., Pol, V., Smart, J.H., Stein, T.S., (1982) Phys. Rev. A, 25, p. 1393Sueoka, O., Mori, S., (1986) J. Phys. B, 19, p. 4035Sueoka, O., Makochekanwa, C., Kawate, H., (2002) Nucl. Instrum. Methods Phys. Res. B, 192, p. 206Tanaka, H., Ishikawa, T., Masai, T., Sagara, T., Boesten, L., Takekawa, M., Itikawa, Y., Kimura, M., (1998) Phys. Rev. A, 57, p. 1798Srivastava, S.K., Chutjian, A., Trajmar, S., (1975) J. Chem. Phys., 63, p. 2659Takatsuka, K., McKoy, V., (1981) Phys. Rev. A, 24, p. 2473. , 1050-2947 10.1103/PhysRevA.24.2473Takatsuka, K., McKoy, V., (1984) Phys. Rev. A, 30, p. 1734Bettega, M.H.F., Ferreira, L.G., Lima, M.A.P., (1993) Phys. Rev. A, 47, p. 1111Bettega, M.H.F., Natalense, A.P.P., Lima, M.A.P., Ferreira, L.G., (2003) J. Phys. B, 36, p. 1263Lopes, A.R., Bettega, M.H.F., (2003) Phys. Rev. A, 67, p. 032711Varellado, T.M.N., Bettega, M.H.F., Lima, M.A.P., Ferreira, L.G., (1999) J. Chem. Phys., 111, p. 6396Rescigno, T.N., McCurdy, C.W., Schneider, B.I., (1989) Appl. Phys. Lett., 63, p. 248Winstead, C., McKoy, V., (1998) Phys. Rev. A, 57, p. 3589Bauschlicher, C.W., (1980) J. Chem. Phys., 72, p. 880(1998) CRC Handbook of Chemistry and Physics, , 79th ed., edited by D. R.Lide (CRC, Boca Raton, FLSueoka, O., Mori, S., (1989) J. Phys. B, 22, p. 963Panajotovic, R., Jelisavcic, M., Kajita, R., Tanaka, T., Kitajima, M., Cho, H., Tanaka, H., Buckman, S.J., (2004) J. Chem. Phys., 121, p. 4559Winstead, C., Sun, Q., McKoy, V., (1992) J. Chem. Phys., 96, p. 4246Kato, H., Makochekanwa, C., Hoshino, M., Kimura, M., Cho, H., Kume, T., Yamamoto, A., Tanaka, H., (2006) Chem. Phys. Lett., 425, p. 1Carlos Jr. J., L., Karl Jr. R., R., Bauer, S.H., (1974) J. Chem. Soc., Faraday Trans. 2, 2, p. 177Chiu, N.S., Burrow, P.D., Jordan, K.D., (1979) Chem. Phys. Lett., 68, p. 121Kimura, M., Sueoka, O., Makochekanwa, C., Kawate, H., Kawada, M., (2001) J. Chem. Phys., 115, p. 744

    Acceleration in perpendicular relativistic shocks for plasmas consisting of leptons and hadrons

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    We investigate the acceleration of light particles in perpendicular shocks for plasmas consisting of a mixture of leptonic and hadronic particles. Starting from the full set of conservation equations for the mixed plasma constituents, we generalize the magneto-hydrodynamical jump conditions for a multi-component plasma, including information about the specific adiabatic constants for the different species. The impact of deviations from the standard model of an ideal gas is compared in theory and particle-in-cell simulations, showing that the standard-MHD model is a good approximation. The simulations of shocks in electron-positron-ion plasmas are for the first time multi-dimensional, transverse effects are small in this configuration and 1D simulations are a good representation if the initial magnetization is chosen high. 1D runs with a mass ratio of 1836 are performed, which identify the Larmor frequency \omega_{ci} as the dominant frequency that determines the shock physics in mixed component plasmas. The maximum energy in the non-thermal tail of the particle spectra evolves in time according to a power-law proportional to t^\alpha with \alpha in the range 1/3 < \alpha < 1, depending on the initial parameters. A connection is made with transport theoretical models by Drury (1983) and Gargate & Spitkovsky (2011), which predict an acceleration time proportional to \gamma and the theory for small wavelength scattering by Kirk & Reville (2010), which predicts a behavior rather as proportional to \gamma^2. Furthermore, we compare different magnetic field orientations with B_0 inside and out of the plane, observing qualitatively different particle spectra than in pure electron-ion shocks

    Anisotropic heating and magnetic field generation due to Raman scattering in laser-plasma interactions

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    We identify a mechanism for magnetic field generation in the interaction of intense electromagnetic waves and underdense plasmas. We show that Raman scattered plasma waves trap and heat the electrons preferentially in their propagation direction, resulting in a temperature anisotropy. In the trail of laser pulse, we observe magnetic field growth that matches the Weibel mechanism due to the temperature anisotropy. We discuss the role of the initial electron temperature in our results. The predictions are confirmed with multidimensional particle-in-cell simulations. We show how this configuration is an experimental platform to study the long-time evolution of the Weibel instabilityinfo:eu-repo/semantics/publishedVersio

    Electron and positron scattering from 1,1-Cā‚‚Hā‚‚Fā‚‚

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    1,1-difluoroethylene (1,1-Cā‚‚Hā‚‚Fā‚‚) molecules have been studied for the first time experimentally and theoretically by electron and positron impact. 0.4-1000 eV electron and 0.2-1000 eV positron impact total cross sections (TCSs) were measured using a retarding potential time-of-flight apparatus. In order to probe the resonances observed in the electron TCSs, a crossed-beam method was used to investigate vibrational excitation cross sections over the energy range of 1.3-49 eV and scattering angles 90 degrees and 120 degrees for the two loss energies 0.115 and 0.381 eV corresponding to the dominant C-H (Ī½ā‚‚ and Ī½ā‚‰) stretching and the combined C-F (Ī½ā‚ƒ) stretching and CHā‚‚ (Ī½ā‚ā‚) rocking vibrations, respectively. Electron impact elastic integral cross sections are also reported for calculations carried out using the Schwinger multichannel method with pseudopotentials for the energy range from 0.5 to 50 eV in the static-exchange approximation and from 0.5 to 20 eV in the static-exchange plus polarization approximation. Resonance peaks observed centered at about 2.3, 6.5, and 16 eV in the TCSs have been shown to be mainly due to the vibrational and elastic channels, and assigned to the Bā‚‚, Bā‚, and Aā‚ symmetries, respectively. The pi* resonance peak at 1.8 eV in Cā‚‚Hā‚„ is observed shifted to 2.3 eV in 1,1-Cā‚‚Hā‚‚Fā‚‚ and to 2.5 eV in Cā‚‚Fā‚„; a phenomenon attributed to the decreasing C=C bond length from Cā‚‚Hā‚„ to Cā‚‚Fā‚„. For positron impact a conspicuous peak is observed below the positronium formation threshold at about 1 eV, and other less pronounced ones centered at about 5 and 20 eV.The work was supported in part by a Grant-in-Aid, the Ministry of Education, Science, Technology, Sport and Culture, Japan, the Japan Society for the Promotion of Science JSPS, and the Japan Atomic Energy Research Institute JAERI. One of the authors C.M. is also grateful to the JSPS for financial support under Grant No. P04064. Another author H.T. acknowledges Dr. T. Ozeki of the JAERI for his encouragement and support during this work. This work was also done under the International Atomic Energy Agency IAEA project for three of the authors C.M., M.H., and H.T.. Two of the authors M.H.F.B. and M.A.P.L. acknowledge support from the Brazilian agency Conselho Nacional de Desenvolvimento CientĆ­fico e TecnolĆ³gico CNPq. MHFB also acknowledges support from the ParanĆ” state agency FundaĆ§Ć£o AraucĆ”ria and from FINEP ( under Project No. CT-Infra 1)

    Electronic Order with Staggered Kondo and Crystalline Electric Field Singlets

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    Novel electronic order is found theoretically for a system where even number of localized electrons per site are coupled with conduction electrons. For precise quantitative study, a variant of the Kondo lattice model is taken with crystalline electric field (CEF) singlet and triplet states for each site. Using the dynamical mean-field theory combined with the continuous-time quantum Monte Carlo method, a staggered order with alternating Kondo and CEF singlets is identified for a case with one conduction electron per site being distributed in two conduction bands each of which is quarter-filled. This electronic order accompanies a charge density wave (CDW) of conduction electrons that accumulate more on Kondo-singlet sites than on CEF-singlet sites. Possible relevance of the present order to the scalar order in PrFe4_4P12_{12} is discussed.Comment: 11 pages, 17 figure

    Nonthermal Electron Acceleration at Collisionless Quasi-perpendicular Shocks

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    Shock waves propagating in collisionless heliospheric and astrophysical plasmas have been studied extensively over the decades. One prime motivation is to understand the nonthermal particle acceleration at shocks. Although the theory of diffusive shock acceleration (DSA) has long been the standard for cosmic-ray acceleration at shocks, plasma physical understanding of particle acceleration remains elusive. In this review, we discuss nonthermal electron acceleration mechanisms at quasi-perpendicular shocks, for which substantial progress has been made in recent years. The discussion presented in this review is restricted to the following three specific topics. The first is stochastic shock drift acceleration (SSDA), which is a relatively new mechanism for electron injection into DSA. The basic mechanism, related in-situ observations and kinetic simulations results, and how it is connected with DSA will be discussed. Second, we discuss shock surfing acceleration (SSA) at very high Mach number shocks relevant to young supernova remnants (SNRs). While the original proposal under the one-dimensional assumption is unrealistic, SSA has now been proven efficient by a fully three-dimensional kinetic simulation. Finally, we discuss the current understanding of the magnetized Weibel-dominated shock. Spontaneous magnetic reconnection of self-generated current sheets within the shock structure is an interesting consequence of Weibel-generated strong magnetic turbulence. We argue that high Mach number shocks with both Alfven and sound Mach numbers exceeding 20-40 will likely behave as a Weibel-dominated shock. Despite a number of interesting recent findings, the relative roles of SSDA, SSA, and magnetic reconnection for electron acceleration at collisionless shocks and how the dominant particle acceleration mechanisms change depending on shock parameters remain to be answered.Comment: To appear in Reviews of Modern Plasma Physics as an invited revie

    Substitution effects in elastic electron collisions with CHā‚ƒX (X=F, Cl, Br, I) molecules

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    We report absolute elastic differential, integral, and momentum transfer cross sections for electron interactions with the series of molecules CHā‚ƒX (X=F, Cl, Br, I). The incident electron energy range is 50ā€“200 eV, while the scattered electron angular range for the differential measurements is 15Ā°ā€“150Ā°. In all cases the absolute scale of the differential cross sections was set using the relative flow method with helium as the reference species. Substitution effects on these cross sections, as we progress along the halomethane series CHā‚ƒF, CHā‚ƒCl, CH3Br, and CHā‚ƒI, are investigated as a part of this study. In addition, atomic-like behavior in these scattering systems is also considered by comparing these halomethane elastic cross sections to results from other workers for the corresponding noble gases Ne, Ar, Kr, and Xe, respectively. Finally we report results for calculations of elastic differential and integral cross sections for electrons scattering from each of the CHā‚ƒX species, within an optical potential method and assuming a screened corrected independent atom representation. The level of agreement between these calculations and our measurements was found to be quite remarkable in each case.This work was conducted under the support of the Japanese Ministry of Education, Sport, Culture and Technology and also by the Ministerio de EducaciĆ³n Ciencia e InnovaciĆ³n Plan Nacional de Fisica, Project No. FIS2006- 00702, the Consejo de Seguridad Nuclear and the European Science Foundation COST Action No. CM0601. Additional support from the Australian Research Council, through its Centres of Excellence Program, and the Korea Science and Engineering Foundation Grant No. 2009-0052415 is further noted. One of us H.K. also acknowledges the Japan Society for the Promotion of Science JSPS for his fellowships as grants-in-aid for scientific research and, most recently, to facilitate his visit to Flinders University and the ANU
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