Localized exciton-polariton modes in dye-doped nanospheres: a quantum approach

We model a dye-doped polymeric nanosphere as an ensemble of quantum emitters and use it to investigate the localized exciton-polaritons supported by such a nanosphere. By determining the time evolution of the density matrix of the collective system, we explore how an incident laser field may cause transient optical field enhancement close to the surface of such nanoparticles. Our results provide further evidence that excitonic materials can be used to good effect in nanophotonics.Comment: 16 pages, 4 figure

Time varying gratings model Hawking radiation

Diffraction gratings synthetically moving at trans-luminal velocities contain points where wave and grating velocities are equal. We show these points can be understood as a series of optical event horizons where wave energy can be trapped and amplified, leading to radiation from the quantum vacuum state. We calculate the spectrum of this emitted radiation, finding a quasi-thermal spectrum with features that depend on the grating profile, and an effective temperature that scales exponentially with the length of the grating, emitting a measurable flux even for very small grating contrast.Comment: 13 pages, 4 figure

Graph theory approach to exceptional points in wave scattering

In this paper, we use graph theory to solve wave scattering problems in the discrete dipole approximation. As a key result of this work, in the presence of active scatterers, we show how one can find arbitrary large-order zero eigenvalue exceptional points (EPs) in parameter space by solving a set of non-linear equations. We interpret these equations in a graph theory picture as vanishing sums of scattering events. We also show how the total field of the system responds to parameter perturbations at the EP. Finally, we investigate the sensitivity of the power output to imaginary perturbation in the design frequency. This perturbation can be employed to trade sensitivity for a different dissipation balance of the system.Comment: 15 pages, 11 figure

High-dimensional spatial mode sorting and optical circuit design using multi-plane light conversion

Multi-plane light converters (MPLCs) are an emerging class of optical device capable of converting a set of input spatial light modes to a new target set of output modes. This operation represents a linear optical transformation - a much sought after capability in photonics. MPLCs have potential applications in both the classical and quantum optics domains, in fields ranging from optical communications, to optical computing and imaging. They consist of a series of diffractive optical elements (the 'planes'), typically separated by free-space. The phase delays imparted by each plane are determined by the process of inverse-design, most often using an adjoint algorithm known as the wavefront matching method (WMM), which optimises the correlation between the target and actual MPLC outputs. In this work we investigate high mode capacity MPLCs to create arbitrary spatial mode sorters and linear optical circuits. We focus on designs possessing low numbers of phase planes to render these MPLCs experimentally feasible. To best control light in this scenario, we develop a new inverse-design algorithm, based on gradient ascent with a specifically tailored objective function, and show how in the low-plane limit it converges to MPLC designs with substantially lower modal cross-talk and higher fidelity than achievable using the WMM. We experimentally demonstrate several prototype few-plane high-dimensional spatial mode sorters, operating on up to 55 modes, capable of sorting photons based on their Zernike mode, orbital angular momentum state, or an arbitrarily randomized spatial mode basis. We discuss the advantages and drawbacks of these proof-of-principle prototypes, and describe future improvements. Our work points to a bright future for high-dimensional MPLC-based technologies

All-optically untangling light propagation through multimode fibres

When light propagates through a complex medium, such as a multimode optical fibre (MMF), the spatial information it carries is scrambled. In this work we experimentally demonstrate an all-optical strategy to unscramble this light again. We first create a digital model capturing the way light has been scattered, and then use this model to inverse-design and build a complementary optical system - which we call an optical inverter - that reverses this scattering process. Our implementation of this concept is based on multi-plane light conversion, and can also be understood as a diffractive artificial neural network or a physical matrix pre-conditioner. We present three design strategies allowing different aspects of device performance to be prioritised. We experimentally demonstrate a prototype optical inverter capable of simultaneously unscrambling up to 30 spatial modes that have propagated through a 1m long MMF, and show how this enables near instantaneous incoherent imaging, without the need for any beam scanning or computational processing. We also demonstrate the reconfigurable nature of this prototype, allowing it to adapt and deliver a new optical transformation if the MMF it is matched to changes configuration. Our work represents a first step towards a new way to see through scattering media. Beyond imaging, this concept may also have applications to the fields of optical communications, optical computing and quantum photonics.Comment: 18 pages, 11 figure

Classical antennae, quantum emitters, and densities of optical states

We provide a pedagogical introduction to the concept of the local density of optical states (LDOS), illustrating its application to both the classical and quantum theory of radiation. We show that the LDOS governs the efficiency of a macroscopic classical antenna, determining how the antenna's emission depends on its environment. The LDOS is shown to similarly modify the spontaneous emission rate of a quantum emitter, such as an excited atom, molecule, ion, or quantum dot that is embedded in a nanostructured optical environment. The difference between the number density of optical states, the local density of optical states, and the partial local density of optical states is elaborated and examples are provided for each density of states to illustrate where these are required. We illustrate the universal effect of the LDOS on emission by comparing systems with emission wavelengths that differ by more than 5 orders of magnitude, and systems whose decay rates differ by more than 5 orders of magnitude. To conclude we discuss and resolve an apparent difference between the classical and quantum expressions for the spontaneous emission rate that often seems to be overlooked, and discuss the experimental determination of the LDOS.Comment: 80 pages, 19 figure

Optical simulation of quantum mechanics on the Mobius strip, Klein's bottle and other manifolds, and Talbot effect

We analyse the evolution of the wavefunction of a quantum particle propagating on several compact manifolds, including the Klein bottle, Mobius strip and projective plane. We find analytically the stationary states and the energy spectrum and show that the wavefunction exhibits perfect revivals. Using the orbifold structure of the discussed manifolds, we establish the relation of wave evolution on the manifolds to Fresnel diffraction and consequently to the Talbot effect. This connection provides a novel method of optical simulation of the quantum motion on compact manifolds. We discuss some novel phenomena as well as the effects of topology on the properties of the waves on the manifolds

Quantum-classical correspondence in spin-boson equilibrium states at arbitrary coupling

It is known that the equilibrium properties of nanoscale systems can deviate significantly from standard thermodynamics due to their coupling to an environment. For the generalized $\theta$-angled spin-boson model, here we derive an explicit form of the classical mean force equilibrium state. Taking the large spin limit of the quantum spin-boson model, we demonstrate that the quantum-classical correspondence is maintained at arbitrary coupling strength. This correspondence gives insight into the conditions for a quantum system to be well-approximated by its classical counterpart. We further demonstrate that, counterintuitively, previously identified environment-induced 'coherences' in the equilibrium state of weakly coupled quantum spins, do not disappear in the classical case. Finally, we categorise various coupling regimes, from ultra-weak to ultra-strong, and find that the same value of coupling strength can either be 'weak' or 'strong', depending on whether the system is quantum or classical. Our results shed light on the interplay of quantum and mean force corrections in equilibrium states of the spin-boson model, and will help draw the quantum to classical boundary in a range of fields, such as magnetism and exciton dynamics