885 research outputs found
Crystallization Kinetics of Colloidal Spheres under Stationary Shear Flow
A systematic experimental study of dispersions of charged colloidal spheres
is presented on the effect of steady shear flow on nucleation and
crystal-growth rates. In addition, the non-equilibrium phase diagram as far as
the melting line is concerned is measured. Shear flow is found to strongly
affect induction times, crystal growth rates and the location of the melting
line. The main findings are that (i) the crystal growth rate for a given
concentration exhibits a maximum as a function of the shear rate, (ii) contrary
to the monotonous increase of the growth rate with increasing concentration in
the absence of flow, a maximum of the crystal growth rate as a function of
concentration is observed for sheared systems, and (iii) the induction time for
a given concentration exhibits a maximum as a function of the shear rate. These
findings will be partly explained on a qualitative level.Comment: 17 pages, 10 figures, accepted in Langmui
Supersaturated dispersions of rod-like viruses with added attraction
The kinetics of isotropic-nematic (I-N) and nematic-isotropic (N-I) phase
transitions in dispersions of rod-like {\it fd}-viruses are studied.
Concentration quenches were applied using pressure jumps in combination with
polarization microscopy, birefringence and turbidity measurements. The full
biphasic region could be accessed, resulting in the construction of a first
experimental analogue of the bifurcation diagram. The N-I spinodal points for
dispersions of rods with varying concentrations of depletion agents (dextran)
were obtained from orientation quenches, using cessation of shear flow in
combination with small angle light scattering. We found that the location of
the N-I spinodal point is independent of the attraction, which was confirmed by
theoretical calculations. Surprisingly, the experiments showed that also the
absolute induction time, the critical nucleus and the growth rate are
insensitive of the attraction, when the concentration is scaled to the distance
to the phase boundaries.Comment: 13 pages, 14 figures. accepted in Phsical Review
Primary tunnel junction thermometry
We describe the concept and experimental demonstration of primary thermometry
based on a four probe measurement of a single tunnel junction embedded within
four arrays of junctions. We show that in this configuration random sample
specific and environment-related errors can be avoided. This method relates
temperature directly to Boltzmann constant, which will form the basis of the
definition of temperature and realization of official temperature scales in the
future
Josephson current through a quantum dot coupled to a molecular magnet
Josephson currents are carried by sharp Andreev states within the
superconducting energy gap. We theoretically study the electronic transport of
a magnetically tunable nanoscale junction consisting of a quantum dot connected
to two superconducting leads and coupled to the spin of a molecular magnet. The
exchange interaction between the molecular magnet and the quantum dot modifies
the Andreev states due to a spin-dependent renormalization of the quantum dot's
energy level and the induction of spin-flips. A magnetic field applied to the
central region of the quantum dot and the molecular magnet further tunes the
Josephson current and starts a precession of the molecular magnet's spin. We
use a non-equilibrium Green's function approach to evaluate the transport
properties of the junction. Our calculations reveal that the energy level of
the dot, the magnetic field and the exchange interaction between the molecular
magnet and the electrons occupying the energy level of the quantum dot can
trigger transitions from a 0 to a state of the Josephson junction. The
redistribution of the occupied states induced by the magnetic field strongly
modifies the current-phase relation. The critical current exhibits a sharp
increase as a function of either the energy level of the dot, the magnetic
field or the exchange interaction.Comment: 10 pages, 7 figure
Double oxidation scheme for tunnel junction fabrication
The authors report a method to achieve Al–AlOx–Al tunnel junctions with high specific resistance in a controlled manner using a double oxidation technique. The technique is based on the standard method for oxidation repeated on an additional Al layer. The tunnel junctions were characterized with standard methods, such as comparison of room temperature resistance with liquid helium resistance and the authors found them to be of comparable quality to junctions fabricated with standard single oxidation. Fitting with the Simmons model suggests that both the barrier width and barrier height are consistent with those obtained in a single oxidation step. The junction specific capacitance was determined at low temperature to be 68fF/μm2. These junctions, employed in low temperature measurements and applications, demonstrate expected and stable conductance characteristics. The double oxidation method is straightforward to implement in a basic setup for tunnel junction fabrication.Peer reviewe
Pupil dilation as an implicit measure of appetitive Pavlovian learning
Appetitive Pavlovian conditioning is a learning mechanism of fundamental biological and pathophysiological significance. Nonetheless, its exploration in humans remains sparse, which is partly attributed to the lack of an established psychophysiological parameter that aptly represents conditioned responding. This study evaluated pupil diameter and other ocular response measures (gaze dwelling time, blink duration and count) as indices of conditioning. Additionally, a learning model was used to infer participants' learning progress on the basis of their pupil dilation. Twenty-nine healthy volunteers completed an appetitive differential delay conditioning paradigm with a primary reward, while the ocular response measures along with other psychophysiological (heart rate, electrodermal activity, postauricular and eyeblink reflex) and behavioral (ratings, contingency awareness) parameters were obtained to examine the relation among different measures. A significantly stronger increase in pupil diameter, longer gaze duration and shorter eyeblink duration was observed in response to the reward-predicting cue compared to the control cue. The Pearce-Hall attention model best predicted the trial-by-trial pupil diameter. This conditioned response was corroborated by a pronounced heart rate deceleration to the reward-predicting cue, while no conditioning effect was observed in the electrodermal activity or startle responses. There was no discernible correlation between the psychophysiological response measures. These results highlight the potential value of ocular response measures as sensitive indices for representing appetitive conditioning
Collective diffusion in charge-stabilized suspensions: Concentration and salt effects
The authors present a joint experimental-theoretical study of collective diffusion properties in aqueous suspensions of charge-stabilized fluorinated latex spheres. Small-angle x-ray scattering and x-ray photon correlation spectroscopy have been used to explore the concentration and ionic-strength dependence of the static and short-time dynamic properties including the hydrodynamic function H (q), the wave-number-dependent collective diffusion coefficient D (q), and the intermediate scattering function over the entire accessible range. They show that all experimental data can be quantitatively described and explained by means of a recently developed accelerated Stokesian dynamics simulation method, in combination with a modified hydrodynamic many-body theory. In particular, the behavior of H (q) for de-ionized and dense suspensions can be attributed to the influence of many-body hydrodynamics, without any need for postulating hydrodynamic screening to be present, as it was done in earlier work. Upper and lower boundaries are provided for the peak height of the hydrodynamic function and for the short-time self-diffusion coefficient over the entire range of added salt concentrations.Fil: Gapinski, J.. A. Mickiewicz University; PoloniaFil: Patkowski, A.. A. Mickiewicz University; PoloniaFil: Banchio, Adolfo Javier. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Física Enrique Gaviola. Universidad Nacional de Córdoba. Instituto de Física Enrique Gaviola; ArgentinaFil: Holmqvist, P.. Helmholtz Gemeinschaft. Forschungszentrum Jülich; AlemaniaFil: Meier, Guillermo Enrique. Helmholtz Gemeinschaft. Forschungszentrum Jülich; AlemaniaFil: Lettinga, M.P.. Helmholtz Gemeinschaft. Forschungszentrum Jülich; AlemaniaFil: Nägele, G.. Helmholtz Gemeinschaft. Forschungszentrum Jülich; Alemani
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