Synthesis and Properties of Dipyridylcyclopentenes

A short and general route to the substituted dipyridylcyclopentenes was explored and several new compounds belonging to this new group of diarylethenes were synthesized. The study of their photochromic and thermochromic properties shows that the rate of the thermal ring opening is strongly dependent on the polarity of the solvent.

Soliton dual comb in crystalline microresonators

We present a novel compact dual-comb source based on a monolithic optical crystalline MgF$_2$ multi-resonator stack. The coherent soliton combs generated in two microresonators of the stack with the repetition rate of 12.1 GHz and difference of 1.62 MHz provided after heterodyning a 300 MHz wide radio-frequency comb. Analogous system can be used for dual-comb spectroscopy, coherent LIDAR applications and massively parallel optical communications.Comment: 5 pages, 5 figure

Frequency Comb Assisted Diode Laser Spectroscopy for Measurement of Microcavity Dispersion

While being invented for precision measurement of single atomic transitions, frequency combs have also become a versatile tool for broadband spectroscopy in the last years. In this paper we present a novel and simple approach for broadband spectroscopy, combining the accuracy of an optical fiber-laser-based frequency comb with the ease-of-use of a tunable external cavity diode laser. This scheme enables broadband and fast spectroscopy of microresonator modes and allows for precise measurements of their dispersion, which is an important precondition for broadband optical frequency comb generation that has recently been demonstrated in these devices. Moreover, we find excellent agreement of measured microresonator dispersion with predicted values from finite element simulations and we show that tailoring microresonator dispersion can be achieved by adjusting their geometrical properties

Measuring nanomechanical motion with an imprecision far below the standard quantum limit

We demonstrate a transducer of nanomechanical motion based on cavity enhanced optical near-fields capable of achieving a shot-noise limited imprecision more than 10 dB below the standard quantum limit (SQL). Residual background due to fundamental thermodynamical frequency fluctuations allows a total imprecision 3 dB below the SQL at room temperature (corresponding to 600 am/Hz^(1/2) in absolute units) and is known to reduce to negligible values for moderate cryogenic temperatures. The transducer operates deeply in the quantum backaction dominated regime, prerequisite for exploring quantum backaction, measurement-induced squeezing and accessing sub-SQL sensitivity using backaction evading techniques

Cavity optomechanics with Si3N4 membranes at cryogenic temperatures

We describe a cryogenic cavity-optomechanical system that combines Si3N4 membranes with a mechanically-rigid Fabry-Perot cavity. The extremely high quality-factor frequency products of the membranes allow us to cool a MHz mechanical mode to a phonon occupation of less than 10, starting at a bath temperature of 5 kelvin. We show that even at cold temperatures thermally-occupied mechanical modes of the cavity elements can be a limitation, and we discuss methods to reduce these effects sufficiently to achieve ground state cooling. This promising new platform should have versatile uses for hybrid devices and searches for radiation pressure shot noise.Comment: 19 pages, 5 figures, submitted to New Journal of Physic

Determination of the vacuum optomechanical coupling rate using frequency noise calibration

The strength of optomechanical interactions in a cavity optomechanical system can be quantified by a vacuum coupling rate \vcr analogous to cavity quantum electrodynamics. This single figure of merit removes the ambiguity in the frequently quoted coupling parameter defining the frequency shift for a given mechanical displacement, and the effective mass of the mechanical mode. Here we demonstrate and verify a straightforward experimental technique to derive the vacuum optomechanical coupling rate. It only requires applying a known frequency modulation of the employed electromagnetic probe field and knowledge of the mechanical oscillator's occupation. The method is experimentally verified for a micromechanical mode in a toroidal whispering-gallery-resonator and a nanomechanical oscillator coupled to a toroidal cavity via its near field.Comment: 11 pages, 2 figure