Tailoring the magnetodynamic properties of nanomagnets using magnetocrystalline and shape anisotropies

Magnetodynamical properties of nanomagnets are affected by the demagnetizing fields created by the same nanoelements. In addition, magnetocrystalline anisotropy produces an effective field that also contributes to the spin dynamics. In this article we show how the dimensions of magnetic elements can be used to balance crystalline and shape anisotropies, and that this can be used to tailor the magnetodynamic properties. We study ferromagnetic ellipses patterned from a 10 nm thick epitaxial Fe film with dimensions ranging from 50 x 150 nm to 150 x 450 nm. The study combines ferromagnetic resonance (FMR) spectroscopy with analytical calculations and micromagnetic simulations, and proves that the dynamical properties can be effectively controlled by changing the size of the nanomagnets. We also show how edge defects in the samples influence the magnetization dynamics. Dynamical edge modes localized along the sample edges are strongly influenced by edge defects, and this needs to be taken into account in understanding the full FMR spectrumComment: Accepted for publication in Phys. Rev.

Giant and time-dependent magnetocaloric effect in high-spin molecular magnets

We have measured and calculated the magnetocaloric effect in macroscopic samples of oriented high-spin molecular clusters like Mn12 and Fe8 as a function of the temperature and both the intensity and the sweeping rate of the applied magnetic field. We have observed a high magnetic entropy variation around the blocking temperature of the magnetic moment of molecules and calculated the shift of the entropy variation and cooling temperature, with the sweeping rate of the magnetic field.Comment: 10 pages, 3 figure

Thickness and temperature dependence of the magnetodynamic damping of pulsed laser deposited La0.7Sr0.3MnO3\text{La}_{0.7}\text{Sr}_{0.3}\text{MnO}_3 on (111)-oriented SrTiO3\text{O}_3

We have investigated the magnetodynamic properties of $\text{La}_{0.7}\text{Sr}_{0.3}\text{MnO}_3$ (LSMO) films of thickness 10, 15 and 30 nm grown on (111)-oriented SrTi$\text{O}_3$ (STO) substrates by pulsed laser deposition. Ferromagnetic resonance (FMR) experiments were performed in the temperature range 100--300 K, and the magnetodynamic damping parameter $\alpha$ was extracted as a function of both film thickness and temperature. We found that the damping is lowest for the intermediate film thickness of 15 nm with $\alpha \approx 2 \cdot 10^{-3}$, where $\alpha$ is relatively constant as a function of temperature well below the Curie temperature of the respective films.Comment: Accepted for publication in Journal of Magnetism and Magnetic Material

Magneto-Acoustic Waves in antiferromagnetic CuMnAs excited by Surface Acoustic Waves

Magnetoelastic effects in antiferromagnetic CuMnAs are investigated by applying dynamic strain in the 0.01% range through surface acoustic waves in the GaAs substrate. The magnetic state of the CuMnAs/GaAs is characterized by a multitude of submicron-sized domains which we image by x-ray magnetic linear dichroism combined with photoemission electron microscopy. Within the explored strain range, CuMnAs shows magnetoelastic effects in the form of N\'eel vector waves with micrometer wavelength, which corresponds to an averaged overall spin-axis rotation up to 2.4 deg driven by the time-dependent strain from the surface acoustic wave. Measurements at different temperatures indicate a reduction of the wave amplitude when lowering the temperature. However, no domain wall motion has been detected on the nanosecond timescal

Giant and time-dependent magnetocaloric effect in high-spin molecular magnets

We have measured and calculated the magnetocaloric effect in macroscopic samples of oriented high-spin molecular clusters like Mn12 and Fe8 as a function of the temperature and both the intensity and the sweeping rate of the applied magnetic field. We have observed a high magnetic entropy variation around the blocking temperature of the magnetic moment of molecules and calculated the shift of the entropy variation and cooling temperature, with the sweeping rate of the magnetic field