1,829 research outputs found
Spin dynamics of heterometallic Cr7M wheels (M = Mn, Zn, Ni) probed by inelastic neutron scattering
Inelastic neutron scattering has been applied to the study of the spin
dynamics of Cr-based antiferromagnetic octanuclear rings where a finite total
spin of the ground state is obtained by substituting one Cr(III) ion (s = 3/2)
with Zn (s = 0), Mn (s = 5/2) or Ni (s = 1) di-cations. Energy and intensity
measurements for several intra-multiplet and inter-multiplet magnetic
excitations allow us to determine the spin wavefunctions of the investigated
clusters. Effects due to the mixing of different spin multiplets have been
considered. Such effects proved to be important to correctly reproduce the
energy and intensity of magnetic excitations in the neutron spectra. On the
contrary to what is observed for the parent homonuclear Cr8 ring, the symmetry
of the first excited spin states is such that anticrossing conditions with the
ground state can be realized in the presence of an external magnetic field.
Heterometallic Cr7M wheels are therefore good candidates for macroscopic
observations of quantum effects.Comment: 9 pages, 11 figures, submitted to Phys. Rev. B, corrected typos and
added references, one sentence change
A chi-squared time-frequency discriminator for gravitational wave detection
Searches for known waveforms in gravitational wave detector data are often
done using matched filtering. When used on real instrumental data, matched
filtering often does not perform as well as might be expected, because
non-stationary and non-Gaussian detector noise produces large spurious filter
outputs (events). This paper describes a chi-squared time-frequency test which
is one way to discriminate such spurious events from the events that would be
produced by genuine signals. The method works well only for broad-band signals.
The case where the filter template does not exactly match the signal waveform
is also considered, and upper bounds are found for the expected value of
chi-squared.Comment: 18 pages, five figures, RevTex
Bound states and field-polarized Haldane modes in a quantum spin ladder
The challenge of one-dimensional systems is to understand their physics
beyond the level of known elementary excitations. By high-resolution neutron
spectroscopy in a quantum spin ladder material, we probe the leading
multiparticle excitation by characterizing the two-magnon bound state at zero
field. By applying high magnetic fields, we create and select the singlet
(longitudinal) and triplet (transverse) excitations of the fully spin-polarized
ladder, which have not been observed previously and are close analogs of the
modes anticipated in a polarized Haldane chain. Theoretical modelling of the
dynamical response demonstrates our complete quantitative understanding of
these states.Comment: 6 pages, 3 figures plus supplementary material 7 pages 5 figure
Continuous niobium phosphate catalysed Skraup reaction for quinoline synthesis from solketal
Solketal is derived from the reaction of acetone with glycerol, a by-product product of the biodiesel industry. We report here the continuous reaction of solketal with anilines over a solid acid niobium phosphate (NbP), for the continuous generation of quinolines in the the well-established Skraup reaction. This study shows that NbP can catalyse all stages of this multistep reaction at 250 °C and 10 MPa pressure, with a selectivity for quinoline of up to 60%. We found that the catalyst eventually deactivates, most probably via a combination of coking and reduction processes but nevertheless we show the promise of this approach. We demonstrated here the application of our approach to synthesize both mono- and bis-quinolines from the commodity chemical, 4,4’-methylenedianiline
Channeling and Volume Reflection Based Crystal Collimation of Tevatron Circulating Beam Halo (T-980)
The T980 crystal collimation experiment is underway at the Tevatron to
determine if this technique could increase 980 GeV beam-halo collimation
efficiency at high-energy hadron colliders such as the Tevatron and the LHC.
T980 also studies various crystal types and parameters. The setup has been
substantially enhanced during the Summer 2009 shutdown by installing a new
O-shaped crystal in the horizontal goniometer, as well as adding a vertical
goniometer with two alternating crystals (O-shaped and multi-strip) and
additional beam diagnostics. First measurements with the new system are quite
encouraging, with channeled and volume-reflected beams observed on the
secondary collimators as predicted. Investigation of crystal collimation
efficiencies with crystals in volume reflection and channeling modes are
described in comparison with an amorphous primary collimator. Results on the
system performance are presented for the end-of-store studies and for entire
collider stores. The first investigation of colliding beam collimation
simultaneously using crystals in both the vertical and horizontal plane has
been made in the regime with horizontally channeled and vertically
volume-reflected beams. Planning is underway for significant hardware
improvements during the FY10 summer shutdown and for dedicated studies during
the final year of Tevatron operation and also for a "post-collider beam physics
running" period.Comment: 3 pp. 1st International Particle Accelerator Conference: IPAC'10,
23-28 May 2010: Kyoto, Japa
Crystal experiments on efficient beam extraction
Silicon crystal was channeling and extracting 70-GeV protons from the U-70
accelerator with efficiency of 85.3+-2.8% as measured for a beam of 10^12
protons directed towards crystals of 2 mm length in spills of 1-2 s duration.
The experimental data follow very well the prediction of Monte Carlo
simulations. This success is important to devise a more efficient use of the
U-70 accelerator in Protvino and provides a crucial support for implementation
of crystal-assisted collimation of gold ion beam in RHIC and slow extraction
from AGS onto E952, now in preparation at Brookhaven Nat'l Lab. Future
applications, spanning in the energy from sub-GeV (medical) to order of 1 GeV
(scraping in the SNS, extraction from COSY) to order of 1 TeV and beyond
(scraping in the Tevatron, LHC, VLHC), can benefit from these studies.Comment: 12pp. Presented at 19-th Intern. Conference on Atomic Collisions in
Solids (ICACS-19: Paris, July 29 - August 3, 2001
Progress in crystal extraction and collimation
Recent IHEP Protvino experiments show efficiencies of crystal-assisted slow
extraction and collimation of 85.3+-2.8%, at the intensities of the channeled
beam on the order of 10^12 proton per spill of 2 s duration. The obtained
experimental data well follows the theory predictions. We compare the
measurements against theory and outline the theoretical potential for further
improvement in the efficiency of the technique. This success is important for
the efficient use of IHEP accelerator and for implementation of
crystal-assisted collimation at RHIC and slow extraction from AGS onto E952,
now in preparation. Future applications, spanning in the energy from order of 1
GeV (scraping in SNS, slow extraction from COSY and medical accelerators) to
order of 1 TeV and beyond (scraping in Tevatron, LHC, VLHC), can benefit from
these studies.Comment: 7pp. Presented at HEACC 2001 (Tsukuba, March 25-30
Isavuconazole for the treatment of fungal infections: a real-life experience from the Fungal Infection Network of Switzerland (FUNGINOS)
This analysis of 116 isavuconazole therapy courses shows that hepatic test disturbances (HTD) were relatively frequent (29% cases), but rarely led to treatment interruption (5%). Importantly, patients with baseline HTD, including those attributed to a first-line triazole, did not exhibit a higher risk of subsequent HTD under isavuconazole therapy
Topological triplon modes and bound states in a Shastry–Sutherland magnet
The twin discoveries of the quantum Hall effect, in the 1980's, and of
topological band insulators, in the 2000's, were landmarks in physics that
enriched our view of the electronic properties of solids. In a nutshell, these
discoveries have taught us that quantum mechanical wavefunctions in crystalline
solids may carry nontrivial topological invariants which have ramifications for
the observable physics. One of the side effects of the recent topological
insulator revolution has been that such physics is much more widespread than
was appreciated ten years ago. For example, while topological insulators were
originally studied in the context of electron wavefunctions, recent work has
led to proposals of topological insulators in bosonic systems: in photonic
crystals, in the vibrational modes of crystals, and in the excitations of
ordered magnets. Here we confirm the recent proposal that, in a weak magnetic
field, the dimerized quantum magnet SrCu(BO) is a bosonic
topological insulator with nonzero Chern number in the triplon bands and
topologically protected chiral edge excitations.Comment: 33 pages, 14 figures (preprint format and including supplementary
material
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