Relativistic time dilatation and the spectrum of electrons emitted by 33 TeV lead ions penetrating thin foils

We study the energy distribution of ultrarelativistic electrons produced when a beam of 33 TeV Pb$^{81+}$(1s) ions penetrates a thin Al foil. We show that, because of a prominent role of the excitations of the ions inside the foil which becomes possible due to the relativistic time dilatation, the width of this distribution can be much narrower compared to the case when the ions interact with rarefied gaseous targets. We also show that a very similar shape of the energy distribution may arise when 33 TeV Pb$^{82+}$ ions penetrate a thin Au foil. These results shed some light on the origin of the very narrow electron energy distributions observed experimentally about a decade ago.Comment: Four pages, two figure

Energy and Angular Distribution of Electrons Ejected from Helium by Fast Protons and Electrons: Theory and Experiment

A comprehensive study of the angular and energy distributions of electrons ejected in collisions of fast electrons and protons with He is presented. New experimental results for 300-keV, 1-MeV, and 5-MeV proton impact are reported along with theoretical results for 2-keV electron impact and 100-keV, 300-keV, 1-MeV, and 5-MeV proton impact. The theoretical results, based upon Born approximation with Hartree-Slater initial discrete and final continuum wave functions, show excellent agreement with experimental electron-impact results. Serious discrepancies are found between theory and experiment in the angular distribution of ejected electrons for forward angles for 100- and 300-keV proton impact; the discrepancies decrease markedly for 1-MeV proton impact and are absent for 5-MeV protons. The agreement between theory and experiment for intermediate and backward angles of electron ejection, on the other hand, is uniformly good for all proton impact energies. The reasons for this behavior in terms of a charge-exchange process to a continuum state contributing to electron ejection at forward angles is discussed, and the energy dependence of the data is shown to be consistent with this explanation

The Role of Bulk and Interface Recombination in High‐Efficiency Low‐Dimensional Perovskite Solar Cells

2D Ruddlesden–Popper perovskite (RPP) solar cells have excellent environmental stability. However, the power conversion efficiency (PCE) of RPP cells remains inferior to 3D perovskite-based cells. Herein, 2D (CH(CH)NH)(CHNH)PbI perovskite cells with different numbers of [PbI] sheets (n = 2–4) are analyzed. Photoluminescence quantum yield (PLQY) measurements show that nonradiative open-circuit voltage (V) losses outweigh radiative losses in materials with n > 2. The n = 3 and n = 4 films exhibit a higher PLQY than the standard 3D methylammonium lead iodide perovskite although this is accompanied by increased interfacial recombination at the top perovskite/C interface. This tradeoff results in a similar PLQY in all devices, including the n = 2 system where the perovskite bulk dominates the recombination properties of the cell. In most cases the quasi-Fermi level splitting matches the device V within 20 meV, which indicates minimal recombination losses at the metal contacts. The results show that poor charge transport rather than exciton dissociation is the primary reason for the reduction in fill factor of the RPP devices. Optimized n = 4 RPP solar cells had PCEs of 13% with significant potential for further improvements

Role of charge patches in ion guiding through nanocapillaries in a PET polymer

We studied the dynamic properties of ion guiding through nanocapillaries in insulating polyethylene terephthalate (PET). The angular distribution of the transmitted ions was measured as a function of time. The temporal evolution of the angular transmission profiles was acquired for the capillary diameters of 200 and 400 nm. The tilt angle was varied from 0° to 6.5°. The transmission profiles exhibit significant changes in position as time varies. This observation is explained by the formation of temporary charge patches produced in the interior of the capillary besides the primary charge patch created in the entrance region.</p

Post-Prior discrepancies in CDW-EIS calculations for ion impact ionization fully differential cross sections

In this work we present fully differential cross sections (FDCSs) calculations using post and prior version of CDW--EIS theory for helium single ionization by 100 MeV C$^{6+}$ amu$^{-1}$ and 3.6 MeV amu$^{-1}$ Au$^{24+}$ and Au$^{53+}$ ions. We performed our calculations for different momentum transfer and ejected electron energies. The influence of internuclear potential on the ejected electron spectra is taken into account in all cases. We compare our calculations with absolute experimental measurements. It is shown that prior version calculations give better agreement with experiments in almost all studied cases.Comment: 9 pages, 7 figure

High-order Harmonic Spectroscopy of the Cooper Minimum in Argon: Experimental and Theoretical Study

We study the Cooper minimum in high harmonic generation from argon atoms using long wavelength laser pulses. We find that the minimum in high harmonic spectra is systematically shifted with respect to total photoionization cross section measurements. We use a semi-classical theoretical approach based on Classical Trajectory Monte Carlo and Quantum Electron Scattering methods (CTMC-QUEST) to model the experiment. Our study reveals that the shift between photoionization and high harmonic emission is due to several effects: the directivity of the recombining electrons and emitted polarization, and the shape of the recolliding electron wavepacket.Comment: 13 page

Interactions of Ar(9+) and metastable Ar(8+) with a Si(100) surface at velocities near the image acceleration limit

Auger LMM spectra and preliminary model simulations of Ar(9+) and metastable Ar(8+) ions interacting with a clean monocrystalline n-doped Si(100) surface are presented. By varying the experimental parameters, several yet undiscovered spectroscopic features have been observed providing valuable hints for the development of an adequate interaction model. On our apparatus the ion beam energy can be lowered to almost mere image charge attraction. High data acquisition rates could still be maintained yielding an unprecedented statistical quality of the Auger spectra.Comment: 34 pages, 11 figures, http://pikp28.uni-muenster.de/~ducree

Managing phase purities and crystal orientation for high-performance and photostable cesium lead halide perovskite solar cells

Inorganic perovskites with cesium (Cs+) as the cation have great potential as photovoltaic materials if their phase purity and stability can be addressed. Herein, a series of inorganic perovskites is studied, and it is found that the power conversion efficiency of solar cells with compositions CsPbI1.8Br1.2, CsPbI2.0Br1.0, and CsPbI2.2Br0.8 exhibits a high dependence on the initial annealing step that is found to significantly affect the crystallization and texture behavior of the final perovskite film. At its optimized annealing temperature, CsPbI1.8Br1.2 exhibits a pure orthorhombic phase and only one crystal orientation of the (110) plane. Consequently, this allows for the best efficiency of up to 14.6% and the longest operational lifetime, T S80, of ≈300 h, averaged of over six solar cells, during the maximum power point tracking measurement under continuous light illumination and nitrogen atmosphere. This work provides essential progress on the enhancement of photovoltaic performance and stability of CsPbI3 − x Brx perovskite solar cells

Scaling and Formulary cross sections for ion-atom impact ionization

The values of ion-atom ionization cross sections are frequently needed for many applications that utilize the propagation of fast ions through matter. When experimental data and theoretical calculations are not available, approximate formulas are frequently used. This paper briefly summarizes the most important theoretical results and approaches to cross section calculations in order to place the discussion in historical perspective and offer a concise introduction to the topic. Based on experimental data and theoretical predictions, a new fit for ionization cross sections is proposed. The range of validity and accuracy of several frequently used approximations (classical trajectory, the Born approximation, and so forth) are discussed using, as examples, the ionization cross sections of hydrogen and helium atoms by various fully stripped ions.Comment: 46 pages, 8 figure