Haze and light diffraction of dielectric line-gratings

The optical characterization of dielectric periodic line-gratings for which the period of the grating is significantly larger than the probing wavelength is investigated experimentally, numerically, and analytically. The experimental diffraction efficiencies are analyzed in transmission with the help of a closed-form approximate solution within a single scattering picture. In particular, the angular width of significant scattering and the haze are analyzed for samples of increasing grating profile amplitude.Comment: 13 pages, 9 figure

Generation of high purity microwave signal from a dual-frequency OP-VECSEL (orale)

International audienceCoherent population trapping (CPT) is an interesting technique for the development of compact atomic frequency references. We describe an innovating laser source for the production of the two cross-polarized coherent laser fields which are necessary in CPT-based atomic clocks. It relies on the dual-frequency and dual-polarization operation of an optically-pumped vertical external-cavity semiconductor laser. This particular laser emission is induced by intracavity birefringent components which produce a controllable phase anisotropy within the laser cavity and force emission on two cross-polarized longitudinal modes. The laser emission is tuned at the Cs D2 line (λ = 852.14 nm), and the frequency difference ∆ν between the two laser modes is tunable in the microwave range. The laser line wavelength is stabilized onto an atomic hyperfine transition, and concurrently the frequency difference is locked to an ultra-low noise RF oscillator at 9.2 GHz. The high spectral purity of the optically-carried microwave signal resulting from the beatnote of the two cross-polarized laser lines is assessed through its narrow spectral linewidth (<30 Hz) as well as its low phase noise (≤ -100 dBrad2/Hz). The performance of this laser source is already adequate for the interrogation of atoms in a CPT atomic clock, and should result in an estimated relative stability of 3.10-13τ-1/2 - one order of magnitude better than commercial atomic clocks

Low-noise dual-frequency laser for compact Cs atomic clocks

International audienceWe report the dual-frequency and dual-polarization emission of an optically-pumped vertical external-cavity semiconductor laser (OP-VECSEL). Our laser source provides a high-purity optically-carried RF signal tunable in the GHz range, and is specifically designed for the coherent population trapping (CPT) of Cs atoms in compact atomic clocks. The laser spectrum is stabilized onto a Cs atomic transition at 852.1 nm, and the frequency difference is locked to a local oscillator at 9.2 GHz. Special attention has been paid to the evaluation of the frequency, intensity and phase noise properties. A maximum phase noise of - 90 dBrad2/Hz has been measured. Finally, we estimate the contribution of the laser noise on the short-term frequency stability of a CPT atomic clock, and predict that a value below 3 × 10-13 over one second is a realistic target

High-purity microwave signal from a dual-frequency semiconductor laser for CPT atomic clocks (poster)

Coherent population trapping (CPT) of metal-alkali atoms is an interesting technique for the development of compact atomic frequency references; it relies on the excitation of the atoms by two phase-coherent laser fields. We describe the design and operation of an innovating dual-frequency laser source dedicated to Cs CPT atomic clocks, based on the direct dual-frequency and dual-polarization operation of an optically-pumped semiconductor laser at 852 nm. The phase noise of beatnote generated by the laser source is at maximum of -90 dBrad²/Hz with active stabilization, and the relative intensity noise (RIN) has been measured at -115 dB/Hz. It would potentially results in a clock frequency stability of 1.6 .10^-12 at 1 second, limited by the laser RIN. With proper adjustments in the laser and clock set-up, we target a stability of 3.10^-13 at 1 second

Les phénomènes lies aux polarisation et gain dans micro-lasers en polymère dopes par colorant organique

The demonstration of an electrically pumped organic laser remains a major issue of organic optoelectronics for several decades. This goal requires an improved device configuration so as to reduce losses which are intrinsically higher under electrical excitation compared to optical pumping. Moreover a systematic investigation of the material properties is still missing and should lead to a reliable estimate of the lasing threshold under optical pumping, and then to a lower limit for electrical pumping. In this thesis we addressed the issue of gain and polarization properties of organic materials in the case of dye-doped polymer thin films. The originality of this work lies in the study of materials via the features of dielectric micro-lasers, allowing to investigate the issues of gain and mode coupling and the physics of open systems. We propose a quantitative description of amplification in organic materials. The "gain-loss-threshold" relation was developed and demonstrated for a Fabry- Perot type cavity, opening the way to study both amplification in organic materials and light out-coupling in dielectric micro-cavities via the lasing threshold. Within this context, different cavity shapes were studied, for instance squares, where light out-coupling takes place by diffraction at dielectric corners. We evidence that polarization properties of such lasing system originate from the intrinsic fluorescence anisotropy of dyes, which required to develop a specific anisotropic model going beyond the existing theory. We also investigated the role of the cavity geometry on the polarization states of the micro-lasers and proposed different ways to influence these features.La démonstration de la première diode laser organique reste un défi majeur en optoélectronique organique. Parmi les nombreuses problématiques à étudier, l'aspect " matériau " (gain et pertes) est capital. Par exemple, la limite théorique basse du seuil laser en pompage électrique pourrait être connue s'il existait une méthode d'estimation fiable du seuil laser en pompage optique. Dans cette thèse nous avons étudié le gain et la polarisation de lasers basés sur des couches minces de polymère dopées par des colorants organiques. L'originalité de ce travail repose sur l'étude des propriétés du matériau organique à travers l'analyse des caractéristiques de microlasers. Cela permet aussi de s'intéresser aux problématiques de couplage gain-mode et aux systèmes ouverts. Nous proposons une description quantitative du processus d'amplification dans les matériaux organiques. Une relation liant gain, pertes et seuil est établie dans le cas d'une cavité Fabry-Perot, ce qui permet par la suite l'étude de l'amplification optique et de l'extraction de la lumière dans les cavités diélectriques à travers la mesure précise du seuil laser. Nous avons exploré différentes formes de cavités, comme les carrés où la lumière est couplée vers l'extérieur par diffraction au niveau des coins. Nous avons démontré que l'anisotropie de fluorescence intrinsèque des molécules de colorant gouverne la polarisation de tels systèmes lasers. Nous avons développé à cette occasion un modèle original incluant la distribution non-isotrope des molécules dans le polymère. Nous avons aussi étudié le rôle de la géométrie de la cavité sur l'état de polarisation du laser, et différents moyens de contrôler cet état

Phénomènes liés à la polarisation et au gain dans des micro-lasers en polymère dopé par des colorants organiques

The demonstration of an electrically pumped organic laser remains a major issue of organic optoelectronics for several decades. This goal requires an improved device configuration so as to reduce losses which are intrinsically higher under electrical excitation compared to optical pumping. Moreover a systematic investigation of the material properties is still missing and should lead to a reliable estimate of the lasing threshold under optical pumping, and then to a lower limit for electrical pumping. In this thesis we addressed the issue of gain and polarization properties of organic materials in the case of dye-doped polymer thin films. The originality of this work lies in the study of materials via the features of dielectric micro-lasers, allowing to investigate the issues of gain and mode coupling and the physics of open systems. We propose a quantitative description of amplification in organic materials. The “gain-loss-threshold” relation was developed and demonstrated for a Fabry-Perot type cavity, opening the way to study both amplification in organic materials and light out-coupling in dielectric micro-cavities via the lasing threshold. Within this context, different cavity shapes were studied, for instance squares, where light out-coupling takes place by diffraction at dielectric corners. We evidence that polarization properties of such lasing system originate from the intrinsic fluorescence anisotropy of dyes, which required to develop a specific anisotropic model going beyond the existing theory. We also investigated the role of the cavity geometry on the polarization states of the micro-lasers and proposed different ways to influence these features.La démonstration de la première diode laser organique reste un défi majeur en opto-électronique organique. Parmi les nombreuses problématiques à étudier, l’aspect « matériau » (gain et pertes) est capital. Par exemple, la limite théorique basse du seuil laser en pompage électrique pourrait être connue s’il existait une méthode d’estimation fiable du seuil laser en pompage optique. Dans cette thèse nous avons étudié le gain et la polarisation de lasers basés sur des couches minces de polymère dopées par des colorants organiques. L’originalité de ce travail repose sur l’étude des propriétés du matériau organique à travers l’analyse des caractéristiques de microlasers. Cela permet aussi de s’intéresser aux problématiques de couplage gain-mode et aux systèmes ouverts. Nous proposons une description quantitative du processus d’amplification dans les matériaux organiques. Une relation liant gain, pertes et seuil est établie dans le cas d’une cavité Fabry-Perot, ce qui permet par la suite l’étude de l’amplification optique et de l’extraction de la lumière dans les cavités diélectriques à travers la mesure précise du seuil laser. Nous avons exploré différentes formes de cavités, comme les carrés où la lumière est couplée vers l’extérieur par diffraction au niveau des coins. Nous avons démontré que l’anisotropie de fluorescence intrinsèque des molécules de colorant gouverne la polarisation de tels systèmes lasers. Nous avons développé à cette occasion un modèle original incluant la distribution non-isotrope des molécules dans le polymère. Nous avons aussi étudié le rôle de la géométrie de la cavité sur l’état de polarisation du laser, et différents moyens de contrôler cet état

Plasma emission correction in reflectivity spectroscopy during sputtering deposition

International audienceSurface differential reflectivity spectroscopy is a fast non-destructive in situ and real-time measurement technique which allows following the first stages of thin film deposition. However, when applied to sputtering technique, spectra can strongly be distorted by residual light coming from plasma in a way, as shown herein, that depends on sample reflectivity. Thanks to suitable measurements, before and after growth with and without plasma or illumination lights, a protocol of signal correction is proposed to get rid of the spurious plasma contribution. The interest of the method is illustrated in the case of silver deposition on a silicon substrate

Experimental studies of the transmission of light through low-coverage regular or random arrays of silica micropillars supported by a glass substrate

International audienc

Gestion de la thermique dans les structures actives des lasers vecsels à 850 NM (Orale)

National audienceL'échauffement des structures actives semiconductrices dans les lasers VECSELs constitue une forte limitation à l'émission de puissances élevées. Nous évaluons théoriquement et expérimentalement les effets thermiques dans ces composants, et mettons en œuvre une technologie de report sur substrat Au développée pour améliorer leur résistance thermique

Periodic Arrays of Diamond‐Shaped Silver Nanoparticles: From Scalable Fabrication by Template‐Assisted Solid‐State Dewetting to Tunable Optical Properties

International audiencePeriodic arrays of anisotropic silver nanoparticles having peculiar optical properties are fabricated at a macroscopic scale. The proposed scalable method is based on temperature‐assisted solid‐state dewetting of a continuous thin layer deposited on a silica substrate patterned by the nanoimprint technique. The resulting nanoparticles are shaped like diamonds and are half‐embedded into the patterned silica. A period‐dependent optimum in film thickness for the quality of spatial organization is found and discussed in terms of thermodynamics and, for the first time, in terms of the role of grains in the dewetting process. The optical properties of the arrays are driven by not only simply the particle shape but also the lattice period and the degree of order. A surface lattice resonance that disperses with the underlying period is evidenced experimentally and confirmed by optical simulations. The opportunity to fabricate and tune such an assembly of plasmonic particles on transparent substrate opens interesting perspectives for not only fundamental photonics but also potential optical applications