124 research outputs found
Local effective dynamics of quantum systems: A generalized approach to work and heat
By computing the local energy expectation values with respect to some local
measurement basis we show that for any quantum system there are two
fundamentally different contributions: changes in energy that do not alter the
local von Neumann entropy and changes that do. We identify the former as work
and the latter as heat. Since our derivation makes no assumptions on the system
Hamiltonian or its state, the result is valid even for states arbitrarily far
from equilibrium. Examples are discussed ranging from the classical limit to
purely quantum mechanical scenarios, i.e. where the Hamiltonian and the density
operator do not commute.Comment: 5 pages, 1 figure, published versio
Coherence of single spins coupled to a nuclear spin bath of varying density
The dynamics of single electron and nuclear spins in a diamond lattice with
different 13C nuclear spin concentration is investigated. It is shown that
coherent control of up to three individual nuclei in a dense nuclear spin
cluster is feasible. The free induction decays of nuclear spin Bell states and
single nuclear coherences among 13C nuclear spins are compared and analyzed.
Reduction of a free induction decay time T2* and a coherence time T2 upon
increase of nuclear spin concentration has been found. For diamond material
with depleted concentration of nuclear spin, T2* as long as 30 microseconds and
T2 of up to 1.8 ms for the electron spin has been observed. The 13C
concentration dependence of T2* is explained by Fermi contact and dipolar
interactions with nuclei in the lattice. It has been found that T2 decreases
approximately as 1/n, where n is 13C concentration, as expected for an electron
spin interacting with a nuclear spin bath.Comment: 4 pages, 4 figures, 1 movie (avi), 1 supplementary material (pdf
Towards T1-limited magnetic resonance imaging using Rabi beats
Two proof-of-principle experiments towards T1-limited magnetic resonance
imaging with NV centers in diamond are demonstrated. First, a large number of
Rabi oscillations is measured and it is demonstrated that the hyperfine
interaction due to the NV's 14N can be extracted from the beating oscillations.
Second, the Rabi beats under V-type microwave excitation of the three hyperfine
manifolds is studied experimentally and described theoretically.Comment: 6 pages, 8 figure
The negatively charged nitrogen-vacancy centre in diamond: the electronic solution
The negatively charged nitrogen-vacancy centre is a unique defect in diamond
that possesses properties highly suited to many applications, including quantum
information processing, quantum metrology, and biolabelling. Although the
unique properties of the centre have been extensively documented and utilised,
a detailed understanding of the physics of the centre has not yet been
achieved. Indeed there persists a number of points of contention regarding the
electronic structure of the centre, such as the ordering of the dark
intermediate singlet states. Without a sound model of the centre's electronic
structure, the understanding of the system's unique dynamical properties can
not effectively progress. In this work, the molecular model of the defect
centre is fully developed to provide a self consistent model of the complete
electronic structure of the centre. The application of the model to describe
the effects of electric, magnetic and strain interactions, as well as the
variation of the centre's fine structure with temperature, provides an
invaluable tool to those studying the centre and a means to design future
empirical and ab initio studies of this important defect.Comment: 24 pages, 6 figures, 10 table
Sensing electric fields using single diamond spins
The ability to sensitively detect charges under ambient conditions would be a
fascinating new tool benefitting a wide range of researchers across
disciplines. However, most current techniques are limited to low-temperature
methods like single-electron transistors (SET), single-electron electrostatic
force microscopy and scanning tunnelling microscopy. Here we open up a new
quantum metrology technique demonstrating precision electric field measurement
using a single nitrogen-vacancy defect centre(NV) spin in diamond. An AC
electric field sensitivity reaching ~ 140V/cm/\surd Hz has been achieved. This
corresponds to the electric field produced by a single elementary charge
located at a distance of ~ 150 nm from our spin sensor with averaging for one
second. By careful analysis of the electronic structure of the defect centre,
we show how an applied magnetic field influences the electric field sensing
properties. By this we demonstrate that diamond defect centre spins can be
switched between electric and magnetic field sensing modes and identify
suitable parameter ranges for both detector schemes. By combining magnetic and
electric field sensitivity, nanoscale detection and ambient operation our study
opens up new frontiers in imaging and sensing applications ranging from
material science to bioimaging
Correlation between arterial blood volume obtained by arterial spin labelling and cerebral blood volume in intracranial tumours
Assessment of MRI contrast agent concentration by quantitative susceptibility mapping (QSM): application to estimation of cerebral blood volume during steady state
BOLD Correlates of Trial-by-Trial Reaction Time Variability in Gray and White Matter: A Multi-Study fMRI Analysis
Reaction time (RT) is one of the most widely used measures of performance in experimental psychology, yet relatively few fMRI studies have included trial-by-trial differences in RT as a predictor variable in their analyses. Using a multi-study approach, we investigated whether there are brain regions that show a general relationship between trial-by-trial RT variability and activation across a range of cognitive tasks.The relation between trial-by-trial differences in RT and brain activation was modeled in five different fMRI datasets spanning a range of experimental tasks and stimulus modalities. Three main findings were identified. First, in a widely distributed set of gray and white matter regions, activation was delayed on trials with long RTs relative to short RTs, suggesting delayed initiation of underlying physiological processes. Second, in lateral and medial frontal regions, activation showed a "time-on-task" effect, increasing linearly as a function of RT. Finally, RT variability reliably modulated the BOLD signal not only in gray matter but also in diffuse regions of white matter.The results highlight the importance of modeling trial-by-trial RT in fMRI analyses and raise the possibility that RT variability may provide a powerful probe for investigating the previously elusive white matter BOLD signal
Pion-Myon-Gitterfuehrung in Metallen und Halbleitern
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